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Title: Interplay of screening and superconductivity in low-dimensional materials

Abstract

A quantitative description of Coulomb interactions is developed for two-dimensional superconducting materials, enabling us to compare intrinsic with external screening effects, such as those due to substrates. Therefore, using the example of a doped monolayer of MoS2 embedded in a tunable dielectric environment, we demonstrate that the influence of external screening is limited to a length scale, bounded from below by the effective thickness of the quasi-two-dimensional material and from above by its intrinsic screening length. As a consequence, it is found that unconventional Coulomb-driven superconductivity cannot be induced in MoS2 by tuning the substrate properties alone. Our calculations of the retarded Morel-Anderson Coulomb potential μ* reveal that the Coulomb interactions, renormalized by the reduced layer thickness and the substrate properties, can shift the onset of the electron-phonon driven superconducting phase in monolayer MoS2 but do not significantly affect the critical temperature at optimal doping.

Authors:
 [1];  [1];  [2];  [2];  [1]
  1. Univ. of Bremen (Germany). Inst. fuer Theoretische Physik; Univ. of Bremen (Germany). Bremen Center for Computational Materials Science
  2. Univ. of Southern California, Los Angeles, CA (United States)
Publication Date:
Research Org.:
Univ. of Southern California, Los Angeles, CA (United States)
Sponsoring Org.:
USDOE Office of Science (SC)
OSTI Identifier:
1535772
Alternate Identifier(s):
OSTI ID: 1328518
Grant/Contract Number:  
FG02-05ER46240
Resource Type:
Accepted Manuscript
Journal Name:
Physical Review. B
Additional Journal Information:
Journal Volume: 94; Journal Issue: 13; Journal ID: ISSN 2469-9950
Publisher:
American Physical Society (APS)
Country of Publication:
United States
Language:
English
Subject:
75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND SUPERFLUIDITY; Electron-phonon coupling; electronic structure; superconductivity; transition temperature; 2-dimensional systems; doped semiconductors; heterostructures; transition-metal dichalcogenide; density functional calculations; Eliashberg theory; GW method; methods in superconductivity

Citation Formats

Schönhoff, G., Rösner, M., Groenewald, R. E., Haas, S., and Wehling, T. O. Interplay of screening and superconductivity in low-dimensional materials. United States: N. p., 2016. Web. doi:10.1103/physrevb.94.134504.
Schönhoff, G., Rösner, M., Groenewald, R. E., Haas, S., & Wehling, T. O. Interplay of screening and superconductivity in low-dimensional materials. United States. https://doi.org/10.1103/physrevb.94.134504
Schönhoff, G., Rösner, M., Groenewald, R. E., Haas, S., and Wehling, T. O. Wed . "Interplay of screening and superconductivity in low-dimensional materials". United States. https://doi.org/10.1103/physrevb.94.134504. https://www.osti.gov/servlets/purl/1535772.
@article{osti_1535772,
title = {Interplay of screening and superconductivity in low-dimensional materials},
author = {Schönhoff, G. and Rösner, M. and Groenewald, R. E. and Haas, S. and Wehling, T. O.},
abstractNote = {A quantitative description of Coulomb interactions is developed for two-dimensional superconducting materials, enabling us to compare intrinsic with external screening effects, such as those due to substrates. Therefore, using the example of a doped monolayer of MoS2 embedded in a tunable dielectric environment, we demonstrate that the influence of external screening is limited to a length scale, bounded from below by the effective thickness of the quasi-two-dimensional material and from above by its intrinsic screening length. As a consequence, it is found that unconventional Coulomb-driven superconductivity cannot be induced in MoS2 by tuning the substrate properties alone. Our calculations of the retarded Morel-Anderson Coulomb potential μ* reveal that the Coulomb interactions, renormalized by the reduced layer thickness and the substrate properties, can shift the onset of the electron-phonon driven superconducting phase in monolayer MoS2 but do not significantly affect the critical temperature at optimal doping.},
doi = {10.1103/physrevb.94.134504},
journal = {Physical Review. B},
number = 13,
volume = 94,
place = {United States},
year = {Wed Oct 05 00:00:00 EDT 2016},
month = {Wed Oct 05 00:00:00 EDT 2016}
}

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Cited by: 11 works
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Works referencing / citing this record:

Noninvasive control of excitons in two-dimensional materials
journal, July 2017