An Aqueous Symmetric Sodium-Ion Battery with NASICON-Structured Na3MnTi(PO4)3
Abstract
A symmetric sodium-ion battery with an aqueous electrolyte is demonstrated; it utilizes the NASICON-structured Na3MnTi(PO4)3 as both the anode and the cathode. The NASICON-structured Na3MnTi(PO4)3 possesses two electrochemically active transition metals with the redox couples of Ti4+/Ti3+ and Mn3+/Mn2+ working on the anode and cathode sides, respectively. The symmetric cell based on this bipolar electrode material exhibits a well-defined voltage plateau centered at about 1.4 V in an aqueous electrolyte with a stable cycle performance and superior rate capability. The advent of aqueous symmetric sodium-ion battery with high safety and low cost may provide a solution for large-scale stationary energy storage.
- Authors:
-
- Univ. of Texas, Austin, TX (United States). Texas Materials Inst.
- Publication Date:
- Research Org.:
- Univ. of Texas, Austin, TX (United States)
- Sponsoring Org.:
- USDOE Office of Science (SC), Basic Energy Sciences (BES)
- OSTI Identifier:
- 1533083
- Grant/Contract Number:
- SC0005397
- Resource Type:
- Accepted Manuscript
- Journal Name:
- Angewandte Chemie (International Edition)
- Additional Journal Information:
- Journal Name: Angewandte Chemie (International Edition); Journal Volume: 55; Journal Issue: 41; Journal ID: ISSN 1433-7851
- Publisher:
- Wiley
- Country of Publication:
- United States
- Language:
- English
- Subject:
- 37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CHEMISTRY; 25 ENERGY STORAGE; aqueous electrolyte; energy storage; sodium-ion battery; symmetric battery
Citation Formats
Gao, Hongcai, and Goodenough, John B. An Aqueous Symmetric Sodium-Ion Battery with NASICON-Structured Na3MnTi(PO4)3. United States: N. p., 2016.
Web. doi:10.1002/anie.201606508.
Gao, Hongcai, & Goodenough, John B. An Aqueous Symmetric Sodium-Ion Battery with NASICON-Structured Na3MnTi(PO4)3. United States. https://doi.org/10.1002/anie.201606508
Gao, Hongcai, and Goodenough, John B. Tue .
"An Aqueous Symmetric Sodium-Ion Battery with NASICON-Structured Na3MnTi(PO4)3". United States. https://doi.org/10.1002/anie.201606508. https://www.osti.gov/servlets/purl/1533083.
@article{osti_1533083,
title = {An Aqueous Symmetric Sodium-Ion Battery with NASICON-Structured Na3MnTi(PO4)3},
author = {Gao, Hongcai and Goodenough, John B.},
abstractNote = {A symmetric sodium-ion battery with an aqueous electrolyte is demonstrated; it utilizes the NASICON-structured Na3MnTi(PO4)3 as both the anode and the cathode. The NASICON-structured Na3MnTi(PO4)3 possesses two electrochemically active transition metals with the redox couples of Ti4+/Ti3+ and Mn3+/Mn2+ working on the anode and cathode sides, respectively. The symmetric cell based on this bipolar electrode material exhibits a well-defined voltage plateau centered at about 1.4 V in an aqueous electrolyte with a stable cycle performance and superior rate capability. The advent of aqueous symmetric sodium-ion battery with high safety and low cost may provide a solution for large-scale stationary energy storage.},
doi = {10.1002/anie.201606508},
journal = {Angewandte Chemie (International Edition)},
number = 41,
volume = 55,
place = {United States},
year = {Tue Sep 13 00:00:00 EDT 2016},
month = {Tue Sep 13 00:00:00 EDT 2016}
}
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In Situ SEM Observation of Structured Si/C Anodes Reactions in an Ionic-Liquid-Based Lithium-Ion Battery
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Electrospun NaVPO 4 F/C Nanofibers as Self-Standing Cathode Material for Ultralong Cycle Life Na-Ion Batteries
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Aqueous Batteries Operated at −50 °C
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Nanocrystal-Assembled Porous Na 3 MgTi(PO 4 ) 3 Aggregates as Highly Stable Anode for Aqueous Sodium-Ion Batteries
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Conversion Synthesis of Self‐Standing Potassium Zinc Hexacyanoferrate Arrays as Cathodes for High‐Voltage Flexible Aqueous Rechargeable Sodium‐Ion Batteries
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Sodium-ion batteries: present and future
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An ion-conducting SnS–SnS 2 hybrid coating for commercial activated carbons enabling their use as high performance anodes for sodium-ion batteries
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A Multi-Ion Strategy towards Rechargeable Sodium-Ion Full Batteries with High Working Voltage and Rate Capability
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An Abnormal 3.7 Volt O3-Type Sodium-Ion Battery Cathode
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A Hydrostable Cathode Material Based on the Layered P2@P3 Composite that Shows Redox Behavior for Copper in High-Rate and Long-Cycling Sodium-Ion Batteries
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In Situ SEM Observation of Structured Si/C Anodes Reactions in an Ionic-Liquid-Based Lithium-Ion Battery
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Electrolytes and Interphases in Sodium-Based Rechargeable Batteries : Recent Advances and Perspectives
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Electrolytes and Interphases in Sodium-Based Rechargeable Batteries: Recent Advances and Perspectives
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Intermixed Cation-Anion Aqueous Battery Based on an Extremely Fast and Long-Cycling Di-Block Bipyridinium-Naphthalene Diimide Oligomer
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An Efficient Evaluation of F-doped Polyanion Cathode Materials with Long Cycle Life for Na-Ion Batteries Applications
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