Correlated high-resolution x-ray diffraction photoluminescence and atom probe tomography analysis of continuous and discontinuous InxGa1-xN quantum wells
Abstract
In this study, atom probe tomography (APT) is used to characterize the influence of hydrogen dosing duringGaN barrier growth on the indium distribution of InxGa1-xN quantum wells, and correlatedmicro-photoluminescence is used to measure changes in the emission spectrum and efficiency. We found that relative to the control growth, hydrogen dosing leads to a 50% increase in emission intensity arising from discontinuous quantum wells that are narrower, of lower indium content, and with more abrupt interfaces. Additionally, simulations of carrier distributions based on APT composition profiles indicate that the greater carrier confinement leads to an increased radiative recombination rate. Furthermore, APT analysis of quantum well profiles enables refinement of x-ray diffractionanalysis for more accurate nondestructive measurements of composition.
- Authors:
-
- Northwestern Univ., Evanston, IL (United States)
- Sandia National Lab. (SNL-NM), Albuquerque, NM (United States)
- Publication Date:
- Research Org.:
- Energy Frontier Research Centers (EFRC) (United States). EFRC for Solid State Lighting Science (SSLS); Sandia National Lab. (SNL-NM), Albuquerque, NM (United States)
- Sponsoring Org.:
- USDOE National Nuclear Security Administration (NNSA)
- OSTI Identifier:
- 1235287
- Alternate Identifier(s):
- OSTI ID: 1420582
- Report Number(s):
- SAND-2015-5515J
Journal ID: ISSN 0003-6951; 594846
- Grant/Contract Number:
- AC04-94AL85000
- Resource Type:
- Accepted Manuscript
- Journal Name:
- Applied Physics Letters
- Additional Journal Information:
- Journal Volume: 107; Journal Issue: 02; Journal ID: ISSN 0003-6951
- Publisher:
- American Institute of Physics (AIP)
- Country of Publication:
- United States
- Language:
- English
- Subject:
- 36 MATERIALS SCIENCE; 46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND TECHNOLOGY; quantum wells; indium; photoluminescence; x-ray diffraction; III-V semiconductors
Citation Formats
Ren, Xiaochen, Riley, James R., Koleske, Daniel, and Lauhon, Lincoln J. Correlated high-resolution x-ray diffraction photoluminescence and atom probe tomography analysis of continuous and discontinuous InxGa1-xN quantum wells. United States: N. p., 2015.
Web. doi:10.1063/1.4926808.
Ren, Xiaochen, Riley, James R., Koleske, Daniel, & Lauhon, Lincoln J. Correlated high-resolution x-ray diffraction photoluminescence and atom probe tomography analysis of continuous and discontinuous InxGa1-xN quantum wells. United States. https://doi.org/10.1063/1.4926808
Ren, Xiaochen, Riley, James R., Koleske, Daniel, and Lauhon, Lincoln J. Tue .
"Correlated high-resolution x-ray diffraction photoluminescence and atom probe tomography analysis of continuous and discontinuous InxGa1-xN quantum wells". United States. https://doi.org/10.1063/1.4926808. https://www.osti.gov/servlets/purl/1235287.
@article{osti_1235287,
title = {Correlated high-resolution x-ray diffraction photoluminescence and atom probe tomography analysis of continuous and discontinuous InxGa1-xN quantum wells},
author = {Ren, Xiaochen and Riley, James R. and Koleske, Daniel and Lauhon, Lincoln J.},
abstractNote = {In this study, atom probe tomography (APT) is used to characterize the influence of hydrogen dosing duringGaN barrier growth on the indium distribution of InxGa1-xN quantum wells, and correlatedmicro-photoluminescence is used to measure changes in the emission spectrum and efficiency. We found that relative to the control growth, hydrogen dosing leads to a 50% increase in emission intensity arising from discontinuous quantum wells that are narrower, of lower indium content, and with more abrupt interfaces. Additionally, simulations of carrier distributions based on APT composition profiles indicate that the greater carrier confinement leads to an increased radiative recombination rate. Furthermore, APT analysis of quantum well profiles enables refinement of x-ray diffractionanalysis for more accurate nondestructive measurements of composition.},
doi = {10.1063/1.4926808},
journal = {Applied Physics Letters},
number = 02,
volume = 107,
place = {United States},
year = {Tue Jul 14 00:00:00 EDT 2015},
month = {Tue Jul 14 00:00:00 EDT 2015}
}
Web of Science
Works referenced in this record:
Atom Probe Tomography 2012
journal, August 2012
- Kelly, Thomas F.; Larson, David J.
- Annual Review of Materials Research, Vol. 42, Issue 1
Laser-assisted atom probe tomography of MBE grown GaN nanowire heterostructures: Laser-assisted atom probe tomography of MBE grown GaN nanowire heterostructures
journal, February 2014
- Sanford, N. A.; Blanchard, P. T.; Brubaker, M.
- physica status solidi (c), Vol. 11, Issue 3-4
Effect of interface grading and lateral thickness variation on x-ray diffraction by InGaN/GaN multiple quantum wells
journal, September 2012
- Lee, S. R.; Koleske, D. D.; Crawford, M. H.
- Journal of Crystal Growth, Vol. 355, Issue 1
Theoretical simulations of radiative recombination time in polar InGaN quantum wells
journal, May 2011
- Gladysiewicz, M.; Kudrawiec, R.; Syperek, M.
- physica status solidi (c), Vol. 8, Issue 7-8
Atom Probe Tomography Studies of GaN-Based Semiconductor Materials
journal, July 2009
- Bennett, Se; Oliver, Ra; Saxey, Dw
- Microscopy and Microanalysis, Vol. 15, Issue S2
Controlling indium incorporation in InGaN barriers with dilute hydrogen flows
journal, March 2014
- Koleske, D. D.; Wierer, J. J.; Fischer, A. J.
- Journal of Crystal Growth, Vol. 390
In surface segregation in InGaN/GaN quantum wells
journal, April 2003
- Dussaigne, A.; Damilano, B.; Grandjean, N.
- Journal of Crystal Growth, Vol. 251, Issue 1-4
On the increased efficiency in InGaN-based multiple quantum wells emitting at 530–590 nm with AlGaN interlayers
journal, April 2015
- Koleske, D. D.; Fischer, A. J.; Bryant, B. N.
- Journal of Crystal Growth, Vol. 415
Atom probe tomography assessment of the impact of electron beam exposure on In x Ga 1−x N/GaN quantum wells
journal, July 2011
- Bennett, Samantha E.; Saxey, David W.; Kappers, Menno J.
- Applied Physics Letters, Vol. 99, Issue 2
Effect of hydrogen during growth of quantum barriers on the properties of InGaN quantum wells
journal, March 2015
- Czernecki, Robert; Grzanka, Ewa; Smalc-Koziorowska, Julita
- Journal of Crystal Growth, Vol. 414
Indium segregation in InGaN quantum-well structures
journal, March 2000
- Duxbury, N.; Bangert, U.; Dawson, P.
- Applied Physics Letters, Vol. 76, Issue 12
Correlation of Microphotoluminescence Spectroscopy, Scanning Transmission Electron Microscopy, and Atom Probe Tomography on a Single Nano-object Containing an InGaN/GaN Multiquantum Well System
journal, December 2013
- Rigutti, Lorenzo; Blum, Ivan; Shinde, Deodatta
- Nano Letters, Vol. 14, Issue 1
Evaluation of strain and In content in (InGaN/GaN) multiquantum wells by x-ray analysis
journal, August 1999
- Krost, A.; Bläsing, J.; Lünenbürger, M.
- Applied Physics Letters, Vol. 75, Issue 5
Structural origin of V-defects and correlation with localized excitonic centers in InGaN/GaN multiple quantum wells
journal, February 1998
- Wu, X. H.; Elsass, C. R.; Abare, A.
- Applied Physics Letters, Vol. 72, Issue 6
Indium clustering in a -plane InGaN quantum wells as evidenced by atom probe tomography
journal, February 2015
- Tang, Fengzai; Zhu, Tongtong; Oehler, Fabrice
- Applied Physics Letters, Vol. 106, Issue 7
Structural analysis of InGaN epilayers
journal, July 2001
- O'Donnell, K. P.; Mosselmans, J. F. W.; Martin, R. W.
- Journal of Physics: Condensed Matter, Vol. 13, Issue 32
Three-Dimensional Atom-Probe Tomography: Advances and Applications
journal, August 2007
- Seidman, David N.
- Annual Review of Materials Research, Vol. 37, Issue 1
X-ray diffraction of III-nitrides
journal, February 2009
- Moram, M. A.; Vickers, M. E.
- Reports on Progress in Physics, Vol. 72, Issue 3
Three-Dimensional Mapping of Quantum Wells in a GaN/InGaN Core–Shell Nanowire Light-Emitting Diode Array
journal, August 2013
- Riley, James R.; Padalkar, Sonal; Li, Qiming
- Nano Letters, Vol. 13, Issue 9
Quantitative Chemical Mapping of InGaN Quantum Wells from Calibrated High-Angle Annular Dark Field Micrographs
journal, June 2015
- Carvalho, Daniel; Morales, Francisco M.; Ben, Teresa
- Microscopy and Microanalysis, Vol. 21, Issue 4
Indium Surface Segregation during Growth of (In,Ga)N/GaN Multiple Quantum Wells by Plasma-Assisted Molecular Beam Epitaxy
journal, November 2001
- Waltereit, P.; Brandt, O.; Ploog, K. H.
- physica status solidi (b), Vol. 228, Issue 1
Effect of growth interruption and the introduction of H[sub 2] on the growth of InGaN/GaN multiple quantum wells
journal, January 2000
- Moon, Yong-Tae; Kim, Dong-Joon; Song, Keun-Man
- Journal of Vacuum Science & Technology B: Microelectronics and Nanometer Structures, Vol. 18, Issue 6
In situ site-specific specimen preparation for atom probe tomography
journal, February 2007
- Thompson, K.; Lawrence, D.; Larson, D. J.
- Ultramicroscopy, Vol. 107, Issue 2-3
Toward Smart and Ultra-efficient Solid-State Lighting
journal, June 2014
- Tsao, Jeffrey Y.; Crawford, Mary H.; Coltrin, Michael E.
- Advanced Optical Materials, Vol. 2, Issue 9
Determination of the indium content and layer thicknesses in InGaN/GaN quantum wells by x-ray scattering
journal, August 2003
- Vickers, M. E.; Kappers, M. J.; Smeeton, T. M.
- Journal of Applied Physics, Vol. 94, Issue 3
Atomic-scale nanofacet structure in semipolar $(20\bar{2}\bar{1})$ and $(20\bar{2}1)$ InGaN single quantum wells
journal, January 2014
- Zhao, Yuji; Wu, Feng; Yang, Tsung-Jui
- Applied Physics Express, Vol. 7, Issue 2
Characterization of structures from X-ray scattering data using genetic algorithms
journal, October 1999
- Wormington, Matthew; Panaccione, Charles; Matney, Kevin M.
- Philosophical Transactions of the Royal Society of London. Series A: Mathematical, Physical and Engineering Sciences, Vol. 357, Issue 1761
Atom probe tomography characterisation of a laser diode structure grown by molecular beam epitaxy
journal, March 2012
- Bennett, Samantha E.; Smeeton, Tim M.; Saxey, David W.
- Journal of Applied Physics, Vol. 111, Issue 5
Influence of hydrogen on local phase separation in InGaN thin layers and properties of light-emitting structures based on them
journal, February 2011
- Tsatsulnikov, A. F.; Lundin, W. V.; Zavarin, E. E.
- Semiconductors, Vol. 45, Issue 2
Composition and interface analysis of InGaN/GaN multiquantum-wells on GaN substrates using atom probe tomography
journal, September 2014
- Liu, Fang; Huang, Li; Davis, Robert F.
- Journal of Vacuum Science & Technology B, Nanotechnology and Microelectronics: Materials, Processing, Measurement, and Phenomena, Vol. 32, Issue 5
Analyzing the physical properties of InGaN multiple quantum well light emitting diodes from nano scale structure
journal, August 2012
- Wu, Yuh-Renn; Shivaraman, Ravi; Wang, Kuang-Chung
- Applied Physics Letters, Vol. 101, Issue 8
Review of Atom Probe FIB-Based Specimen Preparation Methods
journal, November 2007
- Miller, Michael K.; Russell, Kaye F.; Thompson, Keith
- Microscopy and Microanalysis, Vol. 13, Issue 6
On the reliable analysis of indium mole fraction within In x Ga 1−x N quantum wells using atom probe tomography
journal, April 2014
- Riley, James R.; Detchprohm, Theeradetch; Wetzel, Christian
- Applied Physics Letters, Vol. 104, Issue 15
The impact of gross well width fluctuations on the efficiency of GaN-based light emitting diodes
journal, September 2013
- Oliver, R. A.; Massabuau, F. C. -P.; Kappers, M. J.
- Applied Physics Letters, Vol. 103, Issue 14
Works referencing / citing this record:
Impact of microscopic In fluctuations on the optical properties of InxGa1-xN blue light-emitting diodes assessed by low-energy X-ray fluorescence mapping using synchrotron radiation
journal, March 2019
- Sakaki, Atsushi; Funato, Mitsuru; Miyano, Munehiko
- Scientific Reports, Vol. 9, Issue 1
Indium segregation in N-polar InGaN quantum wells evidenced by energy dispersive X-ray spectroscopy and atom probe tomography
journal, April 2017
- Bonef, Bastien; Catalano, Massimo; Lund, Cory
- Applied Physics Letters, Vol. 110, Issue 14
Impact of microscopic In fluctuations on the optical properties of InxGa1-xN blue light-emitting diodes assessed by low-energy X-ray fluorescence mapping using synchrotron radiation
journal, March 2019
- Sakaki, Atsushi; Funato, Mitsuru; Miyano, Munehiko
- Scientific Reports, Vol. 9, Issue 1