Ultrathin Two-dimensional Metallic Nanocrystals for Renewable Energy Electrocatalysis [Ultrathin Two-dimensional Metallic Nanocrystals for Heterogeneous Catalysis]
Abstract
Even since the discovery of exfoliated graphene, exponentially growing efforts have been devoted to the search of novel 2 dimensional (2D) nanomaterials with atomic thickness and the extension of their applications. Among the huge 2D materials family, ultrathin 2D metallic nanocrystals gain vast attentions due to the unique importance of transition metals to heterogeneous catalysis. Here, we review recent representative advances in ultrathin 2D metallic nanocrystals and their catalytic applications towards a variety of reactions, including the hydrogen generation, oxygen reduction/evolution, CO2 activation and small molecules oxidation/hydrogenation. Special focuses are placed in currently mechanical understanding of bottom-up fabrication of ultrathin 2D metallic nanocrystals, the establishment of their structure-performance relationship as well as the implication of their real applications in devices. Here, we also shed light on further structural modification of the ultrathin 2D metallic nanocrystals to achieve the optimized catalytic performance. At end of this review, we discuss the remaining challenges and future opportunities in this burgeoning research area.
- Authors:
-
[2];
- Peking Univ., Beijing (China)
- Brookhaven National Lab. (BNL), Upton, NY (United States)
- Peking Univ., Beijing (China); Qingdao Univ. of Science and Technology, Qingdao (China)
- Univ. of Virginia, Charlottesville, VA (United States)
- Publication Date:
- Research Org.:
- Brookhaven National Lab. (BNL), Upton, NY (United States)
- Sponsoring Org.:
- USDOE Office of Science (SC), Basic Energy Sciences (BES)
- OSTI Identifier:
- 1508104
- Report Number(s):
- BNL-211567-2019-JAAM
Journal ID: ISSN 1369-7021
- Grant/Contract Number:
- SC0012704
- Resource Type:
- Accepted Manuscript
- Journal Name:
- Materials Today
- Additional Journal Information:
- Journal Volume: 23; Journal ID: ISSN 1369-7021
- Publisher:
- Elsevier
- Country of Publication:
- United States
- Language:
- English
- Subject:
- 29 ENERGY PLANNING, POLICY AND ECONOMY; Nanostructure; 2D materials; Heterogeneous Catalysis
Citation Formats
Luo, Mingchuan, Su, Dong, Yang, Yong, Sun, Yingjun, Qin, Yingnan, Li, Chunji, Li, Yingjie, Li, Menggang, Zhang, Sen, and Guo, Shaojun. Ultrathin Two-dimensional Metallic Nanocrystals for Renewable Energy Electrocatalysis [Ultrathin Two-dimensional Metallic Nanocrystals for Heterogeneous Catalysis]. United States: N. p., 2018.
Web. doi:10.1016/j.mattod.2018.06.005.
Luo, Mingchuan, Su, Dong, Yang, Yong, Sun, Yingjun, Qin, Yingnan, Li, Chunji, Li, Yingjie, Li, Menggang, Zhang, Sen, & Guo, Shaojun. Ultrathin Two-dimensional Metallic Nanocrystals for Renewable Energy Electrocatalysis [Ultrathin Two-dimensional Metallic Nanocrystals for Heterogeneous Catalysis]. United States. https://doi.org/10.1016/j.mattod.2018.06.005
Luo, Mingchuan, Su, Dong, Yang, Yong, Sun, Yingjun, Qin, Yingnan, Li, Chunji, Li, Yingjie, Li, Menggang, Zhang, Sen, and Guo, Shaojun. Mon .
"Ultrathin Two-dimensional Metallic Nanocrystals for Renewable Energy Electrocatalysis [Ultrathin Two-dimensional Metallic Nanocrystals for Heterogeneous Catalysis]". United States. https://doi.org/10.1016/j.mattod.2018.06.005. https://www.osti.gov/servlets/purl/1508104.
@article{osti_1508104,
title = {Ultrathin Two-dimensional Metallic Nanocrystals for Renewable Energy Electrocatalysis [Ultrathin Two-dimensional Metallic Nanocrystals for Heterogeneous Catalysis]},
author = {Luo, Mingchuan and Su, Dong and Yang, Yong and Sun, Yingjun and Qin, Yingnan and Li, Chunji and Li, Yingjie and Li, Menggang and Zhang, Sen and Guo, Shaojun},
abstractNote = {Even since the discovery of exfoliated graphene, exponentially growing efforts have been devoted to the search of novel 2 dimensional (2D) nanomaterials with atomic thickness and the extension of their applications. Among the huge 2D materials family, ultrathin 2D metallic nanocrystals gain vast attentions due to the unique importance of transition metals to heterogeneous catalysis. Here, we review recent representative advances in ultrathin 2D metallic nanocrystals and their catalytic applications towards a variety of reactions, including the hydrogen generation, oxygen reduction/evolution, CO2 activation and small molecules oxidation/hydrogenation. Special focuses are placed in currently mechanical understanding of bottom-up fabrication of ultrathin 2D metallic nanocrystals, the establishment of their structure-performance relationship as well as the implication of their real applications in devices. Here, we also shed light on further structural modification of the ultrathin 2D metallic nanocrystals to achieve the optimized catalytic performance. At end of this review, we discuss the remaining challenges and future opportunities in this burgeoning research area.},
doi = {10.1016/j.mattod.2018.06.005},
journal = {Materials Today},
number = ,
volume = 23,
place = {United States},
year = {Mon Jul 30 00:00:00 EDT 2018},
month = {Mon Jul 30 00:00:00 EDT 2018}
}
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