Optical spectroscopy of laser-produced plasmas for standoff isotopic analysis
Abstract
This review article covers the present status of isotope detection through emission, absorption, and fluorescence spectroscopy of atoms and molecules in a laser-produced plasma formed from a solid sample. A description of the physics behind isotope shifts in atoms and molecules is presented, followed by the physics behind solid sampling of laser ablation plumes, optical methods for isotope measurements, the suitable physical conditions of laser-produced plasma plumes for isotopic analysis, and the current status. Finally, concluding remarks will be made on the existing gaps between previous works in the literature and suggestions for future work.
- Authors:
-
- Pacific Northwest National Lab. (PNNL), Richland, WA (United States)
- Pacific Northwest National Lab. (PNNL), Richland, WA (United States); Univ. of Florida, Gainesville, FL (United States)
- Publication Date:
- Research Org.:
- Pacific Northwest National Laboratory (PNNL), Richland, WA (United States)
- Sponsoring Org.:
- USDOE
- OSTI Identifier:
- 1437537
- Alternate Identifier(s):
- OSTI ID: 1434190; OSTI ID: 1513207
- Report Number(s):
- PNNL-SA-130702
Journal ID: ISSN 1931-9401; DN2001000; TRN: US1900331
- Grant/Contract Number:
- AC05-76RL01830
- Resource Type:
- Accepted Manuscript
- Journal Name:
- Applied Physics Reviews
- Additional Journal Information:
- Journal Volume: 5; Journal Issue: 2; Journal ID: ISSN 1931-9401
- Publisher:
- American Institute of Physics (AIP)
- Country of Publication:
- United States
- Language:
- English
- Subject:
- 70 PLASMA PHYSICS AND FUSION TECHNOLOGY; Isotope shifts; Laser-induced breakdown; Optical Sensing; Plasma Diagnostics; Fluorescence; Spectroscopy
Citation Formats
Harilal, S. S., Brumfield, B. E., LaHaye, N. L., Hartig, K. C., and Phillips, M. C. Optical spectroscopy of laser-produced plasmas for standoff isotopic analysis. United States: N. p., 2018.
Web. doi:10.1063/1.5016053.
Harilal, S. S., Brumfield, B. E., LaHaye, N. L., Hartig, K. C., & Phillips, M. C. Optical spectroscopy of laser-produced plasmas for standoff isotopic analysis. United States. https://doi.org/10.1063/1.5016053
Harilal, S. S., Brumfield, B. E., LaHaye, N. L., Hartig, K. C., and Phillips, M. C. Fri .
"Optical spectroscopy of laser-produced plasmas for standoff isotopic analysis". United States. https://doi.org/10.1063/1.5016053. https://www.osti.gov/servlets/purl/1437537.
@article{osti_1437537,
title = {Optical spectroscopy of laser-produced plasmas for standoff isotopic analysis},
author = {Harilal, S. S. and Brumfield, B. E. and LaHaye, N. L. and Hartig, K. C. and Phillips, M. C.},
abstractNote = {This review article covers the present status of isotope detection through emission, absorption, and fluorescence spectroscopy of atoms and molecules in a laser-produced plasma formed from a solid sample. A description of the physics behind isotope shifts in atoms and molecules is presented, followed by the physics behind solid sampling of laser ablation plumes, optical methods for isotope measurements, the suitable physical conditions of laser-produced plasma plumes for isotopic analysis, and the current status. Finally, concluding remarks will be made on the existing gaps between previous works in the literature and suggestions for future work.},
doi = {10.1063/1.5016053},
journal = {Applied Physics Reviews},
number = 2,
volume = 5,
place = {United States},
year = {Fri Apr 20 00:00:00 EDT 2018},
month = {Fri Apr 20 00:00:00 EDT 2018}
}
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