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Title: Protonic ceramic electrochemical cells for hydrogen production and electricity generation: exceptional reversibility, stability, and demonstrated faradaic efficiency

Abstract

We demonstrate excellent performance and durability at intermediate temperatures (500–650 °C) upon reversible operation of an electrochemical cell incorporating a proton-permeable, high-activity mixed conducting oxide as the air electrode, a highly proton-conductive and chemically stable perovskite oxide as the electrolyte, and a composite of Ni and the electrolyte as the fuel electrode.

Authors:
ORCiD logo [1]; ORCiD logo [2]; ORCiD logo [2]
  1. Materials Science and Engineering, Northwestern University, Evanston, USA, Department of Mechanical Engineering
  2. Materials Science and Engineering, Northwestern University, Evanston, USA
Publication Date:
Sponsoring Org.:
USDOE Advanced Research Projects Agency - Energy (ARPA-E)
OSTI Identifier:
1488346
Grant/Contract Number:  
AR0000498
Resource Type:
Publisher's Accepted Manuscript
Journal Name:
Energy & Environmental Science
Additional Journal Information:
Journal Name: Energy & Environmental Science Journal Volume: 12 Journal Issue: 1; Journal ID: ISSN 1754-5692
Publisher:
Royal Society of Chemistry (RSC)
Country of Publication:
United Kingdom
Language:
English

Citation Formats

Choi, Sihyuk, Davenport, Timothy C., and Haile, Sossina M. Protonic ceramic electrochemical cells for hydrogen production and electricity generation: exceptional reversibility, stability, and demonstrated faradaic efficiency. United Kingdom: N. p., 2019. Web. doi:10.1039/C8EE02865F.
Choi, Sihyuk, Davenport, Timothy C., & Haile, Sossina M. Protonic ceramic electrochemical cells for hydrogen production and electricity generation: exceptional reversibility, stability, and demonstrated faradaic efficiency. United Kingdom. doi:10.1039/C8EE02865F.
Choi, Sihyuk, Davenport, Timothy C., and Haile, Sossina M. Wed . "Protonic ceramic electrochemical cells for hydrogen production and electricity generation: exceptional reversibility, stability, and demonstrated faradaic efficiency". United Kingdom. doi:10.1039/C8EE02865F.
@article{osti_1488346,
title = {Protonic ceramic electrochemical cells for hydrogen production and electricity generation: exceptional reversibility, stability, and demonstrated faradaic efficiency},
author = {Choi, Sihyuk and Davenport, Timothy C. and Haile, Sossina M.},
abstractNote = {We demonstrate excellent performance and durability at intermediate temperatures (500–650 °C) upon reversible operation of an electrochemical cell incorporating a proton-permeable, high-activity mixed conducting oxide as the air electrode, a highly proton-conductive and chemically stable perovskite oxide as the electrolyte, and a composite of Ni and the electrolyte as the fuel electrode.},
doi = {10.1039/C8EE02865F},
journal = {Energy & Environmental Science},
number = 1,
volume = 12,
place = {United Kingdom},
year = {2019},
month = {1}
}

Journal Article:
Free Publicly Available Full Text
Publisher's Version of Record
DOI: 10.1039/C8EE02865F

Citation Metrics:
Cited by: 13 works
Citation information provided by
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