Assessment of long-term WRF–CMAQ simulations for understanding direct aerosol effects on radiation "brightening" in the United States
Abstract
Long-term simulations with the coupled WRF–CMAQ (Weather Research and Forecasting–Community Multi-scale Air Quality) model have been conducted to systematically investigate the changes in anthropogenic emissions of SO2 and NOx over the past 16 years (1995–2010) across the United States (US), their impacts on anthropogenic aerosol loading over North America, and subsequent impacts on regional radiation budgets. In particular, this study attempts to determine the consequences of the changes in tropospheric aerosol burden arising from substantial reductions in emissions of SO2 and NOx associated with control measures under the Clean Air Act (CAA) especially on trends in solar radiation. Extensive analyses conducted by Gan et al. (2014a) utilizing observations (e.g., SURFRAD, CASTNET, IMPROVE, and ARM) over the past 16 years (1995–2010) indicate a shortwave (SW) radiation (both all-sky and clear-sky) "brightening" in the US. The relationship of the radiation brightening trend with decreases in the aerosol burden is less apparent in the western US. One of the main reasons for this is that the emission controls under the CAA were aimed primarily at reducing pollutants in areas violating national air quality standards, most of which were located in the eastern US, while the relatively less populated areas in the western USmore »
- Authors:
- Publication Date:
- Research Org.:
- U.S. Environmental Protection Agency, Research Triangle Park, NC (United States)
- Sponsoring Org.:
- USDOE Office of Science (SC)
- OSTI Identifier:
- 1224934
- Alternate Identifier(s):
- OSTI ID: 1458717
- Grant/Contract Number:
- SC0003782
- Resource Type:
- Published Article
- Journal Name:
- Atmospheric Chemistry and Physics (Online)
- Additional Journal Information:
- Journal Name: Atmospheric Chemistry and Physics (Online) Journal Volume: 15 Journal Issue: 21; Journal ID: ISSN 1680-7324
- Publisher:
- Copernicus Publications, EGU
- Country of Publication:
- Germany
- Language:
- English
- Subject:
- 54 ENVIRONMENTAL SCIENCES
Citation Formats
Gan, C.-M., Pleim, J., Mathur, R., Hogrefe, C., Long, C. N., Xing, J., Wong, D., Gilliam, R., and Wei, C. Assessment of long-term WRF–CMAQ simulations for understanding direct aerosol effects on radiation "brightening" in the United States. Germany: N. p., 2015.
Web. doi:10.5194/acp-15-12193-2015.
Gan, C.-M., Pleim, J., Mathur, R., Hogrefe, C., Long, C. N., Xing, J., Wong, D., Gilliam, R., & Wei, C. Assessment of long-term WRF–CMAQ simulations for understanding direct aerosol effects on radiation "brightening" in the United States. Germany. https://doi.org/10.5194/acp-15-12193-2015
Gan, C.-M., Pleim, J., Mathur, R., Hogrefe, C., Long, C. N., Xing, J., Wong, D., Gilliam, R., and Wei, C. Tue .
"Assessment of long-term WRF–CMAQ simulations for understanding direct aerosol effects on radiation "brightening" in the United States". Germany. https://doi.org/10.5194/acp-15-12193-2015.
@article{osti_1224934,
title = {Assessment of long-term WRF–CMAQ simulations for understanding direct aerosol effects on radiation "brightening" in the United States},
author = {Gan, C.-M. and Pleim, J. and Mathur, R. and Hogrefe, C. and Long, C. N. and Xing, J. and Wong, D. and Gilliam, R. and Wei, C.},
abstractNote = {Long-term simulations with the coupled WRF–CMAQ (Weather Research and Forecasting–Community Multi-scale Air Quality) model have been conducted to systematically investigate the changes in anthropogenic emissions of SO2 and NOx over the past 16 years (1995–2010) across the United States (US), their impacts on anthropogenic aerosol loading over North America, and subsequent impacts on regional radiation budgets. In particular, this study attempts to determine the consequences of the changes in tropospheric aerosol burden arising from substantial reductions in emissions of SO2 and NOx associated with control measures under the Clean Air Act (CAA) especially on trends in solar radiation. Extensive analyses conducted by Gan et al. (2014a) utilizing observations (e.g., SURFRAD, CASTNET, IMPROVE, and ARM) over the past 16 years (1995–2010) indicate a shortwave (SW) radiation (both all-sky and clear-sky) "brightening" in the US. The relationship of the radiation brightening trend with decreases in the aerosol burden is less apparent in the western US. One of the main reasons for this is that the emission controls under the CAA were aimed primarily at reducing pollutants in areas violating national air quality standards, most of which were located in the eastern US, while the relatively less populated areas in the western US were less polluted at the beginning of this study period. Comparisons of model results with observations of aerosol optical depth (AOD), aerosol concentration, and radiation demonstrate that the coupled WRF–CMAQ model is capable of replicating the trends well even though it tends to underestimate the AOD. In particular, the sulfate concentration predictions were well matched with the observations. As a result, the discrepancies found in the clear-sky diffuse SW radiation are likely due to several factors such as the potential increase of ice particles associated with increasing air traffic, the definition of "clear-sky" in the radiation retrieval methodology, and aerosol semi-direct and/or indirect effects which cannot be readily isolated from the observed data.},
doi = {10.5194/acp-15-12193-2015},
journal = {Atmospheric Chemistry and Physics (Online)},
number = 21,
volume = 15,
place = {Germany},
year = {Tue Nov 03 00:00:00 EST 2015},
month = {Tue Nov 03 00:00:00 EST 2015}
}
https://doi.org/10.5194/acp-15-12193-2015
Web of Science
Works referenced in this record:
Global dimming and brightening: An update beyond 2000
journal, January 2009
- Wild, Martin; Trüssel, Barbara; Ohmura, Atsumu
- Journal of Geophysical Research, Vol. 114
A case study of the radiative forcing of persistent contrails evolving into contrail-induced cirrus
journal, January 2009
- Haywood, James M.; Allan, Richard P.; Bornemann, Jorge
- Journal of Geophysical Research, Vol. 114, Issue D24
An analysis of 25 Years of balloonborne aerosol data in search of a signature of the subsonic commercial aircraft fleet
journal, July 1998
- Hofmann, David J.; Stone, Robert S.; Wood, Matthew E.
- Geophysical Research Letters, Vol. 25, Issue 13
The Southeastern Aerosol Research and Characterization (SEARCH) study: Temporal trends in gas and PM concentrations and composition, 1999–2010
journal, September 2012
- Blanchard, C. L.; Hidy, G. M.; Tanenbaum, S.
- Journal of the Air & Waste Management Association, Vol. 63, Issue 3
Assessment of the aerosol optics component of the coupled WRF–CMAQ model using CARES field campaign data and a single column model
journal, August 2015
- Gan, Chuen Meei; Binkowski, Francis; Pleim, Jonathan
- Atmospheric Environment, Vol. 115
Significant decadal brightening of downwelling shortwave in the continental United States
journal, January 2009
- Long, C. N.; Dutton, E. G.; Augustine, J. A.
- Journal of Geophysical Research, Vol. 114
WRF-CMAQ two-way coupled system with aerosol feedback: software development and preliminary results
journal, January 2012
- Wong, D. C.; Pleim, J.; Mathur, R.
- Geoscientific Model Development, Vol. 5, Issue 2
Aerosol indirect effect on the grid-scale clouds in the two-way coupled WRF–CMAQ: model description, development, evaluation and regional analysis
journal, January 2014
- Yu, S.; Mathur, R.; Pleim, J.
- Atmospheric Chemistry and Physics, Vol. 14, Issue 20
Historical gaseous and primary aerosol emissions in the United States from 1990 to 2010
journal, January 2013
- Xing, J.; Pleim, J.; Mathur, R.
- Atmospheric Chemistry and Physics, Vol. 13, Issue 15
Incremental testing of the Community Multiscale Air Quality (CMAQ) modeling system version 4.7
journal, January 2010
- Foley, K. M.; Roselle, S. J.; Appel, K. W.
- Geoscientific Model Development, Vol. 3, Issue 1
Multi-decadal aerosol variations from 1980 to 2009: a perspective from observations and a global model
journal, January 2014
- Chin, M.; Diehl, T.; Tan, Q.
- Atmospheric Chemistry and Physics, Vol. 14, Issue 7
Spatial and Temporal Trends in PM 2.5 Organic and Elemental Carbon across the United States
journal, January 2013
- Hand, J. L.; Schichtel, B. A.; Malm, W. C.
- Advances in Meteorology, Vol. 2013
Retrieving Cloud Characteristics from Ground-Based Daytime Color All-Sky Images
journal, May 2006
- Long, C. N.; Sabburg, J. M.; Calbó, J.
- Journal of Atmospheric and Oceanic Technology, Vol. 23, Issue 5
Evaluation of cloudless-sky periods detected by shortwave and longwave algorithms using lidar measurements: EVALUATION OF CLOUDLESS-SKY PERIODS
journal, May 2008
- Dupont, Jean-Charles; Haeffelin, Martial; Long, Charles N.
- Geophysical Research Letters, Vol. 35, Issue 10
An Indirect Data Assimilation Scheme for Deep Soil Temperature in the Pleim–Xiu Land Surface Model
journal, July 2009
- Pleim, Jonathan E.; Gilliam, Robert
- Journal of Applied Meteorology and Climatology, Vol. 48, Issue 7
Large Asian dust layers continuously reached North America in April 2010
journal, January 2011
- Uno, I.; Eguchi, K.; Yumimoto, K.
- Atmospheric Chemistry and Physics, Vol. 11, Issue 14
Analysis of the Interaction of Aerosol Transport Layers on Local Air Quality
conference, July 2008
- Gan, Chuen-Meei; Charles, Leona; Gross, Barry
- IGARSS 2008 - 2008 IEEE International Geoscience and Remote Sensing Symposium
Variability of the surface radiation budget over the United States from 1996 through 2011 from high-quality measurements: U.S. SURFACE RADIATION BUDGET CLIMATOLOGY
journal, January 2013
- Augustine, John A.; Dutton, Ellsworth G.
- Journal of Geophysical Research: Atmospheres, Vol. 118, Issue 1
Assessment of the effect of air pollution controls on trends in shortwave radiation over the United States from 1995 through 2010 from multiple observation networks
journal, January 2014
- Gan, C. -M.; Pleim, J.; Mathur, R.
- Atmospheric Chemistry and Physics, Vol. 14, Issue 3
Particulate sulfate ion concentration and SO 2 emission trends in the United States from the early 1990s through 2010
journal, January 2012
- Hand, J. L.; Schichtel, B. A.; Malm, W. C.
- Atmospheric Chemistry and Physics, Vol. 12, Issue 21
Factors affecting the detection of trends: Statistical considerations and applications to environmental data
journal, July 1998
- Weatherhead, Elizabeth C.; Reinsel, Gregory C.; Tiao, George C.
- Journal of Geophysical Research: Atmospheres, Vol. 103, Issue D14
Aerosol and cloud effects on solar brightening and the recent rapid warming: AEROSOL EFFECTS AND SOLAR BRIGHTENING
journal, June 2008
- Ruckstuhl, Christian; Philipona, Rolf; Behrens, Klaus
- Geophysical Research Letters, Vol. 35, Issue 12
Assessing boreal forest fire smoke aerosol impacts on U.S. air quality: A case study using multiple data sets: BIOMASS BURNING AIR QUALITY IMPACTS
journal, November 2011
- Miller, David J.; Sun, Kang; Zondlo, Mark A.
- Journal of Geophysical Research: Atmospheres, Vol. 116, Issue D22
Estimating the impact of the 2004 Alaskan forest fires on episodic particulate matter pollution over the eastern United States through assimilation of satellite-derived aerosol optical depths in a regional air quality model
journal, January 2008
- Mathur, Rohit
- Journal of Geophysical Research, Vol. 113, Issue D17
Model Representation of Secondary Organic Aerosol in CMAQv4.7
journal, November 2010
- Carlton, Annmarie G.; Bhave, Prakash V.; Napelenok, Sergey L.
- Environmental Science & Technology, Vol. 44, Issue 22
Scale effect and scale correction of land-surface albedo in rugged terrain
journal, September 2009
- Wen, Jianguang; Liu, Qiang; Liu, Qinhuo
- International Journal of Remote Sensing, Vol. 30, Issue 20
The roles of aerosol, water vapor and cloud in future global dimming/brightening
journal, January 2011
- Haywood, Jim M.; Bellouin, Nicolas; Jones, Andy
- Journal of Geophysical Research, Vol. 116, Issue D20
Uncertainties of simulated aerosol optical properties induced by assumptions on aerosol physical and chemical properties: An AQMEII-2 perspective
journal, August 2015
- Curci, G.; Hogrefe, C.; Bianconi, R.
- Atmospheric Environment, Vol. 115
Evaluation of dust and trace metal estimates from the Community Multiscale Air Quality (CMAQ) model version 5.0
journal, January 2013
- Appel, K. W.; Pouliot, G. A.; Simon, H.
- Geoscientific Model Development, Vol. 6, Issue 4
Observations and modeling of air quality trends over 1990–2010 across the Northern Hemisphere: China, the United States and Europe
journal, January 2015
- Xing, J.; Mathur, R.; Pleim, J.
- Atmospheric Chemistry and Physics, Vol. 15, Issue 5
Annual application and evaluation of the online coupled WRF–CMAQ system over North America under AQMEII phase 2
journal, August 2015
- Hogrefe, Christian; Pouliot, George; Wong, David
- Atmospheric Environment, Vol. 115
Impact of aerosol–meteorology interactions on fine particle pollution during China’s severe haze episode in January 2013
journal, September 2014
- Wang, Jiandong; Wang, Shuxiao; Jiang, Jingkun
- Environmental Research Letters, Vol. 9, Issue 9