Communication: Towards first principles theory of relaxation in supercooled liquids formulated in terms of cooperative motion

Freed, Karl F.

doi:10.1063/1.4897973

Title: Communication: Towards first principles theory of relaxation in supercooled liquids formulated in terms of cooperative motion

Authors:

Freed, Karl F. ^[1]

James Franck Institute and Department of Chemistry, University of Chicago, 929 East 57 Street, Chicago, Illinois 60637, USA

Publication Date:: Tue Oct 14 00:00:00 EDT 2014

Sponsoring Org.:: USDOE Office of Science (SC), Basic Energy Sciences (BES)

OSTI Identifier:: 1420699

Grant/Contract Number:: SC0008631

Resource Type:: Publisher's Accepted Manuscript

Journal Name:: Journal of Chemical Physics

Additional Journal Information:: Journal Name: Journal of Chemical Physics Journal Volume: 141 Journal Issue: 14; Journal ID: ISSN 0021-9606

Publisher:: American Institute of Physics

Country of Publication:: United States

Language:: English

Citation Formats


                    Freed, Karl F. Communication: Towards first principles theory of relaxation in supercooled liquids formulated in terms of cooperative motion.  United States: N. p., 2014. 
Web.  doi:10.1063/1.4897973.

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                    Freed, Karl F. Communication: Towards first principles theory of relaxation in supercooled liquids formulated in terms of cooperative motion.  United States.  https://doi.org/10.1063/1.4897973

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                    Freed, Karl F. Tue .  
"Communication: Towards first principles theory of relaxation in supercooled liquids formulated in terms of cooperative motion".  United States.  https://doi.org/10.1063/1.4897973.

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@article{osti_1420699,

  title        = {Communication: Towards first principles theory of relaxation in supercooled liquids formulated in terms of cooperative motion},

  author       = {Freed, Karl F.},

  abstractNote = {},

  doi          = {10.1063/1.4897973},

  journal      = {Journal of Chemical Physics},

  number       = 14,

  volume       = 141,

  place        = {United States},

  year         = {Tue Oct 14 00:00:00 EDT 2014},

  month        = {Tue Oct 14 00:00:00 EDT 2014}

}

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https://doi.org/10.1063/1.4897973

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Works referenced in this record:

Two glass transitions in miscible polymer blends?
journal, June 2014

Dudowicz, Jacek; Douglas, Jack F.; Freed, Karl F.
The Journal of Chemical Physics, Vol. 140, Issue 24
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Fragility of Glass-Forming Polymer Liquids ^†
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Dudowicz, Jacek; Freed, Karl F.; Douglas, Jack F.
The Journal of Physical Chemistry B, Vol. 109, Issue 45
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Kunal, Kumar; Robertson, Christopher G.; Pawlus, Sebastian
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Lattice model of equilibrium polymerization. IV. Influence of activation, chemical initiation, chain scission and fusion, and chain stiffness on polymerization and phase separation
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Dudowicz, Jacek; Freed, Karl F.; Douglas, Jack F.
The Journal of Chemical Physics, Vol. 119, Issue 23
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Modifying Fragility and Collective Motion in Polymer Melts with Nanoparticles
journal, March 2011

Starr, Francis W.; Douglas, Jack F.
Physical Review Letters, Vol. 106, Issue 11
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Cooperativity in self-limiting equilibrium self-associating systems
journal, November 2012

Freed, Karl F.
The Journal of Chemical Physics, Vol. 137, Issue 20
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The relationship of dynamical heterogeneity to the Adam-Gibbs and random first-order transition theories of glass formation
journal, March 2013

Starr, Francis W.; Douglas, Jack F.; Sastry, Srikanth
The Journal of Chemical Physics, Vol. 138, Issue 12
DOI: 10.1063/1.4790138

Dynamics of glass-forming liquids. V. On the link between molecular dynamics and configurational entropy
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Richert, R.; Angell, C. A.
The Journal of Chemical Physics, Vol. 108, Issue 21
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Stringlike Cooperative Motion in a Supercooled Liquid
journal, March 1998

Donati, Claudio; Douglas, Jack F.; Kob, Walter
Physical Review Letters, Vol. 80, Issue 11
DOI: 10.1103/PhysRevLett.80.2338

The Glass Transition Temperature of Polymer Melts ^†
journal, November 2005

Dudowicz, Jacek; Freed, Karl F.; Douglas, Jack F.
The Journal of Physical Chemistry B, Vol. 109, Issue 45
DOI: 10.1021/jp0523266

Entropy theory of polymer glass formation revisited. I. General formulation
journal, February 2006

Dudowicz, Jacek; Freed, Karl F.; Douglas, Jack F.
The Journal of Chemical Physics, Vol. 124, Issue 6
DOI: 10.1063/1.2166391

Influence of small rings on the thermodynamics of equilibrium self-assembly
journal, June 2012

Freed, Karl F.
The Journal of Chemical Physics, Vol. 136, Issue 24
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Influence of monomer molecular structure on the glass transition in polymers I. Lattice cluster theory for the configurational entropy
journal, September 2003

Freed, Karl F.
The Journal of Chemical Physics, Vol. 119, Issue 11
DOI: 10.1063/1.1600716

The Descent into Glass Formation in Polymer Fluids
journal, March 2011

Freed, Karl F.
Accounts of Chemical Research, Vol. 44, Issue 3
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Glassy interfacial dynamics of Ni nanoparticles: part I Colored noise, dynamic heterogeneity and collective atomic motion
journal, January 2013

Zhang, Hao; Douglas, Jack F.
Soft Matter, Vol. 9, Issue 4
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Influence of Monomer Molecular Structure on the Miscibility of Polymer Blends
book, January 2005

Freed, Karl F.; Dudowicz, Jacek
Phase Behaviour of Polymer Blends
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A thermodynamic connection to the fragility of glass-forming liquids
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Does equilibrium polymerization describe the dynamic heterogeneity of glass-forming liquids?
journal, October 2006

Douglas, Jack F.; Dudowicz, Jacek; Freed, Karl F.
The Journal of Chemical Physics, Vol. 125, Issue 14
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Direct computation of characteristic temperatures and relaxation times for glass-forming polymer liquids
journal, September 2005

Dudowicz, Jacek; Freed, Karl F.; Douglas, Jack F.
The Journal of Chemical Physics, Vol. 123, Issue 11
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Plasticization and antiplasticization of polymer melts diluted by low molar mass species
journal, February 2010

Stukalin, Evgeny B.; Douglas, Jack F.; Freed, Karl F.
The Journal of Chemical Physics, Vol. 132, Issue 8
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Through the Glass Lightly
journal, March 1995

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Current Status of Transition-State Theory
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The Journal of Physical Chemistry, Vol. 100, Issue 31
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String model for the dynamics of glass-forming liquids
journal, May 2014

Pazmiño Betancourt, Beatriz A.; Douglas, Jack F.; Starr, Francis W.
The Journal of Chemical Physics, Vol. 140, Issue 20
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Application of the entropy theory of glass formation to poly(α-olefins)
journal, September 2009

Stukalin, Evgeny B.; Douglas, Jack F.; Freed, Karl F.
The Journal of Chemical Physics, Vol. 131, Issue 11
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Evolution of collective motion in a model glass-forming liquid during physical aging
journal, March 2013

Shavit, Amit; Douglas, Jack F.; Riggleman, Robert A.
The Journal of Chemical Physics, Vol. 138, Issue 12
DOI: 10.1063/1.4775781

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Similar Records

Title: Communication: Towards first principles theory of relaxation in supercooled liquids formulated in terms of cooperative motion

Citation Formats

Two glass transitions in miscible polymer blends? journal, June 2014

Fragility of Glass-Forming Polymer Liquids † journal, November 2005

Role of Chemical Structure in Fragility of Polymers: A Qualitative Picture journal, October 2008

Lattice model of equilibrium polymerization. IV. Influence of activation, chemical initiation, chain scission and fusion, and chain stiffness on polymerization and phase separation journal, December 2003

Modifying Fragility and Collective Motion in Polymer Melts with Nanoparticles journal, March 2011

Cooperativity in self-limiting equilibrium self-associating systems journal, November 2012

The relationship of dynamical heterogeneity to the Adam-Gibbs and random first-order transition theories of glass formation journal, March 2013

Dynamics of glass-forming liquids. V. On the link between molecular dynamics and configurational entropy journal, June 1998

Stringlike Cooperative Motion in a Supercooled Liquid journal, March 1998

The Glass Transition Temperature of Polymer Melts † journal, November 2005

Entropy theory of polymer glass formation revisited. I. General formulation journal, February 2006

Influence of small rings on the thermodynamics of equilibrium self-assembly journal, June 2012

Influence of monomer molecular structure on the glass transition in polymers I. Lattice cluster theory for the configurational entropy journal, September 2003

The Descent into Glass Formation in Polymer Fluids journal, March 2011

Glassy interfacial dynamics of Ni nanoparticles: part I Colored noise, dynamic heterogeneity and collective atomic motion journal, January 2013

Influence of Monomer Molecular Structure on the Miscibility of Polymer Blends book, January 2005

A thermodynamic connection to the fragility of glass-forming liquids journal, April 2001

Does equilibrium polymerization describe the dynamic heterogeneity of glass-forming liquids? journal, October 2006

Direct computation of characteristic temperatures and relaxation times for glass-forming polymer liquids journal, September 2005

Plasticization and antiplasticization of polymer melts diluted by low molar mass species journal, February 2010

Through the Glass Lightly journal, March 1995

Current Status of Transition-State Theory journal, January 1996

String model for the dynamics of glass-forming liquids journal, May 2014

On the Temperature Dependence of Cooperative Relaxation Properties in Glass‐Forming Liquids journal, July 1965

Application of the entropy theory of glass formation to poly(α-olefins) journal, September 2009

Evolution of collective motion in a model glass-forming liquid during physical aging journal, March 2013

Two glass transitions in miscible polymer blends?
journal, June 2014

Fragility of Glass-Forming Polymer Liquids ^†
journal, November 2005

Role of Chemical Structure in Fragility of Polymers: A Qualitative Picture
journal, October 2008

Lattice model of equilibrium polymerization. IV. Influence of activation, chemical initiation, chain scission and fusion, and chain stiffness on polymerization and phase separation
journal, December 2003

Modifying Fragility and Collective Motion in Polymer Melts with Nanoparticles
journal, March 2011

Cooperativity in self-limiting equilibrium self-associating systems
journal, November 2012

The relationship of dynamical heterogeneity to the Adam-Gibbs and random first-order transition theories of glass formation
journal, March 2013

Dynamics of glass-forming liquids. V. On the link between molecular dynamics and configurational entropy
journal, June 1998

Stringlike Cooperative Motion in a Supercooled Liquid
journal, March 1998

The Glass Transition Temperature of Polymer Melts ^†
journal, November 2005

Entropy theory of polymer glass formation revisited. I. General formulation
journal, February 2006

Influence of small rings on the thermodynamics of equilibrium self-assembly
journal, June 2012

Influence of monomer molecular structure on the glass transition in polymers I. Lattice cluster theory for the configurational entropy
journal, September 2003

The Descent into Glass Formation in Polymer Fluids
journal, March 2011

Glassy interfacial dynamics of Ni nanoparticles: part I Colored noise, dynamic heterogeneity and collective atomic motion
journal, January 2013

Influence of Monomer Molecular Structure on the Miscibility of Polymer Blends
book, January 2005

A thermodynamic connection to the fragility of glass-forming liquids
journal, April 2001

Does equilibrium polymerization describe the dynamic heterogeneity of glass-forming liquids?
journal, October 2006

Direct computation of characteristic temperatures and relaxation times for glass-forming polymer liquids
journal, September 2005

Plasticization and antiplasticization of polymer melts diluted by low molar mass species
journal, February 2010

Through the Glass Lightly
journal, March 1995

Current Status of Transition-State Theory
journal, January 1996

String model for the dynamics of glass-forming liquids
journal, May 2014

On the Temperature Dependence of Cooperative Relaxation Properties in Glass‐Forming Liquids
journal, July 1965

Application of the entropy theory of glass formation to poly(α-olefins)
journal, September 2009

Evolution of collective motion in a model glass-forming liquid during physical aging
journal, March 2013