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Title: Observation of Out-of-Plane Spin Texture in a SrTiO 3 ( 111 ) Two-Dimensional Electron Gas

Abstract

Here, we explore the second order bilinear magnetoelectric resistance (BMER) effect in the d-electron-based two-dimensional electron gas (2DEG) at the SrTiO3 (111) surface. We find evidence of a spin-split band structure with the archetypal spin-momentum locking of the Rashba effect for the in-plane component. Applying an out-of-plane magnetic field, we find a BMER signal that breaks the six-fold symmetry of the electronic dispersion, which is a fingerprint for the presence of a momentum dependent out-of-plane spin component. Relativistic electronic structure calculations reproduce this spin-texture and indicate that the out-of-plane component is a ubiquitous property of oxide 2DEGs arising from strong crystal field effects. We further show that the BMER response of the SrTiO3 (111) 2DEG is tunable and unexpectedly large.

Authors:
 [1];  [2];  [3];  [2];  [4];  [1];  [1];  [1];  [3];  [5];  [6];  [1]
  1. National Univ. of Singapore (Singapore). Dept. of Electrical and Computer Engineering and NUS Nanoscience & Nanotechnology Inst. (NUSNNI)
  2. Univ. of Geneva (Switzerland). Dept. of Quantum Matter Physics
  3. Argonne National Lab. (ANL), Argonne, IL (United States). Materials Science Division
  4. Univ. of Tokyo (Japan). Dept. of Applied Physics and Quantum-Phase Electronics Center; RIKEN Center for Emergent Matter Science (CEMS), Wako (Japan)
  5. Univ. of Missouri, Columbia, MO (United States). Dept. of Physics and Astronomy
  6. Univ. of Geneva (Switzerland). Dept. of Quantum Matter Physics; Paul Scherrer Inst. (PSI), Villigen (Switzerland). Swiss Light Source
Publication Date:
Research Org.:
Argonne National Laboratory (ANL), Argonne, IL (United States)
Sponsoring Org.:
USDOE Office of Science (SC), Basic Energy Sciences (BES) (SC-22). Materials Sciences & Engineering Division; National Research Foundation of Korea (NRF); Swiss National Science Foundation (SNF); Japan Science and Technology Agency (JST); National Science Foundation (NSF)
OSTI Identifier:
1462733
Alternate Identifier(s):
OSTI ID: 1457817
Grant/Contract Number:  
AC02-06CH11357; NRFCRP12-2013-01; 200020-165791; PZ00P2-161327; JPMJCR16F1; DMR-1406568
Resource Type:
Accepted Manuscript
Journal Name:
Physical Review Letters
Additional Journal Information:
Journal Volume: 120; Journal Issue: 26; Journal ID: ISSN 0031-9007
Publisher:
American Physical Society (APS)
Country of Publication:
United States
Language:
English
Subject:
74 ATOMIC AND MOLECULAR PHYSICS; magnetotransport; rashba coupling; spin texture; spin-orbit coupling; spintronics; two-dimensional electron gas

Citation Formats

He, Pan, Walker, S. McKeown, Zhang, Steven S. -L., Bruno, F. Y., Bahramy, M. S., Lee, Jong Min, Ramaswamy, Rajagopalan, Cai, Kaiming, Heinonen, Olle, Vignale, Giovanni, Baumberger, F., and Yang, Hyunsoo. Observation of Out-of-Plane Spin Texture in a SrTiO3(111) Two-Dimensional Electron Gas. United States: N. p., 2018. Web. doi:10.1103/PhysRevLett.120.266802.
He, Pan, Walker, S. McKeown, Zhang, Steven S. -L., Bruno, F. Y., Bahramy, M. S., Lee, Jong Min, Ramaswamy, Rajagopalan, Cai, Kaiming, Heinonen, Olle, Vignale, Giovanni, Baumberger, F., & Yang, Hyunsoo. Observation of Out-of-Plane Spin Texture in a SrTiO3(111) Two-Dimensional Electron Gas. United States. https://doi.org/10.1103/PhysRevLett.120.266802
He, Pan, Walker, S. McKeown, Zhang, Steven S. -L., Bruno, F. Y., Bahramy, M. S., Lee, Jong Min, Ramaswamy, Rajagopalan, Cai, Kaiming, Heinonen, Olle, Vignale, Giovanni, Baumberger, F., and Yang, Hyunsoo. Fri . "Observation of Out-of-Plane Spin Texture in a SrTiO3(111) Two-Dimensional Electron Gas". United States. https://doi.org/10.1103/PhysRevLett.120.266802. https://www.osti.gov/servlets/purl/1462733.
@article{osti_1462733,
title = {Observation of Out-of-Plane Spin Texture in a SrTiO3(111) Two-Dimensional Electron Gas},
author = {He, Pan and Walker, S. McKeown and Zhang, Steven S. -L. and Bruno, F. Y. and Bahramy, M. S. and Lee, Jong Min and Ramaswamy, Rajagopalan and Cai, Kaiming and Heinonen, Olle and Vignale, Giovanni and Baumberger, F. and Yang, Hyunsoo},
abstractNote = {Here, we explore the second order bilinear magnetoelectric resistance (BMER) effect in the d-electron-based two-dimensional electron gas (2DEG) at the SrTiO3 (111) surface. We find evidence of a spin-split band structure with the archetypal spin-momentum locking of the Rashba effect for the in-plane component. Applying an out-of-plane magnetic field, we find a BMER signal that breaks the six-fold symmetry of the electronic dispersion, which is a fingerprint for the presence of a momentum dependent out-of-plane spin component. Relativistic electronic structure calculations reproduce this spin-texture and indicate that the out-of-plane component is a ubiquitous property of oxide 2DEGs arising from strong crystal field effects. We further show that the BMER response of the SrTiO3 (111) 2DEG is tunable and unexpectedly large.},
doi = {10.1103/PhysRevLett.120.266802},
journal = {Physical Review Letters},
number = 26,
volume = 120,
place = {United States},
year = {Fri Jun 29 00:00:00 EDT 2018},
month = {Fri Jun 29 00:00:00 EDT 2018}
}

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Works referenced in this record:

Spin galvanic effect at the conducting SrTiO 3 surfaces
journal, December 2016

  • Zhang, Wenxu; Wang, Qiuru; Peng, Bin
  • Applied Physics Letters, Vol. 109, Issue 26
  • DOI: 10.1063/1.4973479

Blue-light emission at room temperature from Ar+-irradiated SrTiO3
journal, October 2005

  • Kan, Daisuke; Terashima, Takahito; Kanda, Ryoko
  • Nature Materials, Vol. 4, Issue 11
  • DOI: 10.1038/nmat1498

Control of a Two-Dimensional Electron Gas on SrTiO 3 ( 111 ) by Atomic Oxygen
journal, October 2014


Efficient spin-to-charge conversion in the 2D electron liquid at the LAO/STO interface
journal, October 2016


Electrostatic modulation of anisotropic magnetotransport in Ar + -irradiated SrTiO 3 : Effects of boundary scattering
journal, January 2011


Highly efficient and tunable spin-to-charge conversion through Rashba coupling at oxide interfaces
journal, August 2016

  • Lesne, E.; Fu, Yu; Oyarzun, S.
  • Nature Materials, Vol. 15, Issue 12
  • DOI: 10.1038/nmat4726

Room-Temperature Giant Charge-to-Spin Conversion at the SrTiO 3 –LaAlO 3 Oxide Interface
journal, November 2017


Anisotropic magneto-transport properties of electron gases at SrTiO 3 (111) and (110) surfaces
journal, December 2016

  • Miao, Ludi; Du, Renzhong; Yin, Yuewei
  • Applied Physics Letters, Vol. 109, Issue 26
  • DOI: 10.1063/1.4972985

Unidirectional spin Hall magnetoresistance in ferromagnet/normal metal bilayers
journal, June 2015

  • Avci, Can Onur; Garello, Kevin; Ghosh, Abhijit
  • Nature Physics, Vol. 11, Issue 7
  • DOI: 10.1038/nphys3356

Observation of inverse Edelstein effect in Rashba-split 2DEG between SrTiO 3 and LaAlO 3 at room temperature
journal, March 2017


Nonlinear spin current generation in noncentrosymmetric spin-orbit coupled systems
journal, June 2017


Bilinear magnetoelectric resistance as a probe of three-dimensional spin texture in topological surface states
journal, February 2018


Interference of spin states in photoemission from Sb/Ag(111) surface alloys
journal, February 2011

  • Meier, Fabian; Petrov, Vladimir; Mirhosseini, Hossein
  • Journal of Physics: Condensed Matter, Vol. 23, Issue 7
  • DOI: 10.1088/0953-8984/23/7/072207

Experimental Evidence of Cubic Rashba Effect in an Inversion-Symmetric Oxide
journal, May 2012


Magnetic breakdown and the de Haas–van Alphen effect in Hg 1 x Fe x Se
journal, August 1988


Towards Two-Dimensional Metallic Behavior at LaAlO 3 / SrTiO 3 Interfaces
journal, May 2009


Microscopic Theory of the Inverse Edelstein Effect
journal, March 2014


Electrical Transport Anisotropy Controlled by Oxygen Vacancy Concentration in (111) LaAlO 3 /SrTiO 3 Interface Structures
journal, December 2016

  • Davis, Samuel Kenneth; Huang, Zhen; Han, Kun
  • Advanced Materials Interfaces, Vol. 4, Issue 3
  • DOI: 10.1002/admi.201600830

Nonmonotonically tunable Rashba spin-orbit coupling by multiple-band filling control in SrTiO 3 -based interfacial d -electron gases
journal, August 2015


Theory of unidirectional spin Hall magnetoresistance in heavy-metal/ferromagnetic-metal bilayers
journal, October 2016


Magnetism, Spin Texture, and In-Gap States: Atomic Specialization at the Surface of Oxygen-Deficient SrTiO 3
journal, April 2016


Spin-to-charge conversion using Rashba coupling at the interface between non-magnetic materials
journal, December 2013

  • Sánchez, J. C. Rojas; Vila, L.; Desfonds, G.
  • Nature Communications, Vol. 4, Issue 1
  • DOI: 10.1038/ncomms3944

Quasiparticle dynamics and spin–orbital texture of the SrTiO3 two-dimensional electron gas
journal, February 2014

  • King, P. D. C.; McKeown Walker, S.; Tamai, A.
  • Nature Communications, Vol. 5, Issue 1
  • DOI: 10.1038/ncomms4414

Nature of orbital and spin Rashba coupling in the surface bands of SrTiO 3 and KTaO 3
journal, November 2014


Massive Symmetry Breaking in LaAlO 3 / SrTiO 3 ( 111 ) Quantum Wells: A Three-Orbital Strongly Correlated Generalization of Graphene
journal, September 2013


Six-fold crystalline anisotropic magnetoresistance in the (111) LaAlO 3 / SrTiO 3 oxide interface
journal, June 2017


Theory of spin-orbit coupling at LaAlO 3 /SrTiO 3 interfaces and SrTiO 3 surfaces
journal, April 2013


Orientational Tuning of the Fermi Sea of Confined Electrons at the SrTiO 3 (110) and (111) Surfaces
journal, June 2014


Theory of the SrTiO 3 surface state two-dimensional electron gas
journal, September 2012


Bulk rectification effect in a polar semiconductor
journal, March 2017

  • Ideue, T.; Hamamoto, K.; Koshikawa, S.
  • Nature Physics, Vol. 13, Issue 6
  • DOI: 10.1038/nphys4056

Charge-to-Spin Conversion and Spin Diffusion in Bi/Ag Bilayers Observed by Spin-Polarized Positron Beam
journal, April 2015


Absence of giant spin splitting in the two-dimensional electron liquid at the surface of SrTiO 3 (001)
journal, June 2016


Topological insulators from complex orbital order in transition-metal oxides heterostructures
journal, November 2011


New perspectives for Rashba spin–orbit coupling
journal, August 2015

  • Manchon, A.; Koo, H. C.; Nitta, J.
  • Nature Materials, Vol. 14, Issue 9
  • DOI: 10.1038/nmat4360

Tunable Rashba Spin-Orbit Interaction at Oxide Interfaces
journal, March 2010


Quasiparticle dynamics and spin-orbital texture of the SrTiO3 two-dimensional electron gas
text, January 2014


New Perspectives for Rashba Spin-Orbit Coupling
text, January 2015


Spin galvanic effect at the conducting SrTiO3 surfaces
text, January 2016


Room Temperature Giant Charge-to-Spin Conversion at SrTiO3/LaAlO3 Oxide Interface
text, January 2017


Works referencing / citing this record:

Band Structure and Spin–Orbital Texture of the (111)‐KTaO 3 2D Electron Gas
journal, March 2019

  • Bruno, Flavio Y.; McKeown Walker, Siobhan; Riccò, Sara
  • Advanced Electronic Materials, Vol. 5, Issue 5
  • DOI: 10.1002/aelm.201800860

Nonlinear magnetotransport shaped by Fermi surface topology and convexity
journal, March 2019


Nonreciprocal charge transport at topological insulator/superconductor interface
journal, June 2019


Gate-tunable giant nonreciprocal charge transport in noncentrosymmetric oxide interfaces
journal, October 2019


Coexistence of large conventional and planar spin Hall effect with long spin diffusion length in a low-symmetry semimetal at room temperature
journal, February 2020


Band Structure and Spin–Orbital Texture of the $(111)‐KTaO_{3}$ 2D Electron Gas
text, January 2019

  • Bruno, Flavio Y.; McKeown Walker, Siobhan; Riccò, Sara
  • Deutsches Elektronen-Synchrotron, DESY, Hamburg
  • DOI: 10.3204/pubdb-2019-05605