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Title: Charge modulation and structural transformation in TaTe2 studied by scanning tunneling microscopy/spectroscopy

Abstract

Here, we show that the (3 × 1) stripe structure observed in TaTe2 at room temperature arises from the formation of Ta4+–Ta4+ dimer chains along with a separate chain of Ta3+. More importantly, we reveal an intriguing lattice distortion and charge modulation at low temperature, which suggests an interplay and competition between the triple-axis (3 × 3) charge density wave-like modulation and the single-axis (3 × 1) stripe configuration. This work highlights the importance of TaTe2 as an alternative platform with rich structural and electrical phases to explore charge-lattice coupling.

Authors:
 [1];  [1];  [1]; ORCiD logo [2];  [2];  [1];  [1]
  1. Michigan State Univ., East Lansing, MI (United States). Dept. of Physics and Astronomy
  2. Tulane Univ., New Orleans, LA (United States). Dept. of Physics and Engineering Physics
Publication Date:
Research Org.:
Michigan State Univ., East Lansing, MI (United States)
Sponsoring Org.:
USDOE Office of Science (SC), Basic Energy Sciences (BES); National Science Foundation (NSF)
OSTI Identifier:
1467851
Alternate Identifier(s):
OSTI ID: 1261219
Grant/Contract Number:  
SC0006400; DMR-1410417; SC0012432
Resource Type:
Accepted Manuscript
Journal Name:
Applied Physics Letters
Additional Journal Information:
Journal Volume: 109; Journal Issue: 2; Journal ID: ISSN 0003-6951
Publisher:
American Institute of Physics (AIP)
Country of Publication:
United States
Language:
English
Subject:
75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND SUPERFLUIDITY; 36 MATERIALS SCIENCE; phase transitions; x-ray diffraction; crystal structure; tantalum; low energy electron diffraction; charge coupled devices; charge density waves; orbital charge; scanning tunneling microscopy; topography

Citation Formats

Feng, Jiagui, Tan, Andrew, Wagner, Sean, Liu, Jinyu, Mao, Zhiqiang, Ke, Xianglin, and Zhang, Pengpeng. Charge modulation and structural transformation in TaTe2 studied by scanning tunneling microscopy/spectroscopy. United States: N. p., 2016. Web. doi:10.1063/1.4958616.
Feng, Jiagui, Tan, Andrew, Wagner, Sean, Liu, Jinyu, Mao, Zhiqiang, Ke, Xianglin, & Zhang, Pengpeng. Charge modulation and structural transformation in TaTe2 studied by scanning tunneling microscopy/spectroscopy. United States. https://doi.org/10.1063/1.4958616
Feng, Jiagui, Tan, Andrew, Wagner, Sean, Liu, Jinyu, Mao, Zhiqiang, Ke, Xianglin, and Zhang, Pengpeng. Mon . "Charge modulation and structural transformation in TaTe2 studied by scanning tunneling microscopy/spectroscopy". United States. https://doi.org/10.1063/1.4958616. https://www.osti.gov/servlets/purl/1467851.
@article{osti_1467851,
title = {Charge modulation and structural transformation in TaTe2 studied by scanning tunneling microscopy/spectroscopy},
author = {Feng, Jiagui and Tan, Andrew and Wagner, Sean and Liu, Jinyu and Mao, Zhiqiang and Ke, Xianglin and Zhang, Pengpeng},
abstractNote = {Here, we show that the (3 × 1) stripe structure observed in TaTe2 at room temperature arises from the formation of Ta4+–Ta4+ dimer chains along with a separate chain of Ta3+. More importantly, we reveal an intriguing lattice distortion and charge modulation at low temperature, which suggests an interplay and competition between the triple-axis (3 × 3) charge density wave-like modulation and the single-axis (3 × 1) stripe configuration. This work highlights the importance of TaTe2 as an alternative platform with rich structural and electrical phases to explore charge-lattice coupling.},
doi = {10.1063/1.4958616},
journal = {Applied Physics Letters},
number = 2,
volume = 109,
place = {United States},
year = {Mon Jul 11 00:00:00 EDT 2016},
month = {Mon Jul 11 00:00:00 EDT 2016}
}

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Works referencing / citing this record:

Origin of the structural phase transition in single-crystal TaT e 2
journal, December 2018