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Title: Ionic liquids and derived materials for lithium and sodium batteries

Abstract

The ever-growing demand for advanced energy storage devices in portable electronics, electric vehicles and large scale power grids has triggered intensive research efforts over the past decade on lithium and sodium batteries. The key to improve their electrochemical performance and enhance the service safety lies in the development of advanced electrode, electrolyte, and auxiliary materials. Ionic liquids (ILs) are liquids consisting entirely of ions near room temperature, and are characterized by many unique properties such as ultralow volatility, high ionic conductivity, good thermal stability, low flammability, a wide electrochemical window, and tunable polarity and basicity/acidity. These properties create the possibilities of designing batteries with excellent safety, high energy/power density and long-term stability, and also provide better ways to synthesize known materials. IL-derived materials, such as poly(ionic liquids), ionogels and IL-tethered nanoparticles, retain most of the characteristics of ILs while being endowed with other favourable features, and thus they have received a great deal of attention as well. This paper provides a comprehensive review of the various applications of ILs and derived materials in lithium and sodium batteries including Li/Na-ion, dual-ion, Li/Na–S and Li/Na–air (O 2) batteries, with a particular emphasis on recent advances in the literature. Their unique characteristics enablemore » them to serve as advanced resources, medium, or ingredient for almost all the components of batteries, including electrodes, liquid electrolytes, solid electrolytes, artificial solid–electrolyte interphases, and current collectors. Finally, some thoughts on the emerging challenges and opportunities are also presented in this review for further development.« less

Authors:
ORCiD logo [1]; ORCiD logo [1]; ORCiD logo [2]; ORCiD logo [3]; ORCiD logo [1]; ORCiD logo [4]
  1. Zhejiang Univ., Hangzhou (China). Key Lab. of Biomass Chemical Engineering of Ministry of Education. College of Chemical and Biological Engineering
  2. Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States). Chemical Sciences Division
  3. Univ. of Chinese Academy of Sciences, Beijing (China). Key Lab. for Renewable Energy. Beijing Key Lab. for New Energy Materials and Devices. Inst. of Physics
  4. Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States). Chemical Sciences Division; Univ. of Tennessee, Knoxville, TN (United States). Dept. of Chemistry
Publication Date:
Research Org.:
Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States); Zhejiang Univ., Hangzhou (China); Univ. of Chinese Academy of Sciences, Beijing (China)
Sponsoring Org.:
USDOE Office of Science (SC), Basic Energy Sciences (BES) (SC-22); National Natural Science Foundation of China (NNSFC); Zhejiang Provincial Natural Science Foundation of China; National Program for Support of Top-notch Young Professionals (China)
OSTI Identifier:
1462843
Grant/Contract Number:  
AC05-00OR22725; 2172500185; 21476192; LZ18B060001
Resource Type:
Accepted Manuscript
Journal Name:
Chemical Society Reviews
Additional Journal Information:
Journal Volume: 47; Journal Issue: 6; Journal ID: ISSN 0306-0012
Publisher:
Royal Society of Chemistry
Country of Publication:
United States
Language:
English
Subject:
25 ENERGY STORAGE

Citation Formats

Yang, Qiwei, Zhang, Zhaoqiang, Sun, Xiao-Guang, Hu, Yong-Sheng, Xing, Huabin, and Dai, Sheng. Ionic liquids and derived materials for lithium and sodium batteries. United States: N. p., 2018. Web. doi:10.1039/c7cs00464h.
Yang, Qiwei, Zhang, Zhaoqiang, Sun, Xiao-Guang, Hu, Yong-Sheng, Xing, Huabin, & Dai, Sheng. Ionic liquids and derived materials for lithium and sodium batteries. United States. doi:10.1039/c7cs00464h.
Yang, Qiwei, Zhang, Zhaoqiang, Sun, Xiao-Guang, Hu, Yong-Sheng, Xing, Huabin, and Dai, Sheng. Fri . "Ionic liquids and derived materials for lithium and sodium batteries". United States. doi:10.1039/c7cs00464h. https://www.osti.gov/servlets/purl/1462843.
@article{osti_1462843,
title = {Ionic liquids and derived materials for lithium and sodium batteries},
author = {Yang, Qiwei and Zhang, Zhaoqiang and Sun, Xiao-Guang and Hu, Yong-Sheng and Xing, Huabin and Dai, Sheng},
abstractNote = {The ever-growing demand for advanced energy storage devices in portable electronics, electric vehicles and large scale power grids has triggered intensive research efforts over the past decade on lithium and sodium batteries. The key to improve their electrochemical performance and enhance the service safety lies in the development of advanced electrode, electrolyte, and auxiliary materials. Ionic liquids (ILs) are liquids consisting entirely of ions near room temperature, and are characterized by many unique properties such as ultralow volatility, high ionic conductivity, good thermal stability, low flammability, a wide electrochemical window, and tunable polarity and basicity/acidity. These properties create the possibilities of designing batteries with excellent safety, high energy/power density and long-term stability, and also provide better ways to synthesize known materials. IL-derived materials, such as poly(ionic liquids), ionogels and IL-tethered nanoparticles, retain most of the characteristics of ILs while being endowed with other favourable features, and thus they have received a great deal of attention as well. This paper provides a comprehensive review of the various applications of ILs and derived materials in lithium and sodium batteries including Li/Na-ion, dual-ion, Li/Na–S and Li/Na–air (O2) batteries, with a particular emphasis on recent advances in the literature. Their unique characteristics enable them to serve as advanced resources, medium, or ingredient for almost all the components of batteries, including electrodes, liquid electrolytes, solid electrolytes, artificial solid–electrolyte interphases, and current collectors. Finally, some thoughts on the emerging challenges and opportunities are also presented in this review for further development.},
doi = {10.1039/c7cs00464h},
journal = {Chemical Society Reviews},
number = 6,
volume = 47,
place = {United States},
year = {2018},
month = {2}
}

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Behavior of Germanium and Silicon Nanowire Anodes with Ionic Liquid Electrolytes
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Li-Metal Symmetrical Cell Studies Using Ionic Organic Plastic Crystal Electrolyte
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Achieving Low Overpotential Li–O 2 Battery Operations by Li 2 O 2 Decomposition through One-Electron Processes
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Different roles of ionic liquids in lithium batteries
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Evaluation of decomposition products of EMImCl·1.5AlCl3 during aluminium electrodeposition with different analytical methods
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High-Modulus, High-Conductivity Nanostructured Polymer Electrolyte Membranes via Polymerization-Induced Phase Separation
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Promising Cell Configuration for Next-Generation Energy Storage: Li 2 S/Graphite Battery Enabled by a Solvate Ionic Liquid Electrolyte
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Use of natural binders and ionic liquid electrolytes for greener and safer lithium-ion batteries
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From lithium to sodium: cell chemistry of room temperature sodium–air and sodium–sulfur batteries
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Poly(ionic liquid)s: An update
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Thiazolium Poly(ionic liquid)s: Synthesis and Application as Binder for Lithium-Ion Batteries
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Insights into the Transport of Alkali Metal Ions Doped into a Plastic Crystal Electrolyte
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Natural cellulose as binder for lithium battery electrodes
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Electrochemical Intercalation of Bis(Trifluoromethanesulfonyl) Imide Anion into Various Graphites for Dual-Ion Cells
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The synergetic effect of lithium polysulfide and lithium nitrate to prevent lithium dendrite growth
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Designing Imidazole-Based Ionic Liquids and Ionic Liquid Monomers for Emerging Technologies
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Preparation and performance of spherical FeF 2.5 ·0.5H 2 O nanoparticles wrapped by MWCNTs as cathode material of lithium ion batteries
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Ionic-Liquid-Assisted Synthesis of Nanostructured and Carbon-Coated Li 3 V 2 (PO 4 ) 3 for High-Power Electrochemical Storage Devices
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A Synergistic System for Lithium-Oxygen Batteries in Humid Atmosphere Integrating a Composite Cathode and a Hydrophobic Ionic Liquid-Based Electrolyte
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An Advanced Lithium–Air Battery Exploiting an Ionic Liquid-Based Electrolyte
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Polymerized Ionic Networks with High Charge Density: Quasi-Solid Electrolytes in Lithium-Metal Batteries
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Nitrogen-Doped Carbon Electrodes: Influence of Microstructure and Nitrogen Configuration on the Electrical Conductivity of Carbonized Polyacrylonitrile and Poly(ionic liquid) Blends
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Design Principles for Heteroatom-Doped Nanocarbon to Achieve Strong Anchoring of Polysulfides for Lithium-Sulfur Batteries
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Ionic-Liquid-Assisted Synthesis of Self-Assembled TiO 2 -B Nanosheets under Microwave Irradiation and Their Enhanced Lithium Storage Properties : Self-Assembled TiO
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Ionic liquid electrodeposition of strain-released Germanium nanowires as stable anodes for lithium ion batteries
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High Voltage LiNi 0.5 Mn 1.5 O 4 /Li 4 Ti 5 O 12 Lithium Ion Cells at Elevated Temperatures: Carbonate- versus Ionic Liquid-Based Electrolytes
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Low-Temperature Ionic-Liquid-Based Synthesis of Nanostructured Iron-Based Fluoride Cathodes for Lithium Batteries
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Role of 1,3-Dioxolane and LiNO 3 Addition on the Long Term Stability of Nanostructured Silicon/Carbon Anodes for Rechargeable Lithium Batteries
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Novel polyvinylimidazolium nanoparticles as high-performance binders for lithium-ion batteries
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Review—Development of Advanced Rechargeable Batteries: A Continuous Challenge in the Choice of Suitable Electrolyte Solutions
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Porous Hollow Carbon@Sulfur Composites for High-Power Lithium-Sulfur Batteries
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Hexagonal Boron Nitride-Based Electrolyte Composite for Li-Ion Battery Operation from Room Temperature to 150 °C
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Lithium-Ion Textile Batteries with Large Areal Mass Loading
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Optimization of Pore Structure of Cathodic Carbon Supports for Solvate Ionic Liquid Electrolytes Based Lithium–Sulfur Batteries
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Phosphate-Functionalized Carbon Monoliths from Deep Eutectic Solvents and their Use as Monolithic Electrodes in Supercapacitors
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An Artificial Solid Electrolyte Interphase Layer for Stable Lithium Metal Anodes
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High-Energy All-Solid-State Lithium Batteries with Ultralong Cycle Life
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Chemical bonding between antimony and ionic liquid-derived nitrogen-doped carbon for sodium-ion battery anode
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Deep eutectic solvents as both precursors and structure directing agents in the synthesis of nitrogen doped hierarchical carbons highly suitable for CO2 capture
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A High-Rate Ionic Liquid Lithium-O 2 Battery with LiOH Product
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Preparation of Poly(ionic liquid) Hollow Particles with Switchable Permeability
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A Stabilized PAN-FeS 2 Cathode with an EC/DEC Liquid Electrolyte
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Room-temperature stationary sodium-ion batteries for large-scale electric energy storage
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A new strategy for preparing oligomeric ionic liquid gel polymer electrolytes for high-performance and nonflammable lithium ion batteries
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Hollow-in-hollow carbon spheres with hollow foam-like cores for lithium–sulfur batteries
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Ionic Liquids as Precursors for Efficient Mesoporous Iron-Nitrogen-Doped Oxygen Reduction Electrocatalysts
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3D ordered macroporous germanium fabricated by electrodeposition from an ionic liquid and its lithium storage properties
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Chemistry of Sputter-Deposited Lithium Sulfide Films
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A Mesoporous Iron-Based Fluoride Cathode of Tunnel Structure for Rechargeable Lithium Batteries
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Passivation of Lithium Metal Anode via Hybrid Ionic Liquid Electrolyte toward Stable Li Plating/Stripping
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Nitrogen-Doped Porous Carbon Nanofiber Webs as Anodes for Lithium Ion Batteries with a Superhigh Capacity and Rate Capability
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A review of advanced and practical lithium battery materials
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Ternary nanoarray electrode with corn-inspired hierarchical design for synergistic lithium storage
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Challenges in the development of advanced Li-ion batteries: a review
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Ultrathin few-layered molybdenum selenide/graphene hybrid with superior electrochemical Li-storage performance
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Poly(ionic liquid)-Mediated Hybridization of Single-Walled Carbon Nanotubes and Conducting Polymers
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Li-Storage via Heterogeneous Reaction in Selected Binary Metal Fluorides and Oxides
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Synthesis Of Nitrogen-Doped Graphene Films For Lithium Battery Application
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Effect of Anion on Behaviour of Li-S Battery Electrolyte Solutions Based on N-Methyl-N-Butyl-Pyrrolidinium Ionic Liquids
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Ionic liquid-derived Fe–N/C catalysts for highly efficient oxygen reduction reaction without any supports, templates, or multi-step pyrolysis
journal, January 2016

  • He, Fei; Chen, Xinghua; Shen, Yanfei
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Programmable Polymer Memory Device Based on Hydrophilic Polythiophene and Poly(ionic liquid) Electrolyte
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Positive Electrode Materials for Li-Ion and Li-Batteries
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Safety focused modeling of lithium-ion batteries: A review
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Plastic Crystal Electrolyte Materials: New Perspectives on Solid State Ionics
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Reversible Intercalation of Bis(trifluoromethanesulfonyl)imide Anions from an Ionic Liquid Electrolyte into Graphite for High Performance Dual-Ion Cells
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Influence of Graphite Characteristics on the Electrochemical Intercalation of Bis(trifluoromethanesulfonyl) imide Anions into a Graphite-Based Cathode
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Multifunctional Mesoporous Ionic Gels and Scaffolds Derived from Polyhedral Oligomeric Silsesquioxanes
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Ionic Liquid-Assisted Synthesis of TiO 2 -Carbon Hybrid Nanostructures for Lithium-Ion Batteries
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A review of electrolyte materials and compositions for electrochemical supercapacitors
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Application of Ionic Liquids to Energy Storage and Conversion Materials and Devices
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Ionic liquid-nanoparticle hybrid electrolytes
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Study on Polymer Binders for High-Capacity SiO Negative Electrode of Li-Ion Batteries
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Piperidinium tethered nanoparticle-hybrid electrolyte for lithium metal batteries
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N-methyl-N-alkylpyrrolidinium nonafluoro-1-butanesulfonate salts: Ionic liquid properties and plastic crystal behaviour
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Nitrogen-doped carbon nanostructures and their composites as catalytic materials for proton exchange membrane fuel cell
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Complexes of Lithium Imide Salts with Tetraglyme and Their Polyelectrolyte Composite Materials
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Efficient nitrogen-doping and structural control of hierarchical carbons using unconventional precursors in the form of deep eutectic solvents
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Atom transfer radical polymerization of styrenic ionic liquid monomers and carbon dioxide absorption of the polymerized ionic liquids
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An excellent rechargeable PP 14 TFSI ionic liquid dual-ion battery
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Direct electrodeposition of aluminium nano-rods
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Ionic Liquid Electrolytes for Lithium–Sulfur Batteries
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Ionic Liquid-based Electrolytes for Li Metal/Air Batteries: A Review of Materials and the New 'LABOHR' Flow Cell Concept
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A review of recent developments in rechargeable lithium–sulfur batteries
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A critical review on lithium–air battery electrolytes
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Oxygen Reduction Reactions in Ionic Liquids and the Formulation of a General ORR Mechanism for Li–Air Batteries
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Ionic liquids and reactions at the electrochemical interface
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Ionic liquid decorated mesoporous silica nanoparticles: a new high-performance hybrid electrolyte for lithium batteries
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Plastic crystal behaviour in tetraethylammonium dicyanamide
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3D Anhydrous Proton-Transporting Nanochannels Formed by Self-Assembly of Liquid Crystals Composed of a Sulfobetaine and a Sulfonic Acid
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Dual-graphite cells based on the reversible intercalation of bis(trifluoromethanesulfonyl)imide anions from an ionic liquid electrolyte
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Optimized Silicon Electrode Architecture, Interface, and Microgeometry for Next-Generation Lithium-Ion Batteries
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Exceptional long-life performance of lithium-ion batteries using ionic liquid-based electrolytes
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Dehydrating bronze iron fluoride as a high capacity conversion cathode for lithium batteries
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Physical properties of high Li-ion content N-propyl-N-methylpyrrolidinium bis(fluorosulfonyl)imide based ionic liquid electrolytes
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An FeF 3 ·0.5H 2 O Polytype: A Microporous Framework Compound with Intersecting Tunnels for Li and Na Batteries
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A review of flexible lithium–sulfur and analogous alkali metal–chalcogen rechargeable batteries
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High Lithium Transference Number Electrolytes via Creation of 3-Dimensional, Charged, Nanoporous Networks from Dense Functionalized Nanoparticle Composites
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X-ray diffraction studies of the electrochemical intercalation of bis(trifluoromethanesulfonyl)imide anions into graphite for dual-ion cells
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A rechargeable Na–CO 2 /O 2 battery enabled by stable nanoparticle hybrid electrolytes
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Atom transfer radical polymerization of ionic liquid 2-(1-butylimidazolium-3-yl)ethyl methacrylate tetrafluoroborate
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Lithium-Sulfur Batteries Based on Nitrogen-Doped Carbon and an Ionic-Liquid Electrolyte
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Prospects and Limits of Energy Storage in Batteries
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On the Comparative Stability of Li and Na Metal Anode Interfaces in Conventional Alkyl Carbonate Electrolytes
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Ternary polymer electrolytes containing pyrrolidinium-based polymeric ionic liquids for lithium batteries
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Flexible Dimensional Control of High-Capacity Li-Ion-Battery Anodes: From 0D Hollow to 3D Porous Germanium Nanoparticle Assemblies
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Li/air Flow Battery Employing Ionic Liquid Electrolytes
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Li-Ion Diffusion in the Equilibrium Nanomorphology of Spinel Li 4+ x Ti 5 O 12
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Ionic liquid based electrolytes for sodium-ion batteries: Na+ solvation and ionic conductivity
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Solvate Ionic Liquid Electrolyte for Li–S Batteries
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Electrolytes and Interphases in Li-Ion Batteries and Beyond
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Instability of Ionic Liquid-Based Electrolytes in Li–O 2 Batteries
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Characteristics of a Graphene Nanoplatelet Anode in Advanced Lithium-Ion Batteries Using Ionic Liquid Added by a Carbonate Electrolyte
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Rechargeable Na/Na0.44MnO2 cells with ionic liquid electrolytes containing various sodium solutes
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Advances in lithium–sulfur batteries based on multifunctional cathodes and electrolytes
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Porous Li4Ti5O12 Coated with N-Doped Carbon from Ionic Liquids for Li-Ion Batteries
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Effect of the cation on the stability of cation–glyme complexes and their interactions with the [TFSA] anion
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A hybrid polymer/oxide/ionic-liquid solid electrolyte for Na-metal batteries
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Ambient Lithium-SO 2 Batteries with Ionic Liquids as Electrolytes
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A High-Capacity Cathode for Lithium Batteries Consisting of Porous Microspheres of Highly Amorphized Iron Fluoride Densified from Its Open Parent Phase
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Lithium-Sulfur Batteries: Electrochemistry, Materials, and Prospects
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N-Methyl-N-Alkylpyrrolidinium Bis(perfluoroethylsulfonyl)amide ([NPf2]–) and Tris(trifluoromethanesulfonyl)methide ([CTf3]–) Salts: Synthesis and Characterization
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Efficient removal of both basic and non-basic nitrogen compounds from fuels by deep eutectic solvents
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Solvate Structures and Spectroscopic Characterization of LiTFSI Electrolytes
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Ionic liquid electrolytes as a platform for rechargeable metal–air batteries: a perspective
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Ionic Liquids for Soft Functional Materials with Carbon Nanotubes
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Insertion reactions in advanced electrochemical energy storage
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Towards a Stable Organic Electrolyte for the Lithium Oxygen Battery
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Oxygen Electrode Rechargeability in an Ionic Liquid for the Li–Air Battery
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A stable room-temperature sodium–sulfur battery
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Self-Regulative Nanogelator Solid Electrolyte: A New Option to Improve the Safety of Lithium Battery
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Protic-Salt-Derived Nitrogen/Sulfur-Codoped Mesoporous Carbon for the Oxygen Reduction Reaction and Supercapacitors
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Ionic liquids for energy, materials, and medicine
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Investigation of PF 6 and TFSI anion intercalation into graphitized carbon blacks and its influence on high voltage lithium ion batteries
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Towards safer sodium-ion batteries via organic solvent/ionic liquid based hybrid electrolytes
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Effect of Ionic Size on Solvate Stability of Glyme-Based Solvate Ionic Liquids
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Recent advances in zinc–air batteries
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Lithium–oxygen cells with ionic-liquid-based electrolytes and vertically aligned carbon nanotube cathodes
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Solid-State Li-Ion Batteries Using Fast, Stable, Glassy Nanocomposite Electrolytes for Good Safety and Long Cycle-Life
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Frontiers in poly(ionic liquid)s: syntheses and applications
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Electrochemical investigations of ionic liquids with vinylene carbonate for applications in rechargeable lithium ion batteries
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Bio-inspired synthesis of N,F co-doped 3D graphitized carbon foams containing manganese fluoride nanocrystals for lithium ion batteries
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High-Rate, Ultralong Cycle-Life Lithium/Sulfur Batteries Enabled by Nitrogen-Doped Graphene
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An AlCl3 based ionic liquid with a neutral substituted pyridine ligand for electrochemical deposition of aluminum
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Li + solvation in glyme–Li salt solvate ionic liquids
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Ionic Liquids as Versatile Precursors for Functionalized Porous Carbon and Carbon-Oxide Composite Materials by Confined Carbonization
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A General Salt-Templating Method To Fabricate Vertically Aligned Graphitic Carbon Nanosheets and Their Metal Carbide Hybrids for Superior Lithium Ion Batteries and Water Splitting
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Stability of Glyme Solvate Ionic Liquid as an Electrolyte for Rechargeable Li−O 2 Batteries
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Template-assisted electrodeposition of highly ordered macroporous zinc structures from an ionic liquid
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Safer Electrolytes for Lithium-Ion Batteries: State of the Art and Perspectives
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Lithium batteries: Status, prospects and future
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A Dual−Ion Battery Cathode via Oxidative Insertion of Anions in a Metal–Organic Framework
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Electrochemical Template Deposition of Aluminum Nanorods Using Ionic Liquids
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Towards greener and more sustainable batteries for electrical energy storage
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Ion Gels Prepared by in Situ Radical Polymerization of Vinyl Monomers in an Ionic Liquid and Their Characterization as Polymer Electrolytes
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Dissimilar Crystal Dependence of Vanadium Oxide Cathodes in Organic Carbonate and Safe Ionic Liquid Electrolytes
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Organic ionic plastic crystals: recent advances
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The Design of Polymeric Ionic Liquids for the Preparation of Functional Materials
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Synthesis and characterisation of new polymeric ionic liquid poly(imidazolium chloride-4,6-dinitrobenzene-1,3-diyl)
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A Novel Aluminum-Graphite Dual-Ion Battery
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Freeze-Drying of Aqueous Solutions of Deep Eutectic Solvents: A Suitable Approach to Deep Eutectic Suspensions of Self-Assembled Structures
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Ambient Lithium-SO 2 Batteries with Ionic Liquids as Electrolytes
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Rechargeable Room-Temperature Na-CO 2 Batteries
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Porous Hollow Carbon@Sulfur Composites for High-Power Lithium-Sulfur Batteries
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