DOE PAGES title logo U.S. Department of Energy
Office of Scientific and Technical Information

Title: Electron- and proton-impact excitation of heliumlike uranium in relativistic collisions

Abstract

We have studied the $$K$$-shell excitation of He-like uranium ($$\textbf{U}^{90+}$$) in relativistic collisions with hydrogen and argon atoms. Performing measurements with different targets, as well as with different collision energies, enabled us to explore the proton- (nucleus-) impact excitation as well as the electron-impact excitation process for the heaviest He-like ion. The large fine-structure splitting in uranium allowed us to partially resolve excitation into different $$L$$-shell levels. State-of-the-art relativistic calculations which include excitation mechanisms due to the interaction with both protons (nucleus) and electrons are in good agreement with the experimental findings. Moreover, our experimental data clearly demonstrate the importance of including the generalized Breit interaction in the treatment of the electron-impact excitation process.

Authors:
; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; more »; ; ; ; ; ; ; ; ; ; ; « less
Publication Date:
Research Org.:
Los Alamos National Lab. (LANL), Los Alamos, NM (United States)
Sponsoring Org.:
USDOE National Nuclear Security Administration (NNSA)
OSTI Identifier:
1499210
Alternate Identifier(s):
OSTI ID: 1566111
Report Number(s):
LA-UR-18-31841
Journal ID: ISSN 2469-9926; PLRAAN; 032706
Grant/Contract Number:  
AC52-06NA25396; 89233218CNA000001
Resource Type:
Published Article
Journal Name:
Physical Review A
Additional Journal Information:
Journal Name: Physical Review A Journal Volume: 99 Journal Issue: 3; Journal ID: ISSN 2469-9926
Publisher:
American Physical Society
Country of Publication:
United States
Language:
English
Subject:
74 ATOMIC AND MOLECULAR PHYSICS

Citation Formats

Gumberidze, A., Thorn, D. B., Surzhykov, A., Fontes, C. J., Najjari, B., Voitkiv, A., Fritzsche, S., Banaś, D., Beyer, H. F., Chen, W., Grisenti, R. E., Hagmann, S., Hess, R., Hillenbrand, P. -M., Indelicato, P., Kozhuharov, C., Lestinsky, M., Märtin, R., Petridis, N., Popov, R. V., Schuch, R., Spillmann, U., Tashenov, S., Trotsenko, S., Warczak, A., Weber, G., Wen, W., Winters, D. F. A., Winters, N., Yin, Z., and Stöhlker, Th. Electron- and proton-impact excitation of heliumlike uranium in relativistic collisions. United States: N. p., 2019. Web. doi:10.1103/PhysRevA.99.032706.
Gumberidze, A., Thorn, D. B., Surzhykov, A., Fontes, C. J., Najjari, B., Voitkiv, A., Fritzsche, S., Banaś, D., Beyer, H. F., Chen, W., Grisenti, R. E., Hagmann, S., Hess, R., Hillenbrand, P. -M., Indelicato, P., Kozhuharov, C., Lestinsky, M., Märtin, R., Petridis, N., Popov, R. V., Schuch, R., Spillmann, U., Tashenov, S., Trotsenko, S., Warczak, A., Weber, G., Wen, W., Winters, D. F. A., Winters, N., Yin, Z., & Stöhlker, Th. Electron- and proton-impact excitation of heliumlike uranium in relativistic collisions. United States. https://doi.org/10.1103/PhysRevA.99.032706
Gumberidze, A., Thorn, D. B., Surzhykov, A., Fontes, C. J., Najjari, B., Voitkiv, A., Fritzsche, S., Banaś, D., Beyer, H. F., Chen, W., Grisenti, R. E., Hagmann, S., Hess, R., Hillenbrand, P. -M., Indelicato, P., Kozhuharov, C., Lestinsky, M., Märtin, R., Petridis, N., Popov, R. V., Schuch, R., Spillmann, U., Tashenov, S., Trotsenko, S., Warczak, A., Weber, G., Wen, W., Winters, D. F. A., Winters, N., Yin, Z., and Stöhlker, Th. Wed . "Electron- and proton-impact excitation of heliumlike uranium in relativistic collisions". United States. https://doi.org/10.1103/PhysRevA.99.032706.
@article{osti_1499210,
title = {Electron- and proton-impact excitation of heliumlike uranium in relativistic collisions},
author = {Gumberidze, A. and Thorn, D. B. and Surzhykov, A. and Fontes, C. J. and Najjari, B. and Voitkiv, A. and Fritzsche, S. and Banaś, D. and Beyer, H. F. and Chen, W. and Grisenti, R. E. and Hagmann, S. and Hess, R. and Hillenbrand, P. -M. and Indelicato, P. and Kozhuharov, C. and Lestinsky, M. and Märtin, R. and Petridis, N. and Popov, R. V. and Schuch, R. and Spillmann, U. and Tashenov, S. and Trotsenko, S. and Warczak, A. and Weber, G. and Wen, W. and Winters, D. F. A. and Winters, N. and Yin, Z. and Stöhlker, Th.},
abstractNote = {We have studied the $K$-shell excitation of He-like uranium ($\textbf{U}^{90+}$) in relativistic collisions with hydrogen and argon atoms. Performing measurements with different targets, as well as with different collision energies, enabled us to explore the proton- (nucleus-) impact excitation as well as the electron-impact excitation process for the heaviest He-like ion. The large fine-structure splitting in uranium allowed us to partially resolve excitation into different $L$-shell levels. State-of-the-art relativistic calculations which include excitation mechanisms due to the interaction with both protons (nucleus) and electrons are in good agreement with the experimental findings. Moreover, our experimental data clearly demonstrate the importance of including the generalized Breit interaction in the treatment of the electron-impact excitation process.},
doi = {10.1103/PhysRevA.99.032706},
journal = {Physical Review A},
number = 3,
volume = 99,
place = {United States},
year = {Wed Mar 13 00:00:00 EDT 2019},
month = {Wed Mar 13 00:00:00 EDT 2019}
}

Journal Article:
Free Publicly Available Full Text
Publisher's Version of Record
https://doi.org/10.1103/PhysRevA.99.032706

Citation Metrics:
Cited by: 7 works
Citation information provided by
Web of Science

Figures / Tables:

FIG. 1 FIG. 1: X-ray spectrum recorded for 218-MeV/u U90+ → H2 collisions with a Ge(i) detector at the observation angle of 60° with respect to the ion beam. The REC transitions into $L$, $M$, and higher shells are clearly visible together with the characteristic transitions into the $K$ shell.

Save / Share:

Works referenced in this record:

Low- internal target from a cryogenically cooled liquid microjet source
journal, April 2009

  • Kühnel, M.; Petridis, N.; Winters, D. F. A.
  • Nuclear Instruments and Methods in Physics Research Section A: Accelerators, Spectrometers, Detectors and Associated Equipment, Vol. 602, Issue 2
  • DOI: 10.1016/j.nima.2008.12.212

Electron loss from hydrogen-like highly charged ions in collisions with electrons, protons and light atoms
journal, February 2018

  • Lyashchenko, K. N.; Andreev, O. Yu; Voitkiv, A. B.
  • Journal of Physics B: Atomic, Molecular and Optical Physics, Vol. 51, Issue 5
  • DOI: 10.1088/1361-6455/aaaa11

Excitation of atomic hydrogen by protons and multiply charged ions at intermediate velocities
journal, September 1994

  • Detleffsen, D.; Anton, M.; Werner, A.
  • Journal of Physics B: Atomic, Molecular and Optical Physics, Vol. 27, Issue 18
  • DOI: 10.1088/0953-4075/27/18/017

Electron- and Proton-Impact Excitation of Hydrogenlike Uranium in Relativistic Collisions
journal, May 2013


Zero-degree Auger spectroscopy in energetic, highly charged ion-atom collisions
journal, April 1994


Polarization measurements of the Lyman- α 1 x-ray emission lines of hydrogenlike Ar 17 + and Fe 25 + at high electron-impact energies
journal, August 2006


Alignment of heavy few-electron ions following excitation by relativistic Coulomb collisions
journal, April 2008


Measurement of electron impact excitation cross sections for heliumlike titanium
journal, July 1992


Experimental Demonstration of the Breit Interaction which Dominates the Angular Distribution of X-ray Emission in Dielectronic Recombination
journal, February 2012


Electron impact excitation of hydrogenic ions. II
journal, April 1975


Simultaneous excitation and ionization of He-like uranium ions in relativistic collisions with gaseous targets
journal, April 2000


Relativistic convergent close-coupling method: Calculation of electron scattering from hydrogenlike ions
journal, November 2009


Use of the factorized form for the collision strength in exploration of the effect of the generalized Breit interaction
journal, May 1994

  • Fontes, Christopher J.; Sampson, Douglas H.; Zhang, Hong Lin
  • Physical Review A, Vol. 49, Issue 5
  • DOI: 10.1103/PhysRevA.49.3704

Electron-electron interaction in the ionization of O 7 + by He
journal, April 1997


Time-ordering effects in K -shell excitation of 170-MeV Ne 7 + colliding with gas atoms: Double excitation
journal, January 1995


Ground-state excitation of heavy highly-charged ions
journal, May 2015

  • Gumberidze, A.; Thorn, D. B.; Fontes, C. J.
  • Journal of Physics B: Atomic, Molecular and Optical Physics, Vol. 48, Issue 14
  • DOI: 10.1088/0953-4075/48/14/144006

Application of the Schwinger Principle to Direct Excitation of Atoms or Ions by Impact of Bare Nuclei at Intermediate Velocities
journal, May 1985


Relativistic electron- and proton-impact ionization of highly stripped heavy ions determined from projectile-electron loss in H 2 and He
journal, March 1993


Target nuclear charge dependence of 1s 2 to 1s2p and 1s 2 to 1s3p excitation cross sections of Fe 24+ projectiles in the intermediate velocity range
journal, July 1986

  • Wohrer, K.; Chetioui, A.; Rozet, J. P.
  • Journal of Physics B: Atomic and Molecular Physics, Vol. 19, Issue 13
  • DOI: 10.1088/0022-3700/19/13/011

Electron-electron interaction in projectile ionization investigated by high resolution recoil ion momentum spectroscopy
journal, May 1994


Population of He 4 1 D magnetic sublevels by collisions with protons and multiply charged ions in the intermediate velocity range
journal, July 1993

  • Anton, M.; Detleffsen, D.; Schartner, K. -H
  • Journal of Physics B: Atomic, Molecular and Optical Physics, Vol. 26, Issue 13
  • DOI: 10.1088/0953-4075/26/13/021

Shell- and subshell-resolved projectile excitation of hydrogenlike Au 78 + ions in relativistic ion-atom collisions
journal, November 2010


K -shell excitation studied for H- and He-like bismuth ions in collisions with low- Z target atoms
journal, February 1998


Evidence for Strong Breit Interaction in Dielectronic Recombination of Highly Charged Heavy Ions
journal, February 2008


K α 1 radiation from heavy, heliumlike ions produced in relativistic collisions
journal, November 2006


Breit interaction in dielectronic recombination of hydrogenlike uranium
journal, February 2011


Magnetic-sublevel population and alignment for the excitation of H- and He-like uranium in relativistic collisions
journal, October 2011


Scaling relation for total excitation cross sections of He in collisions with highly charged ions
journal, September 1988


Inclusion of the generalized Breit interaction in excitation of highly charged ions by electron impact
journal, February 1993

  • Fontes, Christopher J.; Sampson, Douglas H.; Zhang, Hong Lin
  • Physical Review A, Vol. 47, Issue 2
  • DOI: 10.1103/PhysRevA.47.1009

Electron-loss-to-continuum cusp in U 88 + + N 2 collisions
journal, October 2014


Excitation of Ar16+ projectiles in intermediate velocity collisions with neutrals
journal, May 1995

  • Adoui, L.; Vernhet, D.; Wohrer, K.
  • Nuclear Instruments and Methods in Physics Research Section B: Beam Interactions with Materials and Atoms, Vol. 98, Issue 1-4
  • DOI: 10.1016/0168-583X(95)00134-4

Radiative electron capture in relativistic ion–atom collisions and the photoelectric effect in hydrogen-like high-Z systems
journal, February 2007


Excitation of heavy hydrogenlike ions by light atoms in relativistic collisions with large momentum transfers
journal, May 2012


Electron-impact excitation cross-section measurements of highly charged heliumlike and lithiumlike ions
journal, February 1995


Excitation in swift heavy ion-atom collisions
journal, February 1996

  • Vernhet, D.; Rozet, J. P.; Wohrer, K.
  • Nuclear Instruments and Methods in Physics Research Section B: Beam Interactions with Materials and Atoms, Vol. 107, Issue 1-4
  • DOI: 10.1016/0168-583X(95)00807-1

Simultaneous Projectile-Target Ionization: A Novel Approach to ( e , 2 e ) Experiments on Ions
journal, February 2002


Energy loss and cooling of relativistic highly charged uranium ions interacting with an internal hydrogen droplet target beam
journal, November 2011

  • Petridis, N.; Kalinin, A.; Popp, U.
  • Nuclear Instruments and Methods in Physics Research Section A: Accelerators, Spectrometers, Detectors and Associated Equipment, Vol. 656, Issue 1
  • DOI: 10.1016/j.nima.2011.07.035

Works referencing / citing this record:

Zero-degree Auger spectroscopy in energetic, highly charged ion-atom collisions
journal, April 1994


Low- internal target from a cryogenically cooled liquid microjet source
journal, April 2009

  • Kühnel, M.; Petridis, N.; Winters, D. F. A.
  • Nuclear Instruments and Methods in Physics Research Section A: Accelerators, Spectrometers, Detectors and Associated Equipment, Vol. 602, Issue 2
  • DOI: 10.1016/j.nima.2008.12.212

Energy loss and cooling of relativistic highly charged uranium ions interacting with an internal hydrogen droplet target beam
journal, November 2011

  • Petridis, N.; Kalinin, A.; Popp, U.
  • Nuclear Instruments and Methods in Physics Research Section A: Accelerators, Spectrometers, Detectors and Associated Equipment, Vol. 656, Issue 1
  • DOI: 10.1016/j.nima.2011.07.035

Radiative electron capture in relativistic ion–atom collisions and the photoelectric effect in hydrogen-like high-Z systems
journal, February 2007


Target nuclear charge dependence of 1s 2 to 1s2p and 1s 2 to 1s3p excitation cross sections of Fe 24+ projectiles in the intermediate velocity range
journal, July 1986

  • Wohrer, K.; Chetioui, A.; Rozet, J. P.
  • Journal of Physics B: Atomic and Molecular Physics, Vol. 19, Issue 13
  • DOI: 10.1088/0022-3700/19/13/011

Electron impact excitation of hydrogenic ions. II
journal, April 1975


Population of He 4 1 D magnetic sublevels by collisions with protons and multiply charged ions in the intermediate velocity range
journal, July 1993

  • Anton, M.; Detleffsen, D.; Schartner, K. -H
  • Journal of Physics B: Atomic, Molecular and Optical Physics, Vol. 26, Issue 13
  • DOI: 10.1088/0953-4075/26/13/021

Excitation of atomic hydrogen by protons and multiply charged ions at intermediate velocities
journal, September 1994

  • Detleffsen, D.; Anton, M.; Werner, A.
  • Journal of Physics B: Atomic, Molecular and Optical Physics, Vol. 27, Issue 18
  • DOI: 10.1088/0953-4075/27/18/017

Ground-state excitation of heavy highly-charged ions
journal, May 2015

  • Gumberidze, A.; Thorn, D. B.; Fontes, C. J.
  • Journal of Physics B: Atomic, Molecular and Optical Physics, Vol. 48, Issue 14
  • DOI: 10.1088/0953-4075/48/14/144006

Electron loss from hydrogen-like highly charged ions in collisions with electrons, protons and light atoms
journal, February 2018

  • Lyashchenko, K. N.; Andreev, O. Yu; Voitkiv, A. B.
  • Journal of Physics B: Atomic, Molecular and Optical Physics, Vol. 51, Issue 5
  • DOI: 10.1088/1361-6455/aaaa11

Electron- and proton-impact excitation of heliumlike uranium in relativistic collisions
text, January 2019

  • Gumberidze, A.; Thorn, D. B.; Surzhykov, A.
  • GSI Helmholtzzentrum fuer Schwerionenforschung, GSI, Darmstadt
  • DOI: 10.15120/gsi-2019-00576

Dominance of the density effects in the magnetic sublevel population and circular polarization of x-ray radiation
journal, October 2019

  • Chen, Zhan-Bin
  • Journal of Physics B: Atomic, Molecular and Optical Physics, Vol. 52, Issue 21
  • DOI: 10.1088/1361-6455/ab3133

Local time dependence of the magnetic sublevel population and polarization of fluorescence radiation
journal, January 2019

  • Chen, Zhan-Bin
  • Journal of Physics B: Atomic, Molecular and Optical Physics, Vol. 53, Issue 1
  • DOI: 10.1088/1361-6455/ab5038

Figures/Tables have been extracted from DOE-funded journal article accepted manuscripts.