Ion-momentum imaging of dissociative attachment of electrons to molecules

Slaughter, D. S.; Belkacem, A.; McCurdy, C. W.; Rescigno, T. N.; Haxton, D. J.

doi:10.1088/0953-4075/49/22/222001

Title: Ion-momentum imaging of dissociative attachment of electrons to molecules

Abstract

Here, we present an overview of experiments and theory relevant to dissociative electron attachment studied by momentum imaging. We describe several key examples of characteristic transient anion dynamics in the form of small polyatomic electron-molecule systems. In each of these examples the so-called axial recoil approximation is found to break down due to correlation of the electronic and nuclear degrees of freedom of the transient anion. Guided by anion fragment momentum measurements and predictions of the electron scattering attachment probability in the molecular frame, we demonstrate that accurate predictions of the dissociation dynamics can be achieved without a detailed investigation of the surface topology of the relevant electronic states or the fragment trajectories on those surfaces.

Authors:

Slaughter, D. S. ^[1]; Belkacem, A. ^[1]; McCurdy, C. W. ^[2]; Rescigno, T. N. ^[1]; Haxton, D. J. ^[1]

Lawrence Berkeley National Laboratory (LBNL), Berkeley, CA (United States). Chemical Sciences
Lawrence Berkeley National Laboratory (LBNL), Berkeley, CA (United States). Chemical Sciences; Univ. of California, Davis, CA (United States). Dept. of Chemistry

Publication Date:: Mon Oct 24 00:00:00 EDT 2016

Research Org.:: Lawrence Berkeley National Laboratory (LBNL), Berkeley, CA (United States)

Sponsoring Org.:: USDOE Office of Science (SC), Basic Energy Sciences (BES). Chemical Sciences, Geosciences, and Biosciences Division

OSTI Identifier:: 1436602

Grant/Contract Number:: AC02-05CH11231

Resource Type:: Accepted Manuscript

Journal Name:: Journal of Physics. B, Atomic, Molecular and Optical Physics

Additional Journal Information:: Journal Volume: 49; Journal Issue: 22; Journal ID: ISSN 0953-4075

Publisher:: IOP Publishing

Country of Publication:: United States

Language:: English

Subject:: 74 ATOMIC AND MOLECULAR PHYSICS; 38 RADIATION CHEMISTRY, RADIOCHEMISTRY, AND NUCLEAR CHEMISTRY

Citation Formats


                    Slaughter, D. S., Belkacem, A., McCurdy, C. W., Rescigno, T. N., and Haxton, D. J. Ion-momentum imaging of dissociative attachment of electrons to molecules.  United States: N. p., 2016. 
Web.  doi:10.1088/0953-4075/49/22/222001.

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                    Slaughter, D. S., Belkacem, A., McCurdy, C. W., Rescigno, T. N., & Haxton, D. J. Ion-momentum imaging of dissociative attachment of electrons to molecules.  United States.  https://doi.org/10.1088/0953-4075/49/22/222001

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                    Slaughter, D. S., Belkacem, A., McCurdy, C. W., Rescigno, T. N., and Haxton, D. J. Mon .  
"Ion-momentum imaging of dissociative attachment of electrons to molecules".  United States.  https://doi.org/10.1088/0953-4075/49/22/222001.  https://www.osti.gov/servlets/purl/1436602.

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@article{osti_1436602,

  title        = {Ion-momentum imaging of dissociative attachment of electrons to molecules},

  author       = {Slaughter, D. S. and Belkacem, A. and McCurdy, C. W. and Rescigno, T. N. and Haxton, D. J.},

  abstractNote = {Here, we present an overview of experiments and theory relevant to dissociative electron attachment studied by momentum imaging. We describe several key examples of characteristic transient anion dynamics in the form of small polyatomic electron-molecule systems. In each of these examples the so-called axial recoil approximation is found to break down due to correlation of the electronic and nuclear degrees of freedom of the transient anion. Guided by anion fragment momentum measurements and predictions of the electron scattering attachment probability in the molecular frame, we demonstrate that accurate predictions of the dissociation dynamics can be achieved without a detailed investigation of the surface topology of the relevant electronic states or the fragment trajectories on those surfaces.},

  doi          = {10.1088/0953-4075/49/22/222001},

  journal      = {Journal of Physics. B, Atomic, Molecular and Optical Physics},

  number       = 22,

  volume       = 49,

  place        = {United States},

  year         = {Mon Oct 24 00:00:00 EDT 2016},

  month        = {Mon Oct 24 00:00:00 EDT 2016}

}

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Figure 1: Left: A schematic illustration of the LBNL DEA reaction microscope. Right: Measured H⁻ kinetic energy distributions from DEA to H₂O at 6.3 eV, for different 3-dimensional momentum image analysis treatments illustrated inset. Solid curve: full 4π acceptance of the anion distribution; blue squares and green circles: slices parallelmore »

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DOI: 10.1103/PhysRevA.45.7800

Dissociative electron attachment resonances in ammonia: A velocity slice imaging based study
journal, April 2012

Ram, N. Bhargava; Krishnakumar, E.
The Journal of Chemical Physics, Vol. 136, Issue 16
DOI: 10.1063/1.4705358

Dissociative electron attachment to gas phase valine: A combined experimental and theoretical study
journal, November 2006

Papp, Peter; Urban, Jan; Matejčík, Štefan
The Journal of Chemical Physics, Vol. 125, Issue 20
DOI: 10.1063/1.2400236

Dissociative electron attachment to gas phase glycine: Exploring the decomposition pathways by mass separation of isobaric fragment anions
journal, January 2007

Mauracher, A.; Denifl, S.; Aleem, A.
Physical Chemistry Chemical Physics, Vol. 9, Issue 42
DOI: 10.1039/b709140k

Tautomerism in Cytosine and Uracil: An Experimental and Theoretical Core Level Spectroscopic Study
journal, May 2009

Feyer, Vitaliy; Plekan, Oksana; Richter, Robert
The Journal of Physical Chemistry A, Vol. 113, Issue 19
DOI: 10.1021/jp900998a

NCO–, a Key Fragment Upon Dissociative Electron Attachment and Electron Transfer to Pyrimidine Bases: Site Selectivity for a Slow Decay Process
journal, September 2013

da Silva, Filipe Ferreira; Matias, Carolina; Almeida, Diogo
Journal of The American Society for Mass Spectrometry, Vol. 24, Issue 11
DOI: 10.1007/s13361-013-0715-9

Dynamics of the Dissociating Uracil Anion Following Resonant Electron Attachment
journal, October 2014

Kawarai, Y.; Weber, Th.; Azuma, Y.
The Journal of Physical Chemistry Letters, Vol. 5, Issue 21
DOI: 10.1021/jz501907d

Colloquium : Aligning molecules with strong laser pulses
journal, April 2003

Stapelfeldt, Henrik; Seideman, Tamar
Reviews of Modern Physics, Vol. 75, Issue 2
DOI: 10.1103/RevModPhys.75.543

Electron Attachment to CO ₂ Embedded in Superfluid He Droplets
journal, April 2014

Postler, Johannes; Vizcaino, Violaine; Denifl, Stephan
The Journal of Physical Chemistry A, Vol. 118, Issue 33
DOI: 10.1021/jp503179d

Resonance-Enhanced Multiphoton Ionization Mass Spectrometry (REMPI-MS): Applications for Process Analysis
journal, June 2014

Streibel, Thorsten; Zimmermann, Ralf
Annual Review of Analytical Chemistry, Vol. 7, Issue 1
DOI: 10.1146/annurev-anchem-062012-092648

Mass-Analyzed Threshold Ionization (MATI) Spectroscopy of Atoms and Molecules Using VUV Synchrotron Radiation ^†
journal, December 2009

Kostko, Oleg; Kim, Sang Kyu; Leone, Stephen R.
The Journal of Physical Chemistry A, Vol. 113, Issue 52
DOI: 10.1021/jp9008338

Works referencing / citing this record:

Electron scattering from molecules and molecular aggregates of biological relevance
journal, September 2017

Gorfinkiel, Jimena D.; Ptasinska, Sylwia
Journal of Physics B: Atomic, Molecular and Optical Physics, Vol. 50, Issue 18
DOI: 10.1088/1361-6455/aa8572

Figures / Tables found in this record:

Figures/Tables have been extracted from DOE-funded journal article accepted manuscripts.

Similar Records in DOE PAGES and OSTI.GOV collections:

Dissociative electron attachment to carbon tetrachloride probed by velocity map imaging

Journal Article Paul, Anirban ; Nandi, Dhananjay ; Slaughter, Daniel S. ; ... - Physical Chemistry Chemical Physics. PCCP

Bond-breaking in CCl₄via dissociative electron attachment (DEA) has been studied using a velocity map imaging (VMI) spectrometer. A number of effects related to the dissociation dynamics have been revealed. The near-zero eV s-wave electron attachment, which leads to the production of Cl^- anions, is accompanied by a very efficient intramolecular vibrational redistribution. This is manifested by a small fraction of the excess energy being released in the form of the fragments' translation energy. A similar effect is observed for higher-lying electronic resonances with one exception: the resonance centered around 6.2 eV leads to the production of fast Cl₂^- fragments andmore »« less
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Imaging the molecular dynamics of dissociative electron attachment to water

Journal Article Adaniya, Hidihito ; Rudek, B ; Osipov, Timur ; ... - Physical Review Letters

Momentum imaging experiments on dissociative electron attachment to the water molecule are combined with ab initio theoretical calculations of the angular dependence of the quantum mechanical amplitude for electron attachment to provide a detailed picture of the molecular dynamics of dissociation attachment via the two lowest energy Feshbach resonances. The combination of momentum imaging experiments and theory can reveal dissociation dynamics for which the axial recoil approximation breaks down and thus provides a powerful reaction microscope for DEA to polyatomics.
https://doi.org/10.1103/PhysRevLett.103.233201

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Electron induced dissociation reactions are relevant to many fields, ranging from prebiotic chemistry to cancer treatments. However, the simulation of dissociation electron attachment (DEA) dynamics is very challenging because the auto-ionization widths of the transient negative ions must be accounted for. We propose an adaptation of the ab initio multiple spawning (AIMS) method for complex-valued potential energy surfaces, along the lines of recent developments based on surface hopping dynamics. Our approach combines models for the energy dependence of the auto-ionization widths, obtained from scattering calculations, with survival probabilities computed for the trajectory basis functions employed in the AIMS dynamics. The method is applied to simulate the DEA dynamics of 5-bromouracil in full dimensionality, i.e., taking all the vibrational modes into consideration. The propagation starts on themore »« less
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Electron attachment was studied in gaseous dinitrogen pentoxide, N{sub 2}O{sub 5}, for incident electron energies between a few meV and 10 eV. No stable parent anion N{sub 2}O{sub 5}{sup -} was observed but several anionic fragments (NO{sub 3}{sup -}, NO{sub 2}{sup -}, NO{sup -}, O{sup -}, and O{sub 2}{sup -}) were detected using quadrupole mass spectrometry. Many of these dissociative pathways were found to be coupled and provide detailed information on the dynamics of N{sub 2}O{sub 5} fragmentation. Estimates of the cross sections for production of each of the anionic fragments were made and suggest that electron attachment to N{submore »« less
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The angular dependence of dissociative electron attachment (DEA) to polyatomic targets is formulated in the local complex potential model, under the assumption that the axial recoil approximation describes the dissociation dynamics. An additional approximation, which is found to be valid in the case of H{sub 2}O but not in the case of H{sub 2}S, makes it possible to describe the angular dependence of DEA solely from an analysis of the fixed-nuclei entrance amplitude, without carrying out nuclear dynamics calculations. For H{sub 2}S, the final-vibrational-state-specific angular dependence of DEA is obtained by incorporating the variation of the angular dependence of themore »« less
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Title: Ion-momentum imaging of dissociative attachment of electrons to molecules

Abstract

Citation Formats

Figures / Tables:

Hybrid modelling of low temperature plasmas for fundamental investigations and equipment design journal, September 2009

Chemical Reactions in CF 2 Cl 2 /Water (Ice) Films Induced by X-ray Radiation journal, November 2003

Small, Minimally Invasive, Direct: Electrons Induce Local Reactions of Adsorbed Functional Molecules on the Nanoscale journal, September 2010

Site-Specific Dissociation of DNA Bases by Slow Electrons at Early Stages of Irradiation journal, April 2004

Resonances in Electron Impact on Diatomic Molecules journal, July 1973

Study of triplet states and short-lived negative ions by means of electron impact spectroscopy journal, January 1989

Gas phase negative ion chemistry journal, April 1989

Angular Distribution of O − from Dissociative Electron Attachment to O 2 journal, November 1970

Angular distribution of O − from dissociative electron attachment to NO journal, November 1974

Dissociative electron attachment in CO: angular distribution of the 0 - ions journal, April 1975

Dissociative electron attachment in H 2 O and D 2 O: energy and angular distribution of H - and D - fragments journal, November 1974

Vibrational excitation and dissociative attachment in the scattering of electrons by hydrogen molecules journal, October 1966

Configuration interaction in the continuum states of molecules journal, May 1968

Theory of Dissociative Attachment journal, October 1966

Recoil-ion and electron momentum spectroscopy: reaction-microscopes journal, August 2003

Cold Target Recoil Ion Momentum Spectroscopy: a ‘momentum microscope’ to view atomic collision dynamics journal, June 2000

A momentum imaging microscope for dissociative electron attachment journal, February 2012

Momentum-imaging apparatus for the study of dissociative electron attachment dynamics journal, March 2013

Two‐dimensional imaging of state‐selected photodissociation products detected by multiphoton ionization journal, July 1987

Velocity slice imaging for dissociative electron attachment journal, May 2005

Positive/negative ion velocity mapping apparatus for electron-molecule reactions journal, January 2012

From isolated molecules through clusters and condensates to the building blocks of life journal, November 2008

Electron impact dissociation of oxygen-containing molecules–A critical review journal, September 2008

Control of chemical reactions and synthesis by low-energy electrons journal, January 2013

Development of an ( e ,2 e ) electron momentum spectroscopy apparatus using an ultrashort pulsed electron gun journal, June 2013

Molecular Orbital Imaging of the Acetone S 2 Excited State Using Time-Resolved ( e , 2 e ) Electron Momentum Spectroscopy journal, March 2015

Coherent femtosecond low-energy single-electron pulses for time-resolved diffraction and imaging: A numerical study journal, December 2012

Ultrafast low-energy electron diffraction in transmission resolves polymer/graphene superstructure dynamics journal, July 2014

Energy partitioning in the O−/CO2 dissociative attachment journal, January 1985

Vibrational structures in electron CO 2 scattering below the 2 u shape resonance journal, August 2002

Selectivity in the Excitation of Fermi-Coupled Vibrations in CO 2 by Impact of Slow Electrons journal, June 2001

Cross Sections and Electron Affinity for O − Ions From O 2 , CO, and C O 2 by Electron Impact journal, October 1962

Vibrational Excitation of CO Fragments in Dissociative Attachment in C O 2 journal, February 1973

Interpretation of low-energy electron- CO 2 scattering journal, September 2002

Threshold Vibrational Excitation of C O 2 by Slow Electrons journal, February 2004

Potential energy surface of the CO2? anion journal, January 2004

Theoretical studies of low-energy electron- CO 2 scattering: Total, elastic, and differential cross sections journal, September 1999

Theoretical study of resonant vibrational excitation of CO 2 by electron impact journal, February 2002

Resonant vibrational excitation of CO 2 by electron impact: Nuclear dynamics on the coupled components of the 2 Π u resonance journal, April 2003

Electron-induced chemistry of alcohols journal, January 2007

Dissociative electron attachment in water and methanol (5–14 eV) journal, January 1992

Photodissociation of cyanogen: Angle and velocity distributions of state resolved fragments journal, December 1984

Recoil-ion momentum spectroscopy journal, July 1997

On the presence of the 4 Σ u − resonance in dissociative electron attachment to O 2 journal, June 2006

Probing site selective fragmentation of molecules containing hydroxyl group using Velocity Slice Imaging journal, September 2007

Imaging the Molecular Dynamics of Dissociative Electron Attachment to Water journal, November 2009

Quantum Superposition of Target and Product States in Reactive Electron Scattering from CF 4 Revealed through Velocity Slice Imaging journal, August 2013

Renner-Teller effect on dissociative electron attachment to carbon dioxide journal, May 2012

Dissociation dynamics in the dissociative electron attachment to carbon dioxide journal, May 2015

Momentum imaging of dissociative electron attachment in biologically relevant molecules journal, September 2015

Dissociative-electron-attachment dynamics near the 8-eV Feshbach resonance of CO 2 journal, August 2013

Multiple hit readout of a microchannel plate detector with a three-layer delay-line anode journal, October 2002

Theory of electron-molecule scattering: Comments on the adiabatic-nuclei approximation journal, November 1975

Theory of resonance and threshold effects in electron-molecule collisions: The projection-operator approach journal, October 1991

Vibrational excitation of N 2 by resonance scattering of electrons journal, January 1971

Complex potential and electron spectrum in atomic collisions involving fast electronic transitions: Penning and associative ionization journal, August 1978

Wave packet formulation of the boomerang model for resonant electron–molecule scattering journal, June 1983

Absolute cross sections from the "boomerang model" for resonant electron-molecule scattering journal, July 1979

Angular dependence of dissociative electron attachment to polyatomic molecules: Application to the B 1 2 metastable state of the H 2 O and H 2 S anions journal, June 2006

Allgemeine Quantentheorie der Stoßprozesse journal, January 1959

Behavior of Eigenphases near a Resonance journal, September 1970

The multiconfiguration time-dependent Hartree (MCTDH) method: a highly efficient algorithm for propagating wavepackets journal, January 2000

Signatures of bond formation and bond scission dynamics in dissociative electron attachment to methane journal, January 2015

Dissociative electron attachment to methyl acetate: evidence for ion/molecule complexes as intermediates journal, January 1991

Stabilization, fragmentation and rearrangement reactions in low-energy electron interaction with tetrafluoro-para-benzoquinone: a combined theoretical and experimental study journal, January 2013

Dissociative electron attachment to methane probed using velocity slice imaging journal, July 2011

Role of Conical Intersections in Molecular Spectroscopy and Photoinduced Chemical Dynamics journal, May 2012

Observation of the dynamics leading to a conical intersection in dissociative electron attachment to water journal, September 2011

Dynamics of dissociative electron attachment to ammonia journal, May 2016

Topology of the adiabatic potential energy surfaces for the resonance states of the water anion journal, August 2005

Dissociative electron attachment to the H 2 O molecule. II. Nuclear dynamics on coupled electronic surfaces within the local complex potential model journal, January 2007

Nonadiabatic theory of triatomics: General formalism and application to Renner–Teller and conical‐intersection effects journal, August 1988

Dynamics of dissociative attachment of electrons to water through the B 1 2 metastable state of the anion journal, June 2004

Vibrational excitation in C O 2 via the 3.8-eV resonance journal, May 1974

Elastic Scattering of Low-Energy Electrons at 180° in C O 2 journal, February 1972

Low-energy electron scattering from CO 2 molecules: elastic channel calculations revisited journal, April 2001

Hybrid modelling of low temperature plasmas for fundamental investigations and equipment design
journal, September 2009

Chemical Reactions in CF ₂ Cl ₂ /Water (Ice) Films Induced by X-ray Radiation
journal, November 2003

Small, Minimally Invasive, Direct: Electrons Induce Local Reactions of Adsorbed Functional Molecules on the Nanoscale
journal, September 2010

Site-Specific Dissociation of DNA Bases by Slow Electrons at Early Stages of Irradiation
journal, April 2004

Resonances in Electron Impact on Diatomic Molecules
journal, July 1973

Study of triplet states and short-lived negative ions by means of electron impact spectroscopy
journal, January 1989

Gas phase negative ion chemistry
journal, April 1989

Angular Distribution of $O^{-}$ from Dissociative Electron Attachment to $O_{2}$
journal, November 1970

Angular distribution of $O^{-}$ from dissociative electron attachment to NO
journal, November 1974

Dissociative electron attachment in CO: angular distribution of the 0 ^- ions
journal, April 1975

Dissociative electron attachment in H ₂ O and D ₂ O: energy and angular distribution of H ^- and D ^- fragments
journal, November 1974

Vibrational excitation and dissociative attachment in the scattering of electrons by hydrogen molecules
journal, October 1966

Configuration interaction in the continuum states of molecules
journal, May 1968

Theory of Dissociative Attachment
journal, October 1966

Recoil-ion and electron momentum spectroscopy: reaction-microscopes
journal, August 2003

Cold Target Recoil Ion Momentum Spectroscopy: a ‘momentum microscope’ to view atomic collision dynamics
journal, June 2000

A momentum imaging microscope for dissociative electron attachment
journal, February 2012

Momentum-imaging apparatus for the study of dissociative electron attachment dynamics
journal, March 2013

Two‐dimensional imaging of state‐selected photodissociation products detected by multiphoton ionization
journal, July 1987

Velocity slice imaging for dissociative electron attachment
journal, May 2005

Positive/negative ion velocity mapping apparatus for electron-molecule reactions
journal, January 2012

From isolated molecules through clusters and condensates to the building blocks of life
journal, November 2008

Electron impact dissociation of oxygen-containing molecules–A critical review
journal, September 2008

Control of chemical reactions and synthesis by low-energy electrons
journal, January 2013

Development of an ( e ,2 e ) electron momentum spectroscopy apparatus using an ultrashort pulsed electron gun
journal, June 2013

Molecular Orbital Imaging of the Acetone $S_{2}$ Excited State Using Time-Resolved ( $e$ , $2 e$ ) Electron Momentum Spectroscopy
journal, March 2015

Coherent femtosecond low-energy single-electron pulses for time-resolved diffraction and imaging: A numerical study
journal, December 2012

Ultrafast low-energy electron diffraction in transmission resolves polymer/graphene superstructure dynamics
journal, July 2014

Energy partitioning in the O−/CO2 dissociative attachment
journal, January 1985

Vibrational structures in electron CO ₂ scattering below the ² _u shape resonance
journal, August 2002

Selectivity in the Excitation of Fermi-Coupled Vibrations in ${CO}_{2}$ by Impact of Slow Electrons
journal, June 2001

Cross Sections and Electron Affinity for $O^{-}$ Ions From $O_{2}$ , CO, and C $O_{2}$ by Electron Impact
journal, October 1962

Vibrational Excitation of CO Fragments in Dissociative Attachment in C $O_{2}$
journal, February 1973

Interpretation of low-energy electron- ${CO}_{2}$ scattering
journal, September 2002

Threshold Vibrational Excitation of ${C O}_{2}$ by Slow Electrons
journal, February 2004

Potential energy surface of the CO2? anion
journal, January 2004

Theoretical studies of low-energy electron- ${CO}_{2}$ scattering: Total, elastic, and differential cross sections
journal, September 1999

Theoretical study of resonant vibrational excitation of ${CO}_{2}$ by electron impact
journal, February 2002

Resonant vibrational excitation of ${CO}_{2}$ by electron impact: Nuclear dynamics on the coupled components of the $^{2} Π_{u}$ resonance
journal, April 2003

Electron-induced chemistry of alcohols
journal, January 2007

Dissociative electron attachment in water and methanol (5–14 eV)
journal, January 1992

Photodissociation of cyanogen: Angle and velocity distributions of state resolved fragments
journal, December 1984

Recoil-ion momentum spectroscopy
journal, July 1997

On the presence of the ⁴ Σ _u ⁻ resonance in dissociative electron attachment to O ₂
journal, June 2006

Probing site selective fragmentation of molecules containing hydroxyl group using Velocity Slice Imaging
journal, September 2007

Imaging the Molecular Dynamics of Dissociative Electron Attachment to Water
journal, November 2009

Quantum Superposition of Target and Product States in Reactive Electron Scattering from ${CF}_{4}$ Revealed through Velocity Slice Imaging
journal, August 2013

Renner-Teller effect on dissociative electron attachment to carbon dioxide
journal, May 2012

Dissociation dynamics in the dissociative electron attachment to carbon dioxide
journal, May 2015

Momentum imaging of dissociative electron attachment in biologically relevant molecules
journal, September 2015

Dissociative-electron-attachment dynamics near the 8-eV Feshbach resonance of CO $_{2}$
journal, August 2013

Multiple hit readout of a microchannel plate detector with a three-layer delay-line anode
journal, October 2002

Theory of electron-molecule scattering: Comments on the adiabatic-nuclei approximation
journal, November 1975

Theory of resonance and threshold effects in electron-molecule collisions: The projection-operator approach
journal, October 1991

Vibrational excitation of N ₂ by resonance scattering of electrons
journal, January 1971

Complex potential and electron spectrum in atomic collisions involving fast electronic transitions: Penning and associative ionization
journal, August 1978

Wave packet formulation of the boomerang model for resonant electron–molecule scattering
journal, June 1983

Absolute cross sections from the "boomerang model" for resonant electron-molecule scattering
journal, July 1979

Angular dependence of dissociative electron attachment to polyatomic molecules: Application to the ${}^{2}B_{1}$ metastable state of the $H_{2} O$ and $H_{2} S$ anions
journal, June 2006

Allgemeine Quantentheorie der Stoßprozesse
journal, January 1959

Behavior of Eigenphases near a Resonance
journal, September 1970

The multiconfiguration time-dependent Hartree (MCTDH) method: a highly efficient algorithm for propagating wavepackets
journal, January 2000

Signatures of bond formation and bond scission dynamics in dissociative electron attachment to methane
journal, January 2015

Dissociative electron attachment to methyl acetate: evidence for ion/molecule complexes as intermediates
journal, January 1991

Stabilization, fragmentation and rearrangement reactions in low-energy electron interaction with tetrafluoro-para-benzoquinone: a combined theoretical and experimental study
journal, January 2013

Dissociative electron attachment to methane probed using velocity slice imaging
journal, July 2011

Role of Conical Intersections in Molecular Spectroscopy and Photoinduced Chemical Dynamics
journal, May 2012

Observation of the dynamics leading to a conical intersection in dissociative electron attachment to water
journal, September 2011

Dynamics of dissociative electron attachment to ammonia
journal, May 2016

Topology of the adiabatic potential energy surfaces for the resonance states of the water anion
journal, August 2005

Dissociative electron attachment to the $H_{2} O$ molecule. II. Nuclear dynamics on coupled electronic surfaces within the local complex potential model
journal, January 2007

Nonadiabatic theory of triatomics: General formalism and application to Renner–Teller and conical‐intersection effects
journal, August 1988

Dynamics of dissociative attachment of electrons to water through the ${}^{2}B_{1}$ metastable state of the anion
journal, June 2004

Vibrational excitation in C $O_{2}$ via the 3.8-eV resonance
journal, May 1974

Elastic Scattering of Low-Energy Electrons at 180° in C $O_{2}$
journal, February 1972

Low-energy electron scattering from CO ₂ molecules: elastic channel calculations revisited
journal, April 2001

Total Cross Sections for Ionization and Attachment in Gases by Electron Impact. II. Negative‐Ion Formation
journal, September 1965

Negative Ions of N ₂ O and CO ₂
journal, October 1969

Temperature Dependence of the Onset for Negative-Ion Formation in C $O_{2}$
journal, January 1969

Dissociative Attachment in Carbon Dioxide
journal, October 1972