DOE PAGES title logo U.S. Department of Energy
Office of Scientific and Technical Information

Title: Multiple generations of grain aggregation in different environments preceded solar system body formation

Journal Article · · Proceedings of the National Academy of Sciences of the United States of America
ORCiD logo [1];  [1];  [2];  [3];  [4];  [4];  [5];  [6];  [3]
  1. Univ. of Hawaii at Manoa, Honolulu, HI (United States). Hawaii Inst. of Geophysics and Planetology
  2. Lawrence Berkeley National Lab. (LBNL), Berkeley, CA (United States). Advanced Light Source (ALS)
  3. Univ. of Washington, Seattle, WA (United States). Dept. of Astronomy
  4. Lawrence Berkeley National Lab. (LBNL), Berkeley, CA (United States). National Center for Electron Microscopy, Molecular Foundry
  5. NASA Ames Research Center (ARC), Moffett Field, Mountain View, CA (United States)
  6. Washington Univ., St. Louis, MO (United States). Lab. for Space Sciences

The solar system formed from interstellar dust and gas in a molecular cloud. Astronomical observations show that typical interstellar dust consists of amorphous (a-) silicate and organic carbon. Bona fide physical samples for laboratory studies would yield unprecedented insight about solar system formation, but they were largely destroyed. The most likely repositories of surviving presolar dust are the least altered extraterrestrial materials, interplanetary dust particles (IDPs) with probable cometary origins. Cometary IDPs contain abundant submicron a-silicate grains called GEMS (glass with embedded metal and sulfides), believed to be carbon-free. Some have detectable isotopically anomalous a-silicate components from other stars, proving they are preserved dust inherited from the interstellar medium. However, it is debated whether the majority of GEMS predate the solar system or formed in the solar nebula by condensation of high-temperature (>1,300 K) gas. Here, we map IDP compositions with single nanometer-scale resolution and find that GEMS contain organic carbon. Mapping reveals two generations of grain aggregation, the key process in growth from dust grains to planetesimals, mediated by carbon. GEMS grains, some with a-silicate subgrains mantled by organic carbon, comprise the earliest generation of aggregates. These aggregates (and other grains) are encapsulated in lower-density organic carbon matrix, indicating a second generation of aggregation. Since this organic carbon thermally decomposes above ~450 K, GEMS cannot have accreted in the hot solar nebula, and formed, instead, in the cold presolar molecular cloud and/or outer protoplanetary disk. We suggest that GEMS are consistent with surviving interstellar dust, condensed in situ, and cycled through multiple molecular clouds.

Research Organization:
Lawrence Berkeley National Laboratory (LBNL), Berkeley, CA (United States)
Sponsoring Organization:
National Aeronautics and Space Administration (NASA); USDOE Office of Science (SC), Basic Energy Sciences (BES) (SC-22). Scientific User Facilities Division
Grant/Contract Number:
AC02-05CH11231
OSTI ID:
1506319
Journal Information:
Proceedings of the National Academy of Sciences of the United States of America, Journal Name: Proceedings of the National Academy of Sciences of the United States of America Journal Issue: 26 Vol. 115; ISSN 0027-8424
Publisher:
National Academy of Sciences, Washington, DC (United States)Copyright Statement
Country of Publication:
United States
Language:
English

References (61)

Study of nucleic acid metabolism in two astronauts journal January 1984
Identification of isotopically primitive interplanetary dust particles: A NanoSIMS isotopic imaging study journal May 2006
Transmission Electron Microscopy of CONCORDIA UltraCarbonaceous Antarctic MicroMeteorites (UCAMMs): Mineralogical properties journal January 2012
The stardust abundance in the local interstellar cloud at the birth of the Solar System journal August 2017
Cold condensation of dust in the ISM journal January 2014
Fluid-induced organic synthesis in the solar nebula recorded in extraterrestrial dust from meteorites journal October 2014
The size distribution of interstellar grains journal October 1977
Laboratory infrared transmission spectra of individual interplanetary dust particles from 2.5 to 25 microns journal April 1985
Condensation processes in astrophysical environments: The composition and structure of cometary grains journal November 2002
Organic Globules in the Tagish Lake Meteorite: Remnants of the Protosolar Disk journal December 2006
Chemically Anomalous, Preaccretionally Irradiated Grains in Interplanetary Dust from Comets journal August 1994
Flux and composition of interstellar dust at Saturn from Cassinis Cosmic Dust Analyzer journal April 2016
Organic Matter in Cosmic Dust journal May 2016
The absence of crystalline silicates in the diffuse interstellar medium text January 2004
Organic grain coatings in primitive interplanetary dust particles: Implications for grain sticking in the Solar Nebula journal October 2013
The Sticking Properties of Water Frost Produced under Various Ambient Conditions journal October 1997
The Core-Mantle Interstellar Dust Model book January 1996
The isotopic composition of cosmic rays journal January 1984
The nature, origin and modification of insoluble organic matter in chondrites, the major source of Earth’s C and N journal May 2017
The origin of organic matter in the solar system: evidence from the interplanetary dust particles journal December 2003
Identification of isotopically primitive interplanetary dust particles: A NanoSIMS isotopic imaging study journal May 2006
On the origins of GEMS grains journal September 2011
Transmission Electron Microscopy of CONCORDIA UltraCarbonaceous Antarctic MicroMeteorites (UCAMMs): Mineralogical properties journal January 2012
UltraCarbonaceous Antarctic micrometeorites, probing the Solar System beyond the nitrogen snow-line journal May 2013
Solubility and stability investigation of Titan aerosol analogs: New insight from NMR analysis journal April 2014
Interstellar dust modelling: Interfacing laboratory, theoretical and observational studies (The THEMIS model) journal August 2015
The stardust abundance in the local interstellar cloud at the birth of the Solar System journal August 2017
Cold condensation of dust in the ISM journal January 2014
Dust coagulation and fragmentation in molecular clouds: I. How collisions between dust aggregates alter the dust size distribution journal June 2009
The evolution of amorphous hydrocarbons in the ISM: dust modelling from a new vantage point journal October 2013
Mantle formation, coagulation, and the origin of cloud/core shine: II. Comparison with observations journal March 2016
IRAS 08572+3915: constraining the aromatic versus aliphatic content of interstellar HACs journal November 2006
Evolution of interstellar dust and stardust in the solar neighbourhood journal December 2007
Fluid-induced organic synthesis in the solar nebula recorded in extraterrestrial dust from meteorites journal October 2014
The size distribution of interstellar grains journal October 1977
Laboratory infrared transmission spectra of individual interplanetary dust particles from 2.5 to 25 microns journal April 1985
Electron energy loss spectra of polycyclic aromatic hydrocarbons journal June 1992
Combined infrared and analytical electron microscope studies of interplanetary dust particles journal August 1992
Grain destruction in shocks in the interstellar medium journal September 1994
A Point in Favor of the Superparamagnetic Grain Hypothesis journal December 1995
The Absence of Crystalline Silicates in the Diffuse Interstellar Medium journal July 2004
Cohesion of Amorphous Silica Spheres: Toward a Better Understanding of the Coagulation Growth of Silicate dust Aggregates journal October 2015
Spectropolarimetric constraints on the nature of interstellar grains journal February 2014
Condensation processes in astrophysical environments: The composition and structure of cometary grains journal November 2002
Experimental study of the degradation of polymers: Application to the origin of extended sources in cometary atmospheres journal April 2004
Isotopic and chemical variation of organic nanoglobules in primitive meteorites journal April 2013
Measuring the level of interstellar inheritance in the solar protoplanetary disk journal June 2017
Samples of Stars Beyond the Solar System: Silicate Grains in Interplanetary Dust journal February 2003
An Astronomical 2175 A Feature in Interplanetary Dust Particles journal January 2005
Organic Globules in the Tagish Lake Meteorite: Remnants of the Protosolar Disk journal December 2006
Organic Synthesis via Irradiation and Warming of Ice Grains in the Solar Nebula journal March 2012
Chemically Anomalous, Preaccretionally Irradiated Grains in Interplanetary Dust from Comets journal August 1994
An Infrared Spectral Match Between GEMS and Interstellar Grains journal September 1999
Flux and composition of interstellar dust at Saturn from Cassinis Cosmic Dust Analyzer journal April 2016
Organic Molecules in the Interstellar Medium, Comets, and Meteorites: A Voyage from Dark Clouds to the Early Earth journal September 2000
Interstellar Dust Grains journal September 2003
Organic Matter in Cosmic Dust journal May 2016
The physical and compositional properties of dust: what do we really know? conference June 2014
Iron: a key Element for Understanding the Origin and Evolution of Interstellar dust journal July 2016
Modeling dust Evolution in Galaxies with a Multiphase, Inhomogeneous ism journal November 2016
Organic grain coatings in primitive interplanetary dust particles: Implications for grain sticking in the Solar Nebula journal October 2013

Cited By (6)

Lifetimes of interstellar dust from cosmic ray exposure ages of presolar silicon carbide journal January 2020
Lifetimes of interstellar dust from cosmic ray exposure ages of presolar silicon carbide journal January 2020
Comparison of GEMS in interplanetary dust particles and GEMS-like objects in a Stardust impact track in aerogel journal August 2018
Refractory inclusions in carbonaceous chondrites: Records of early solar system processes journal June 2019
Measurement of the Oxidation State of Fe in the ISM Using X-Ray Absorption Spectroscopy journal February 2019
Lifetimes of interstellar dust from cosmic ray exposure ages of presolar silicon carbide text January 2020

Similar Records

Interstellar dust as the source of organic molecules in Comet Halley
Conference · Sun Jan 01 04:00:00 UTC 1989 · Advances in Space Research; (USA) · OSTI ID:5594591

On the provenance of GEMS, a quarter century post discovery
Journal Article · Tue Jul 05 00:00:00 UTC 2022 · Geochimica et Cosmochimica Acta · OSTI ID:1894641

Comment on "The shape and composition of interstellar silicate grains"
Journal Article · Thu Sep 27 04:00:00 UTC 2007 · Astronomy and Astrophysics · OSTI ID:943833