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This content will become publicly available on September 24, 2019

Title: Multi-principal element transition metal dichalcogenides via reactive fusion of 3D-heterostructures

Transition metal dichalcogenides combining multiple principal elements in their structures are synthesized via mechanochemical exfoliation and spontaneous reassembly of binary precursors into 3D-heterostructures that are converted into single-phase layered materials by high-temperature reactive fusion. As a result, physical and chemical events enabling these transformations are summarized in the form of a conceivable reaction mechanism.
Authors:
 [1] ;  [1] ;  [1] ; ORCiD logo [1] ; ORCiD logo [1] ; ORCiD logo [1] ; ORCiD logo [1]
  1. Ames Lab. and Iowa State Univ., Ames, IA (United States)
Publication Date:
Report Number(s):
IS-J-9760
Journal ID: ISSN 1359-7345; CHCOFS
Grant/Contract Number:
AC02-07CH11358; Laboratory Directed Research and Development (LDRD) program
Type:
Accepted Manuscript
Journal Name:
ChemComm
Additional Journal Information:
Journal Name: ChemComm; Journal ID: ISSN 1359-7345
Publisher:
Royal Society of Chemistry
Research Org:
Ames Laboratory (AMES), Ames, IA (United States)
Sponsoring Org:
USDOE
Country of Publication:
United States
Language:
English
OSTI Identifier:
1477202
Alternate Identifier(s):
OSTI ID: 1475079