Evolution of ground-state wave function in upon Cd or Sn doping
Abstract
We present linear polarization-dependent soft-x-ray absorption spectroscopy data at the Ce M4,5 edges of Cd- and Sn-doped CeCoIn5. The 4f ground-state wave functions have been determined for their superconducting, antiferromagnetic, and paramagnetic ground states. The absence of changes in the wave functions in CeCo (In1- xCdx)5 suggests that the 4f-conduction-electron (c f) hybridization is not affected by global Cd doping, thus supporting the interpretation of magnetic droplets nucleating long-range magnetic order. This is contrasted by changes in the wave function due to Sn substitution. Increasing Sn in CeCo (In1 - ySny)5 compresses the 4f orbitals into the tetragonal plane of these materials, suggesting enhanced c f hybridization with the in-plane In(1) atoms and a homogeneous altering of the electronic structure. As these experiments show, the 4 f wave functions are a very sensitive probe of small changes in the hybridization of 4f and conduction electrons, even conveying information about direction dependencies.
- Authors:
-
[4];
[4];
[4];
- Univ. of Cologne (Germany). Inst. of Physics II
- Univ. of Cologne (Germany). Inst. of Physics II; Max Planck Inst. for Chemical Physics of Solids, Dresden (Germany)
- Max Planck Inst. for Chemical Physics of Solids, Dresden (Germany)
- Los Alamos National Lab. (LANL), Los Alamos, NM (United States)
- ALBA Synchrotron Light Source, Barcelona (Spain)
- European Synchrotron Radiation Facility (ESRF), Grenoble (France)
- Hiroshima Univ., Higahsi-Hiroshima (Japan). Dept. of Quantum Matter
- Publication Date:
- Research Org.:
- Los Alamos National Lab. (LANL), Los Alamos, NM (United States)
- Sponsoring Org.:
- USDOE Office of Science (SC), Basic Energy Sciences (BES); German Research Foundation (DFG)
- OSTI Identifier:
- 1431074
- Alternate Identifier(s):
- OSTI ID: 1417230
- Report Number(s):
- LA-UR-17-30510
Journal ID: ISSN 2469-9950; PRBMDO; TRN: US1802642
- Grant/Contract Number:
- AC52-06NA25396; NSF-DMR-1708199
- Resource Type:
- Accepted Manuscript
- Journal Name:
- Physical Review B
- Additional Journal Information:
- Journal Volume: 97; Journal Issue: 4; Journal ID: ISSN 2469-9950
- Publisher:
- American Physical Society (APS)
- Country of Publication:
- United States
- Language:
- English
- Subject:
- 36 MATERIALS SCIENCE; Material Science
Citation Formats
Chen, K., Strigari, F., Sundermann, M., Hu, Z., Fisk, Zachary, Bauer, Eric Dietzgen, Ferrari Silveira Rosa, Priscila, Sarrao, John Louis, Thompson, Joe David, Martin-Herero, J., Pellegrin, E., Betto, D., Kummer, K., Tanaka, A., Wirth, S., and Severing, A. Evolution of ground-state wave function in CeCoIn5 upon Cd or Sn doping. United States: N. p., 2018.
Web. doi:10.1103/PhysRevB.97.045134.
Chen, K., Strigari, F., Sundermann, M., Hu, Z., Fisk, Zachary, Bauer, Eric Dietzgen, Ferrari Silveira Rosa, Priscila, Sarrao, John Louis, Thompson, Joe David, Martin-Herero, J., Pellegrin, E., Betto, D., Kummer, K., Tanaka, A., Wirth, S., & Severing, A. Evolution of ground-state wave function in CeCoIn5 upon Cd or Sn doping. United States. https://doi.org/10.1103/PhysRevB.97.045134
Chen, K., Strigari, F., Sundermann, M., Hu, Z., Fisk, Zachary, Bauer, Eric Dietzgen, Ferrari Silveira Rosa, Priscila, Sarrao, John Louis, Thompson, Joe David, Martin-Herero, J., Pellegrin, E., Betto, D., Kummer, K., Tanaka, A., Wirth, S., and Severing, A. Wed .
"Evolution of ground-state wave function in CeCoIn5 upon Cd or Sn doping". United States. https://doi.org/10.1103/PhysRevB.97.045134. https://www.osti.gov/servlets/purl/1431074.
@article{osti_1431074,
title = {Evolution of ground-state wave function in CeCoIn5 upon Cd or Sn doping},
author = {Chen, K. and Strigari, F. and Sundermann, M. and Hu, Z. and Fisk, Zachary and Bauer, Eric Dietzgen and Ferrari Silveira Rosa, Priscila and Sarrao, John Louis and Thompson, Joe David and Martin-Herero, J. and Pellegrin, E. and Betto, D. and Kummer, K. and Tanaka, A. and Wirth, S. and Severing, A.},
abstractNote = {We present linear polarization-dependent soft-x-ray absorption spectroscopy data at the Ce M4,5 edges of Cd- and Sn-doped CeCoIn5. The 4f ground-state wave functions have been determined for their superconducting, antiferromagnetic, and paramagnetic ground states. The absence of changes in the wave functions in CeCo (In1- xCdx)5 suggests that the 4f-conduction-electron (c f) hybridization is not affected by global Cd doping, thus supporting the interpretation of magnetic droplets nucleating long-range magnetic order. This is contrasted by changes in the wave function due to Sn substitution. Increasing Sn in CeCo (In1 - ySny)5 compresses the 4f orbitals into the tetragonal plane of these materials, suggesting enhanced c f hybridization with the in-plane In(1) atoms and a homogeneous altering of the electronic structure. As these experiments show, the 4 f wave functions are a very sensitive probe of small changes in the hybridization of 4f and conduction electrons, even conveying information about direction dependencies.},
doi = {10.1103/PhysRevB.97.045134},
journal = {Physical Review B},
number = 4,
volume = 97,
place = {United States},
year = {Wed Jan 17 00:00:00 EST 2018},
month = {Wed Jan 17 00:00:00 EST 2018}
}
Free Publicly Available Full Text
Publisher's Version of Record
Other availability
Search WorldCat to find libraries that may hold this journal
Cited by: 16 works
Citation information provided by
Web of Science
Web of Science
Figures / Tables:
FIG. 1: (Color online) Temperature–doping phase diagram of CeCo(In1-xCdx)5 and CeCo(In1-ySny)5, adapted from. 24,25 Here, concentrations are given in %. The inset shows the crystallographic structure of CeCoIn5 with Ce (red orbital) in the middle, Co (grey), In(1) (yellow), and In(2) (dark yellow).
All figures and tables
(4 total)
Save to My Library
You must Sign In or Create an Account in order to save documents to your library.
Works referenced in this record:
-Electron Localization in with , Rh, or Ir
journal, October 2004
- Harrison, N.; Alver, U.; Goodrich, R. G.
- Physical Review Letters, Vol. 93, Issue 18
Theoretical Prediction and Spectroscopic Fingerprints of an Orbital Transition in
journal, March 2014
- Pourovskii, L. V.; Hansmann, P.; Ferrero, M.
- Physical Review Letters, Vol. 112, Issue 10
Design and performance of BOREAS, the beamline for resonant X-ray absorption and scattering experiments at the ALBA synchrotron light source
journal, October 2016
- Barla, Alessandro; Nicolás, Josep; Cocco, Daniele
- Journal of Synchrotron Radiation, Vol. 23, Issue 6
A Drastic Change of the Fermi Surface at a Critical Pressure in CeRhIn 5 : dHvA Study under Pressure
journal, April 2005
- Shishido, Hiroaki; Settai, Rikio; Harima, Hisatomo
- Journal of the Physical Society of Japan, Vol. 74, Issue 4
Strong Magnetic Fluctuations in a Superconducting State of
journal, January 2012
- Hu, T.; Xiao, H.; Sayles, T. A.
- Physical Review Letters, Vol. 108, Issue 5
Microscopic investigation of electronic inhomogeneity induced by substitutions in a quantum critical metal
journal, September 2015
- Sakai, H.; Ronning, F.; Zhu, J. -X.
- Physical Review B, Vol. 92, Issue 12
Crystal-field and Kondo-scale investigations of ( , Ir, and Rh): A combined x-ray absorption and inelastic neutron scattering study
journal, May 2010
- Willers, T.; Hu, Z.; Hollmann, N.
- Physical Review B, Vol. 81, Issue 19
Determining the Crystal-Field Ground State in Rare Earth Heavy Fermion Materials Using Soft-X-Ray Absorption Spectroscopy
journal, February 2008
- Hansmann, P.; Severing, A.; Hu, Z.
- Physical Review Letters, Vol. 100, Issue 6
Perturbing the Superconducting Planes in CeCoIn5 by Sn Substitution
journal, July 2005
- Daniel, M.; Bauer, E.; Han, S. -W.
- Physical Review Letters, Vol. 95, Issue 1
Quantitative study of the f occupation in CeMIn5 and other cerium compounds with hard X-rays
journal, May 2016
- Sundermann, M.; Strigari, F.; Willers, T.
- Journal of Electron Spectroscopy and Related Phenomena, Vol. 209
Erratum: Exploring heavy fermions from macroscopic to microscopic length scales
journal, January 2016
- Wirth, Steffen; Steglich, Frank
- Nature Reviews Materials, Vol. 1, Issue 1
Disorder in quantum critical superconductors
journal, December 2013
- Seo, S.; Lu, Xin; Zhu, J-X.
- Nature Physics, Vol. 10, Issue 2
Neutron scattering study of crystal fields in
journal, November 2002
- Christianson, A. D.; Lawrence, J. M.; Pagliuso, P. G.
- Physical Review B, Vol. 66, Issue 19
The high-field magnet endstation for X-ray magnetic dichroism experiments at ESRF soft X-ray beamline ID32
journal, February 2016
- Kummer, K.; Fondacaro, A.; Jimenez, E.
- Journal of Synchrotron Radiation, Vol. 23, Issue 2
Fermi-liquid instabilities at magnetic quantum phase transitions
journal, August 2007
- Löhneysen, Hilbert v.; Rosch, Achim; Vojta, Matthias
- Reviews of Modern Physics, Vol. 79, Issue 3
Occurrence of magnetism in (, Ir)
journal, April 2008
- Bauer, E. D.; Ronning, F.; Maquilon, S.
- Physica B: Condensed Matter, Vol. 403, Issue 5-9
Reversible Tuning of the Heavy-Fermion Ground State in
journal, August 2006
- Pham, L. D.; Park, Tuson; Maquilon, S.
- Physical Review Letters, Vol. 97, Issue 5
Unconventional Quantum Criticality in Heavy-Fermion Compounds
journal, March 2011
- Stockert, O.; Steglich, F.
- Annual Review of Condensed Matter Physics, Vol. 2, Issue 1
de Haas–van Alphen effect of
journal, March 2007
- Shishido, H.; Settai, R.; Kawai, T.
- Journal of Magnetism and Magnetic Materials, Vol. 310, Issue 2
Superconducting Quantum Critical Point in
journal, September 2010
- Ramos, S. M.; Fontes, M. B.; Hering, E. N.
- Physical Review Letters, Vol. 105, Issue 12
Magnetism and superconductivity driven by identical 4f states in a heavy-fermion metal
journal, May 2010
- Nair, S.; Stockert, O.; Witte, U.
- Proceedings of the National Academy of Sciences, Vol. 107, Issue 21
Superconductivity in : Veil over an Ordered State or Novel Quantum Critical Point?
journal, January 2005
- Bauer, E. D.; Capan, C.; Ronning, F.
- Physical Review Letters, Vol. 94, Issue 4
Progress in Heavy-Fermion Superconductivity: Ce115 and Related Materials
journal, January 2012
- D. Thompson, Joe; Fisk, Zachary
- Journal of the Physical Society of Japan, Vol. 81, Issue 1
Quasi-two-dimensional Fermi surfaces of the heavy fermion superconductor
journal, January 2001
- Haga, Yoshinori; Inada, Yoshihiko; Harima, Hisatomo
- Physical Review B, Vol. 63, Issue 6
Correlation between ground state and orbital anisotropy in heavy fermion materials
journal, February 2015
- Willers, Thomas; Strigari, Fabio; Hu, Zhiwei
- Proceedings of the National Academy of Sciences, Vol. 112, Issue 8
Local structure and site occupancy of Cd and Hg substitutions in ( , Rh, and Ir)
journal, April 2009
- Booth, C. H.; Bauer, E. D.; Bianchi, A. D.
- Physical Review B, Vol. 79, Issue 14
Fermi-Surface Reconstruction in
journal, July 2008
- Goh, Swee K.; Paglione, Johnpierre; Sutherland, Mike
- Physical Review Letters, Vol. 101, Issue 5
Local structure around Sn in
journal, April 2005
- Daniel, M.; Han, S. -W.; Booth, C. H.
- Physica B: Condensed Matter, Vol. 359-361
Resonant 3 d , 3 p and 3 s Photoemission in Transition Metal Oxides Predicted at 2 p Threshold
journal, July 1994
- Tanaka, Arata; Jo, Takeo
- Journal of the Physical Society of Japan, Vol. 63, Issue 7
Structurally tuned superconductivity in heavy-fermion CeMIn5 (MCo, Ir, Rh)
journal, July 2002
- Pagliuso, P. G.; Curro, N. J.; Moreno, N. O.
- Physica B: Condensed Matter, Vol. 320, Issue 1-4
Nearly localized nature of electrons in Ir)
journal, April 2003
- Fujimori, Shin-ichi; Okane, Tetsuo; Okamoto, Jun
- Physical Review B, Vol. 67, Issue 14
Recent Advances in Ce-Based Heavy-Fermion Superconductivity and Fermi Surface Properties
journal, May 2007
- Settai, Rikio; Takeuchi, Tetsuya; Ōnuki, Yoshichika
- Journal of the Physical Society of Japan, Vol. 76, Issue 5
Multiple phase transitions in Ce(Rh,Ir,Co)In5
journal, March 2002
- Pagliuso, P. G.; Movshovich, R.; Bianchi, A. D.
- Physica B: Condensed Matter, Vol. 312-313
Pressure effect on superconductivity in studied by thermal expansion
journal, May 2006
- Donath, J. G.; Gegenwart, P.; Küchler, R.
- Physica B: Condensed Matter, Vol. 378-380
Imaging Cooper pairing of heavy fermions in CeCoIn5
journal, July 2013
- Allan, M. P.; Massee, F.; Morr, D. K.
- Nature Physics, Vol. 9, Issue 8
Rapid suppression of superconductivity in
journal, April 2005
- Bauer, E. D.; Moreno, N. O.; Mixson, D. J.
- Physica B: Condensed Matter, Vol. 359-361
Crystalline electric field effects in : Superconductivity and the influence of Kondo spin fluctuations
journal, October 2004
- Christianson, A. D.; Bauer, E. D.; Lawrence, J. M.
- Physical Review B, Vol. 70, Issue 13
Modeling the Localized-to-Itinerant Electronic Transition in the Heavy Fermion System CeIrIn5
journal, December 2007
- Shim, J. H.; Haule, K.; Kotliar, G.
- Science, Vol. 318, Issue 5856
Optical signatures of momentum-dependent hybridization of the local moments and conduction electrons in Kondo lattices
journal, February 2007
- Burch, K. S.; Dordevic, S. V.; Mena, F. P.
- Physical Review B, Vol. 75, Issue 5
Magnetic structure of Cd-doped
journal, August 2007
- Nicklas, M.; Stockert, O.; Park, Tuson
- Physical Review B, Vol. 76, Issue 5
Thermodynamic and transport investigation of
journal, June 2006
- Bauer, E. D.; Ronning, F.; Capan, C.
- Physical Review B, Vol. 73, Issue 24
Heavy-fermion superconductivity in CeCoIn 5 at 2.3 K
journal, April 2001
- Petrovic, C.; Pagliuso, P. G.; Hundley, M. F.
- Journal of Physics: Condensed Matter, Vol. 13, Issue 17
Structural Tuning of Unconventional Superconductivity in ( )
journal, September 2004
- Bauer, E. D.; Thompson, J. D.; Sarrao, J. L.
- Physical Review Letters, Vol. 93, Issue 14
Works referencing / citing this record:
Spin rotation induced by applied pressure in the Cd-doped intermetallic compound
journal, October 2019
- Christovam, D. S.; Giles, C.; Mendonça-Ferreira, L.
- Physical Review B, Vol. 100, Issue 16
Figures / Tables found in this record:
Figures/Tables have been extracted from DOE-funded journal article accepted manuscripts.