LCLS in—photon out: fluorescence measurement of neon using soft x-rays
Abstract
Here, we measured the fluorescence photon yield of neon upon soft x-ray ionization (~1200 eV) from the x-ray free-electron laser at Linac Coherent Light Source, and demonstrated the usage of a grazing incidence spectrometer with a variable line spacing grating to perform x-ray fluorescence spectroscopy on a gas phase system. Our measurements also allowed us to estimate the focal size of the beam from the theoretical description developed, in terms of the rate equation approximation accounting for photoionization shake off of neutral neon and double auger decay of single core holes.
- Authors:
-
[1];
[2];
[4];
- Univ. of Connecticut, Storrs, CT (United States). Dept. of Physics
- Heidelberg Univ. (Germany). Inst. for Theoretische Chemie, Physikalisch-Chemisches
- SLAC National Accelerator Lab., Menlo Park, CA (United States)
- Helmholtz-Inst., Jena (Germany); Friedrich Schiller Univ., Jena (Germany). Theoretisch-Physikalisches Inst.
- Publication Date:
- Research Org.:
- SLAC National Accelerator Lab., Menlo Park, CA (United States)
- Sponsoring Org.:
- USDOE Office of Science (SC), Basic Energy Sciences (BES); German Federal Ministry of Education and Research (BMBF)
- OSTI Identifier:
- 1419969
- Grant/Contract Number:
- AC02-76SF00515; SC0002004; SC0012376; 05K16SJA
- Resource Type:
- Accepted Manuscript
- Journal Name:
- Journal of Physics. B, Atomic, Molecular and Optical Physics
- Additional Journal Information:
- Journal Volume: 51; Journal Issue: 3; Journal ID: ISSN 0953-4075
- Publisher:
- IOP Publishing
- Country of Publication:
- United States
- Language:
- English
- Subject:
- 74 ATOMIC AND MOLECULAR PHYSICS; Ionization; X-ray; Atomic system
Citation Formats
Obaid, Razib, Buth, Christian, Dakovski, Georgi L., Beerwerth, Randolf, Holmes, Michael, Aldrich, Jeff, Lin, Ming-Fu, Minitti, Michael, Osipov, Timur, Schlotter, William, Cederbaum, Lorenz S., Fritzsche, Stephan, and Berrah, Nora. LCLS in—photon out: fluorescence measurement of neon using soft x-rays. United States: N. p., 2018.
Web. doi:10.1088/1361-6455/aaa189.
Obaid, Razib, Buth, Christian, Dakovski, Georgi L., Beerwerth, Randolf, Holmes, Michael, Aldrich, Jeff, Lin, Ming-Fu, Minitti, Michael, Osipov, Timur, Schlotter, William, Cederbaum, Lorenz S., Fritzsche, Stephan, & Berrah, Nora. LCLS in—photon out: fluorescence measurement of neon using soft x-rays. United States. https://doi.org/10.1088/1361-6455/aaa189
Obaid, Razib, Buth, Christian, Dakovski, Georgi L., Beerwerth, Randolf, Holmes, Michael, Aldrich, Jeff, Lin, Ming-Fu, Minitti, Michael, Osipov, Timur, Schlotter, William, Cederbaum, Lorenz S., Fritzsche, Stephan, and Berrah, Nora. Tue .
"LCLS in—photon out: fluorescence measurement of neon using soft x-rays". United States. https://doi.org/10.1088/1361-6455/aaa189. https://www.osti.gov/servlets/purl/1419969.
@article{osti_1419969,
title = {LCLS in—photon out: fluorescence measurement of neon using soft x-rays},
author = {Obaid, Razib and Buth, Christian and Dakovski, Georgi L. and Beerwerth, Randolf and Holmes, Michael and Aldrich, Jeff and Lin, Ming-Fu and Minitti, Michael and Osipov, Timur and Schlotter, William and Cederbaum, Lorenz S. and Fritzsche, Stephan and Berrah, Nora},
abstractNote = {Here, we measured the fluorescence photon yield of neon upon soft x-ray ionization (~1200 eV) from the x-ray free-electron laser at Linac Coherent Light Source, and demonstrated the usage of a grazing incidence spectrometer with a variable line spacing grating to perform x-ray fluorescence spectroscopy on a gas phase system. Our measurements also allowed us to estimate the focal size of the beam from the theoretical description developed, in terms of the rate equation approximation accounting for photoionization shake off of neutral neon and double auger decay of single core holes.},
doi = {10.1088/1361-6455/aaa189},
journal = {Journal of Physics. B, Atomic, Molecular and Optical Physics},
number = 3,
volume = 51,
place = {United States},
year = {Tue Jan 09 00:00:00 EST 2018},
month = {Tue Jan 09 00:00:00 EST 2018}
}
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Cited by: 8 works
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Figures / Tables:
Figure 1: Vertical slice of the Liquid Jet Endstation showing the chamber with the variable line spacing grating spectrometer and the gas capillary.
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Works referencing / citing this record:
Photo-ionization and fragmentation of Sc 3 N@C 80 following excitation above the Sc K-edge
journal, September 2019
- Obaid, Razib; Schnorr, Kirsten; Wolf, Thomas J. A.
- The Journal of Chemical Physics, Vol. 151, Issue 10
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Figures / Tables found in this record:
Figures/Tables have been extracted from DOE-funded journal article accepted manuscripts.