Colloquium : Superheavy elements: Oganesson and beyond

Giuliani, S. A.; Matheson, Z.; Nazarewicz, W.; Olsen, E.; Reinhard, P. -G.; Sadhukhan, J.; Schuetrumpf, B.; Schunck, N.; Schwerdtfeger, P.

doi:10.1103/RevModPhys.91.011001

Title: Colloquium : Superheavy elements: Oganesson and beyond

Abstract

During the last decade, six new superheavy elements were added into the seventh period of the periodic table, with the approval of their names and symbols. This milestone was followed by proclaiming 2019 the International Year of the Periodic Table of Chemical Elements by the United Nations General Assembly. According to theory, due to their large atomic numbers, the new arrivals are expected to be qualitatively and quantitatively different from lighter species. The questions pertaining to superheavy atoms and nuclei are in the forefront of research in nuclear and atomic physics and chemistry. This Colloquium offers a broad perspective on the field and outlines future challenges.

Authors:

Giuliani, S. A. ^[1]; Matheson, Z. ^[1]; Nazarewicz, W. ^[1]; Olsen, E. ^[1]; Reinhard, P. -G. ^[2]; Sadhukhan, J. ^[3]; Schuetrumpf, B. ^[4]; Schunck, N. ^[5]; Schwerdtfeger, P. ^[6]

Michigan State Univ., East Lansing, MI (United States). Dept. of of Physics and Astronomy and FRIB Lab.
Univ. Erlangen-Nürnberg, Erlangen (Germany). Inst. fur Theoretische Physik II
India and Homi Bhabha National Institute, Mumbai (India). Variable Energy Cyclotron Centre
GSI Helmholzzentrum für Schwerionenforschung, Darmstadt (Germany); Technische Univ. Darmstadt (Germany). Inst. fur Kernphysik
Lawrence Livermore National Lab. (LLNL), Livermore, CA (United States). Nuclear and Chemical Science Division
Massey Univ. Auckland, Auckland (New Zealand). Centre for Theoretical Chemistry and Physics, The New Zealand Inst. for Advanced Study

Publication Date:: Tue Jan 01 00:00:00 EST 2019

Research Org.:: Lawrence Livermore National Laboratory (LLNL), Livermore, CA (United States); Michigan State Univ., East Lansing, MI (United States)

Sponsoring Org.:: USDOE National Nuclear Security Administration (NNSA)

OSTI Identifier:: 1513128

Alternate Identifier(s):: OSTI ID: 1491614; OSTI ID: 1513815

Report Number(s):: LLNL-JRNL-757240
Journal ID: ISSN 0034-6861; RMPHAT; 944846

Grant/Contract Number:: AC52-07NA27344; NA0002847; SC0013365; SC0018083; NA0003885

Resource Type:: Accepted Manuscript

Journal Name:: Reviews of Modern Physics

Additional Journal Information:: Journal Volume: 91; Journal Issue: 1; Journal ID: ISSN 0034-6861

Publisher:: American Physical Society (APS)

Country of Publication:: United States

Language:: English

Subject:: 73 NUCLEAR PHYSICS AND RADIATION PHYSICS

Citation Formats


                    Giuliani, S. A., Matheson, Z., Nazarewicz, W., Olsen, E., Reinhard, P. -G., Sadhukhan, J., Schuetrumpf, B., Schunck, N., and Schwerdtfeger, P. Colloquium : Superheavy elements: Oganesson and beyond.  United States: N. p., 2019. 
Web.  doi:10.1103/RevModPhys.91.011001.

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                    Giuliani, S. A., Matheson, Z., Nazarewicz, W., Olsen, E., Reinhard, P. -G., Sadhukhan, J., Schuetrumpf, B., Schunck, N., & Schwerdtfeger, P. Colloquium : Superheavy elements: Oganesson and beyond.  United States.  https://doi.org/10.1103/RevModPhys.91.011001

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                    Giuliani, S. A., Matheson, Z., Nazarewicz, W., Olsen, E., Reinhard, P. -G., Sadhukhan, J., Schuetrumpf, B., Schunck, N., and Schwerdtfeger, P. Tue .  
"Colloquium : Superheavy elements: Oganesson and beyond".  United States.  https://doi.org/10.1103/RevModPhys.91.011001.  https://www.osti.gov/servlets/purl/1513128.

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@article{osti_1513128,

  title        = {Colloquium : Superheavy elements: Oganesson and beyond},

  author       = {Giuliani, S. A. and Matheson, Z. and Nazarewicz, W. and Olsen, E. and Reinhard, P. -G. and Sadhukhan, J. and Schuetrumpf, B. and Schunck, N. and Schwerdtfeger, P.},

  abstractNote = {During the last decade, six new superheavy elements were added into the seventh period of the periodic table, with the approval of their names and symbols. This milestone was followed by proclaiming 2019 the International Year of the Periodic Table of Chemical Elements by the United Nations General Assembly. According to theory, due to their large atomic numbers, the new arrivals are expected to be qualitatively and quantitatively different from lighter species. The questions pertaining to superheavy atoms and nuclei are in the forefront of research in nuclear and atomic physics and chemistry. This Colloquium offers a broad perspective on the field and outlines future challenges.},

  doi          = {10.1103/RevModPhys.91.011001},

  journal      = {Reviews of Modern Physics},

  number       = 1,

  volume       = 91,

  place        = {United States},

  year         = {Tue Jan 01 00:00:00 EST 2019},

  month        = {Tue Jan 01 00:00:00 EST 2019}

}

Copy to clipboard

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Works referencing / citing this record:

Oganesson ist ein Halbleiter: Über die relativitische Bandlückenkontraktion in den schwersten Edelgasen
journal, August 2019

Mewes, Jan‐Michael; Jerabek, Paul; Smits, Odile R.
Angewandte Chemie, Vol. 131, Issue 40
DOI: 10.1002/ange.201908327

Calculation of atomic properties of superheavy elements $Z = 110 - 112$ and their ions
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Lackenby, B. G. C.; Dzuba, V. A.; Flambaum, V. V.
Physical Review A, Vol. 101, Issue 1
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Time-dependent Hartree-Fock plus Langevin approach for hot fusion reactions to synthesize the $Z = 120$ superheavy element
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Sekizawa, K.; Hagino, K.
Physical Review C, Vol. 99, Issue 5
DOI: 10.1103/physrevc.99.051602

Exploring the chemical nature of super-heavy main-group elements by means of efficient plane-wave density-functional theory
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Trombach, Lukas; Ehlert, Sebastian; Grimme, Stefan
Physical Chemistry Chemical Physics, Vol. 21, Issue 33
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An essay on periodic tables
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Pyykkö, Pekka
Pure and Applied Chemistry, Vol. 91, Issue 12
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Rotational properties of nuclei around ${}^{254}{No}$ investigated using a spectroscopic-quality Skyrme energy density functional
journal, March 2014

The fission barriers in Actinides and superheavy nuclei in covariant density functional theory
journal, May 2010

Systematic study of cluster radioactivity of superheavy nuclei
journal, January 2018

The rotation–vibration spectrum of methyl fluoride from first principles
journal, January 2019

Relativistic Coupled Cluster Calculations with Variational Quantum Electrodynamics Resolve the Discrepancy between Experiment and Theory Concerning the Electron Affinity and Ionization Potential of Gold
journal, January 2017

Criteria that must be satisfied for the discovery of a new chemical element to be recognized
journal, January 1991

Equation of state for solid neon from quantum theory
journal, August 2009

Production cross sections of superheavy elements $Z = 119$ and 120 in hot fusion reactions
journal, February 2014

In situ synthesis of volatile carbonyl complexes with short-lived nuclides
journal, November 2014

Physical Conditions for the r -process. I. Radioactive Energy Sources of Kilonovae
journal, November 2018

First Direct Measurements of Superheavy-Element Mass Numbers
journal, November 2018

Theoretical justification of Madelung's rule
journal, November 1979

A Theoretical Study on the Adsorption Behavior of Element 113 and Its Homologue Tl on a Quartz Surface: Relativistic Periodic DFT Calculations
journal, September 2016

Finite nuclear charge density distributions in electronic structure calculations for atoms and molecules
journal, October 2000

Structure of Odd- N Superheavy Elements
journal, August 1999

Closed shells for Z > 82 and N > 126 in a diffuse potential well
journal, September 1966

Californium-254 and Kilonova Light Curves
journal, August 2018

Origin of the heavy elements in binary neutron-star mergers from a gravitational-wave event
journal, October 2017

How elements up to 118 were reached and how to go beyond
journal, January 2017

On search and identification of short-lived super heavy cosmic-ray nuclei (Z ≥ 110) by fossil track study of the extraterrestrial crystals: Results and perspectives [II]
journal, May 2003

Fission barriers and probabilities of spontaneous fission for elements with Z≥ 100
journal, December 2015

Mass spectrometric searches for superheavy elements in terrestrial matter
journal, December 2015

Superheavy Element Flerovium (Element 114) Is a Volatile Metal
journal, January 2014

Reaching the limits of nuclear stability
journal, June 2004

Synthesis of the heaviest nuclei in cold fusion reactions
journal, December 2015

Characterizing the mechanism(s) of heavy element synthesis reactions
journal, January 2016

Prospects of heavy and superheavy element production via inelastic nucleus-nucleus collisions – from ²³⁸ U + ²³⁸ U to ¹⁸ O + ²⁵⁴ Es
journal, January 2016

Decay and Fission Hindrance of Two- and Four-Quasiparticle $K$ Isomers in ${}^{254}{Rf}$
journal, September 2015

Chemistry of the 5g Elements: Relativistic Calculations on Hexafluorides
journal, April 2017

Prediction of the adsorption behavior of elements 112 and 114 on inert surfaces from ab initio Dirac-Coulomb atomic calculations
journal, January 2008

High Intensity heavy ion Accelerator Facility (HIAF) in China
journal, December 2013

Magic numbers of ultraheavy nuclei
journal, July 2005

Neutron-deficient superheavy nuclei obtained in the ${}^{240}{Pu} + {}^{48}{Ca}$ reaction
journal, January 2018

Theoretical predictions of adsorption behavior of elements 112 and 114 and their homologs Hg and Pb
journal, August 2009

[CLC][ITAL]r[/ITAL][/CLC]-Process in Neutron Star Mergers
journal, November 1999

Matter at Large Neutron Excess and the Physics of Neutron-Star Crusts
journal, December 1995

The Pseudopotential Approximation in Electronic Structure Theory
journal, August 2011

Dynamical mass ejection from binary neutron star mergers
journal, May 2016

Synthesis of the Elements in Stars
journal, October 1957

The chemistry of the superheavy elements. II. The stability of high oxidation states in group 11 elements: Relativistic coupled cluster calculations for the di-, tetra- and hexafluoro metallates of Cu, Ag, Au, and element 111
journal, September 1998

Microscopic description of fission in odd-mass uranium and plutonium nuclei with the Gogny energy density functional
journal, December 2017

Are elements 112, 114, and 118 relatively inert gases?
journal, July 1975

The R-process and nucleochronology
journal, November 1991

Predictions for the synthesis of superheavy elements $Z = 119$ and 120
journal, July 2018

A new kind of natural radioactivity
journal, January 1984

Quasifission Dynamics in the Formation of Superheavy Elements
journal, January 2017

Dependence of relativistic effects on electronic configuration in the neutral atoms of d- and f-block elements
journal, April 2002

Shell stabilization of super- and hyperheavy nuclei without magic gaps
journal, August 2001

Discovery of the elements with atomic numbers greater than or equal to 113 (IUPAC Technical Report)
journal, June 2011

Toroidal high-spin isomers in the nucleus ${}^{304}120$
journal, May 2017

$α$ decay and cluster radioactivity of nuclei of interest to the synthesis of $Z = 119$ , 120 isotopes
journal, April 2018

Relativistic effects in structural chemistry
journal, May 1988

Isotope shift and search for metastable superheavy elements in astrophysical data
journal, June 2017

Quadrupole collective inertia in nuclear fission: Cranking approximation
journal, November 2011

Theoretical Predictions of Properties and Chemical Behavior of Superheavy Elements
journal, January 2002

ORNL actinide materials and a new detection system for superheavy nuclei
journal, January 2016

$α$ decay of high- K isomers in ${}^{270}{Ds}$ and ${}^{266}{Hs}$ in a superfluid tunneling model
journal, February 2018

Fission properties for $r$ -process nuclei
journal, February 2012

The new isotope 270110 and its decay products 266Hs and 262Sg
journal, February 2001

Relativistic and quantum electrodynamic effects in superheavy elements
journal, December 2015

Relativistic Quantum Chemistry of the Superheavy Elements. Closed-Shell Element 114 as a Case Study.
journal, January 2002

The transcalifornium elements
journal, January 1959

Systematic study of $α$ -decay energies and half-lives of superheavy nuclei
journal, December 2015

The double-humped fission barrier
journal, October 1980

Recent α decay half-lives and analytic expression predictions including superheavy nuclei
journal, March 2008

Atomic structure calculations of superheavy noble element oganesson $(Z = 118)$
journal, October 2018

Bayesian approach to model-based extrapolation of nuclear observables
journal, September 2018

Octupole deformation in neutron-rich actinides and superheavy nuclei and the role of nodal structure of single-particle wavefunctions in extremely deformed structures of light nuclei
journal, February 2018

Fission barriers for even-even superheavy nuclei
journal, July 2010

Neutron-induced astrophysical reaction rates for translead nuclei
journal, April 2010

Fission properties of the Barcelona-Catania-Paris-Madrid energy density functional
journal, November 2013

Accurate, Large-Scale Density Functional Melting of Hg: Relativistic Effects Decrease Melting Temperature by 160 K
journal, March 2017

The role of radioactive ion beams in nuclear astrophysics
journal, January 2013

Assessing theoretical uncertainties in fission barriers of superheavy nuclei
journal, May 2017

The tidal disruption of neutron stars by black holes in close binaries
journal, November 1976

Nuclear Properties for Astrophysical and Radioactive-Ion-Beam Applications
journal, July 1997