A Local Quantum Phase Transition in YFe2Al10
Abstract
Here, a phase transition occurs when correlated regions of a new phase grow to span the system and the fluctuations within the correlated regions become long-lived. Here we present neutron scattering measurements showing that this conventional picture must be replaced by a new paradigm in YFe2Al10, a compound that forms naturally very close to a T = 0 quantum phase transition. Fully quantum mechanical fluctuations of localized moments are found to diverge at low energies and temperatures, however the fluctuating moments are entirely without spatial correlations. Zero temperature order in YFe2Al10 is achieved by a new and entirely local type of quantum phase transition that may originate with the creation of the moments themselves.
- Authors:
-
- Texas A & M Univ., College Station, TX (United States)
- Brookhaven National Lab. (BNL), Upton, NY (United States)
- Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States)
- National Inst. of Standards and Technology (NIST), Gaithersburg, MD (United States)
- National Inst. of Standards and Technology (NIST), Gaithersburg, MD (United States); Univ. of Maryland, College Park, MD (United States)
- Publication Date:
- Research Org.:
- Brookhaven National Laboratory (BNL), Upton, NY (United States)
- Sponsoring Org.:
- USDOE Office of Science (SC), Basic Energy Sciences (BES)
- OSTI Identifier:
- 1440349
- Report Number(s):
- BNL-205727-2018-JAAM
Journal ID: ISSN 0027-8424
- Grant/Contract Number:
- SC0012704
- Resource Type:
- Accepted Manuscript
- Journal Name:
- Proceedings of the National Academy of Sciences of the United States of America
- Additional Journal Information:
- Journal Volume: 115; Journal Issue: 27; Journal ID: ISSN 0027-8424
- Publisher:
- National Academy of Sciences, Washington, DC (United States)
- Country of Publication:
- United States
- Language:
- English
- Subject:
- 75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND SUPERFLUIDITY
Citation Formats
Gannon, W J., Zaliznyak, Igor A., Wu, L. S., Tsvelik, A. M., Qiu, Y., Rodriguez-Rivera, J. A., and Aronson, M. C. A Local Quantum Phase Transition in YFe2Al10. United States: N. p., 2018.
Web. doi:10.1073/pnas.1721493115.
Gannon, W J., Zaliznyak, Igor A., Wu, L. S., Tsvelik, A. M., Qiu, Y., Rodriguez-Rivera, J. A., & Aronson, M. C. A Local Quantum Phase Transition in YFe2Al10. United States. https://doi.org/10.1073/pnas.1721493115
Gannon, W J., Zaliznyak, Igor A., Wu, L. S., Tsvelik, A. M., Qiu, Y., Rodriguez-Rivera, J. A., and Aronson, M. C. Mon .
"A Local Quantum Phase Transition in YFe2Al10". United States. https://doi.org/10.1073/pnas.1721493115. https://www.osti.gov/servlets/purl/1440349.
@article{osti_1440349,
title = {A Local Quantum Phase Transition in YFe2Al10},
author = {Gannon, W J. and Zaliznyak, Igor A. and Wu, L. S. and Tsvelik, A. M. and Qiu, Y. and Rodriguez-Rivera, J. A. and Aronson, M. C.},
abstractNote = {Here, a phase transition occurs when correlated regions of a new phase grow to span the system and the fluctuations within the correlated regions become long-lived. Here we present neutron scattering measurements showing that this conventional picture must be replaced by a new paradigm in YFe2Al10, a compound that forms naturally very close to a T = 0 quantum phase transition. Fully quantum mechanical fluctuations of localized moments are found to diverge at low energies and temperatures, however the fluctuating moments are entirely without spatial correlations. Zero temperature order in YFe2Al10 is achieved by a new and entirely local type of quantum phase transition that may originate with the creation of the moments themselves.},
doi = {10.1073/pnas.1721493115},
journal = {Proceedings of the National Academy of Sciences of the United States of America},
number = 27,
volume = 115,
place = {United States},
year = {Mon Jun 18 00:00:00 EDT 2018},
month = {Mon Jun 18 00:00:00 EDT 2018}
}
Web of Science
Figures / Tables:
Works referenced in this record:
Equilibrium behaviour of quantum Ising spin glass
journal, March 1995
- Thill, M. J.; Huse, D. A.
- Physica A: Statistical Mechanics and its Applications, Vol. 214, Issue 3
Field-induced quantum fluctuations in the heavy fermion superconductor CeCu2Ge2
journal, October 2011
- Singh, D. K.; Thamizhavel, A.; Lynn, J. W.
- Scientific Reports, Vol. 1, Issue 1
Strange metal without magnetic criticality
journal, July 2015
- Tomita, T.; Kuga, K.; Uwatoko, Y.
- Science, Vol. 349, Issue 6247
Hall-effect evolution across a heavy-fermion quantum critical point
journal, December 2004
- Paschen, S.; Lühmann, T.; Wirth, S.
- Nature, Vol. 432, Issue 7019
Theory of dynamic critical phenomena
journal, July 1977
- Hohenberg, P. C.; Halperin, B. I.
- Reviews of Modern Physics, Vol. 49, Issue 3
Quantum critical fluctuations in layered YFe 2 Al 10
journal, September 2014
- Wu, L. S.; Kim, M. S.; Park, K.
- Proceedings of the National Academy of Sciences, Vol. 111, Issue 39
Quantum criticality in the two-dimensional dissipative quantum XY model
journal, December 2016
- Zhu, Lijun; Hou, Changtao; Varma, Chandra M.
- Physical Review B, Vol. 94, Issue 23
Non-Fermi-liquid behavior in U and Ce alloys: Criticality, disorder, dissipation, and Griffiths-McCoy singularities
journal, December 2000
- Castro Neto, A. H.; Jones, B. A.
- Physical Review B, Vol. 62, Issue 22
Quantum critical response function in quasi-two-dimensional itinerant antiferromagnets
journal, October 2015
- Varma, C. M.; Zhu, Lijun; Schröder, Almut
- Physical Review B, Vol. 92, Issue 15
Detaching the antiferromagnetic quantum critical point from the Fermi-surface reconstruction in YbRh2Si2
journal, May 2009
- Friedemann, S.; Westerkamp, T.; Brando, M.
- Nature Physics, Vol. 5, Issue 7
Anomalous quantum critical spin dynamics in
journal, April 2018
- Huang, K.; Tan, C.; Zhang, J.
- Physical Review B, Vol. 97, Issue 15
Extended versus Local Fluctuations in Quantum Critical ( )
journal, August 2003
- Montfrooij, W.; Aronson, M. C.; Rainford, B. D.
- Physical Review Letters, Vol. 91, Issue 8
Onset of antiferromagnetism in heavy-fermion metals
journal, September 2000
- Schröder, A.; Aeppli, G.; Coldea, R.
- Nature, Vol. 407, Issue 6802
Evidence for a Non-Fermi-Liquid Phase in Ge-Substituted
journal, May 2010
- Custers, J.; Gegenwart, P.; Geibel, C.
- Physical Review Letters, Vol. 104, Issue 18
MACS—a new high intensity cold neutron spectrometer at NIST
journal, January 2008
- Rodriguez, J. A.; Adler, D. M.; Brand, P. C.
- Measurement Science and Technology, Vol. 19, Issue 3
Kinetic frustration and the nature of the magnetic and paramagnetic states in iron pnictides and iron chalcogenides
journal, September 2011
- Yin, Z. P.; Haule, K.; Kotliar, G.
- Nature Materials, Vol. 10, Issue 12
Antiferromagnetic criticality at a heavy-fermion quantum phase transition
journal, September 2009
- Knafo, W.; Raymond, S.; Lejay, P.
- Nature Physics, Vol. 5, Issue 10
Crystal structure of yttrium iron aluminium (1/2/10), YFe2Al10
journal, September 2012
- Kerkau, Alexander
- Zeitschrift für Kristallographie - New Crystal Structures, Vol. 227, Issue 3
Disorder-driven non-Fermi liquid behaviour of correlated electrons
journal, August 2005
- Miranda, E.; Dobrosavljević, V.
- Reports on Progress in Physics, Vol. 68, Issue 10
Locally critical quantum phase transitions in strongly correlated metals
journal, October 2001
- Si, Qimiao; Rabello, Silvio; Ingersent, Kevin
- Nature, Vol. 413, Issue 6858
Field-tuned Fermi liquid in quantum critical YFe Al
journal, September 2011
- Park, K.; Wu, L. S.; Janssen, Y.
- Physical Review B, Vol. 84, Issue 9
Phenomenology of the normal state of Cu-O high-temperature superconductors
journal, October 1989
- Varma, C. M.; Littlewood, P. B.; Schmitt-Rink, S.
- Physical Review Letters, Vol. 63, Issue 18
Orbital-Selective Mott Transition out of Band Degeneracy Lifting
journal, March 2009
- de’ Medici, Luca; Hassan, S. R.; Capone, Massimo
- Physical Review Letters, Vol. 102, Issue 12
Spin dynamics near a putative antiferromagnetic quantum critical point in Cu-substituted and its relation to high-temperature superconductivity
journal, December 2015
- Kim, M. G.; Wang, M.; Tucker, G. S.
- Physical Review B, Vol. 92, Issue 21
Weak magnetism and non-Fermi liquids near heavy-fermion critical points
journal, January 2004
- Senthil, T.; Vojta, Matthias; Sachdev, Subir
- Physical Review B, Vol. 69, Issue 3
Random transverse field Ising spin chains
journal, July 1992
- Fisher, Daniel S.
- Physical Review Letters, Vol. 69, Issue 3
Non-Fermi-Liquid Scaling of the Magnetic Response in UCu
journal, July 1995
- Aronson, M. C.; Osborn, R.; Robinson, R. A.
- Physical Review Letters, Vol. 75, Issue 4
Mott Transition and Kondo Screening in -Electron Metals
journal, August 2005
- de’ Medici, L.; Georges, A.; Kotliar, G.
- Physical Review Letters, Vol. 95, Issue 6
Quantum Griffiths effects in itinerant Heisenberg magnets
journal, July 2005
- Vojta, Thomas; Schmalian, Jörg
- Physical Review B, Vol. 72, Issue 4
Quantum magnetism and criticality
journal, March 2008
- Sachdev, Subir
- Nature Physics, Vol. 4, Issue 3
Ternary aluminides LnT2Al10 (Ln=Y, La–Nd, Sm, Gd–Lu andT=Fe, Ru, Os) with YbFe2Al10 type structure and magneticproperties of the iron-containing series
journal, January 1998
- Thiede, Verena M. T.; Ebel, Thomas; Jeitschko, Wolfgang
- Journal of Materials Chemistry, Vol. 8, Issue 1
Magnetic fluctuations in
journal, February 1991
- Hayden, S. M.; Aeppli, G.; Mook, H.
- Physical Review Letters, Vol. 66, Issue 6
Quantum Criticality Without Tuning in the Mixed Valence Compound -YbAlB4
journal, January 2011
- Matsumoto, Y.; Nakatsuji, S.; Kuga, K.
- Science, Vol. 331, Issue 6015
Coherence–incoherence crossover in the normal state of iron oxypnictides and importance of Hund's rule coupling
journal, February 2009
- Haule, K.; Kotliar, G.
- New Journal of Physics, Vol. 11, Issue 2
Orbital-Selective Mott Transitions: Heavy Fermions and Beyond
journal, August 2010
- Vojta, Matthias
- Journal of Low Temperature Physics, Vol. 161, Issue 1-2
Effect of a nonzero temperature on quantum critical points in itinerant fermion systems
journal, September 1993
- Millis, A. J.
- Physical Review B, Vol. 48, Issue 10
How do Fermi liquids get heavy and die?
journal, August 2001
- Coleman, P.; Pépin, C.; Si, Qimiao
- Journal of Physics: Condensed Matter, Vol. 13, Issue 35
Normal-state spin dynamics and temperature-dependent spin-resonance energy in optimally doped BaFe1.85Co0.15As2
journal, December 2009
- Inosov, D. S.; Park, J. T.; Bourges, P.
- Nature Physics, Vol. 6, Issue 3
Scaling Behavior of the Generalized Susceptibility in
journal, September 1991
- Keimer, B.; Birgeneau, R. J.; Cassanho, A.
- Physical Review Letters, Vol. 67, Issue 14
Phase diagram and correlation functions of the two-dimensional dissipative quantum XY model
journal, November 2016
- Hou, Changtao; Varma, Chandra M.
- Physical Review B, Vol. 94, Issue 20
Orbital-selective Mott-insulator transition in Ca 2 - x Sr x RuO 4
journal, February 2002
- Anisimov, V. I.; Nekrasov, I. A.; Kondakov, D. E.
- The European Physical Journal B, Vol. 25, Issue 2
Critical Fermi surfaces and non-Fermi liquid metals
journal, July 2008
- Senthil, T.
- Physical Review B, Vol. 78, Issue 3
Spin Fluctuations in Itinerant Electron Magnetism
book, January 1985
- Moriya, Tôru
- Springer Series in Solid-State Sciences
wannier90: A tool for obtaining maximally-localised Wannier functions
dataset, January 2019
- Mostofi, Arash A.
- Mendeley
Onset of antiferromagnetism in heavy-fermion metals
journal, September 2000
- Schröder, A.; Aeppli, G.; Coldea, R.
- Nature, Vol. 407, Issue 6802
Hall-effect evolution across a heavy-fermion quantum critical point
journal, December 2004
- Paschen, S.; Lühmann, T.; Wirth, S.
- Nature, Vol. 432, Issue 7019
Absolute cross-section normalization of magnetic neutron scattering data
journal, August 2013
- Xu, Guangyong; Xu, Zhijun; Tranquada, J. M.
- Review of Scientific Instruments, Vol. 84, Issue 8
Strange metal without magnetic criticality
journal, July 2015
- Tomita, T.; Kuga, K.; Uwatoko, Y.
- Science, Vol. 349, Issue 6247
Crystal structure of yttrium iron aluminium (1/2/10), YFe2Al10
journal, September 2012
- Kerkau, Alexander
- Zeitschrift für Kristallographie - New Crystal Structures, Vol. 227, Issue 3
Coherence-incoherence crossover in the normal state of iron-oxypnictides and importance of the Hund's rule coupling
text, January 2008
- Haule, K.; Kotliar, G.
- arXiv
Evidence for a Non-Fermi-Liquid Phase in Ge-Substituted YbRh2Si2
text, January 2010
- Custers, J.; Gegenwart, P.; Geibel, C.
- arXiv
High-throughput electronic band structure calculations: challenges and tools
text, January 2010
- Setyawan, Wahyu; Curtarolo, Stefano
- arXiv
Disorder-Driven Non-Fermi Liquid Behavior of Correlated Electrons
text, January 2005
- Miranda, E.; Dobrosavljevic, V.
- arXiv