DOE PAGES title logo U.S. Department of Energy
Office of Scientific and Technical Information

Title: Emergent reduced dimensionality by vertex frustration in artificial spin ice

Abstract

Reducing the dimensionality of a physical system can have a profound effect on its properties, as in the ordering of low-dimensional magnetic materials, phonon dispersion in mercury chain salts, sliding phases, and the electronic states of graphene. Here we explore the emergence of quasi-one-dimensional behaviour in two-dimensional artificial spin ice, a class of lithographically fabricated nanomagnet arrays used to study geometrical frustration. We extend the implementation of artificial spin ice by fabricating a new array geometry, the so-called tetris lattice. We demonstrate that the ground state of the tetris lattice consists of alternating ordered and disordered bands of nanomagnetic moments. The disordered bands can be mapped onto an emergent thermal one-dimensional Ising model. Furthermore, we show that the level of degeneracy associated with these bands dictates the susceptibility of island moments to thermally induced reversals, thus establishing that vertex frustration can reduce the relevant dimensionality of physical behaviour in a magnetic system.

Authors:
 [1];  [1];  [1];  [2];  [3];  [4];  [4];  [5]; ORCiD logo [6];  [1]
  1. Univ. of Illinois, Urbana-Champaign, IL (United States). Dept. of Physics and Frederick Seitz Materials Research Lab.
  2. Univ. of Minnesota, Minneapolis, MN (United States). Dept. of Chemical Engineering and Materials Science; Univ. of Cambridge (United Kingdom). Dept. of Physics
  3. Univ. of Minnesota, Minneapolis, MN (United States). Dept. of Chemical Engineering and Materials Science and School of Physics and Astronomy
  4. Univ. of Minnesota, Minneapolis, MN (United States). Dept. of Chemical Engineering and Materials Science
  5. Lawrence Berkeley National Lab. (LBNL), Berkeley, CA (United States)
  6. Los Alamos National Lab. (LANL), Los Alamos, NM (United States). Theoretical Division and Center for Nonlinear Studies
Publication Date:
Research Org.:
Lawrence Berkeley National Laboratory (LBNL), Berkeley, CA (United States); Los Alamos National Laboratory (LANL), Los Alamos, NM (United States)
Sponsoring Org.:
USDOE Office of Science (SC), Basic Energy Sciences (BES); National Science Foundation (NSF)
OSTI Identifier:
1377411
Alternate Identifier(s):
OSTI ID: 1418755
Report Number(s):
LA-UR-15-25679
Journal ID: ISSN 1745-2473; ark:/13030/qt8g58b8hs; TRN: US1702571
Grant/Contract Number:  
AC02-05CH11231; SC00170778; AC52-06NA253962; DMR-1420013; AC52-06NA25396
Resource Type:
Accepted Manuscript
Journal Name:
Nature Physics
Additional Journal Information:
Journal Volume: 12; Journal Issue: 2; Journal ID: ISSN 1745-2473
Publisher:
Nature Publishing Group (NPG)
Country of Publication:
United States
Language:
English
Subject:
36 MATERIALS SCIENCE; magnetic properties and materials; statistical physics

Citation Formats

Gilbert, Ian, Lao, Yuyang, Carrasquillo, Isaac, O’Brien, Liam, Watts, Justin D., Manno, Michael, Leighton, Chris, Scholl, Andreas, Nisoli, Cristiano, and Schiffer, Peter. Emergent reduced dimensionality by vertex frustration in artificial spin ice. United States: N. p., 2015. Web. doi:10.1038/nphys3520.
Gilbert, Ian, Lao, Yuyang, Carrasquillo, Isaac, O’Brien, Liam, Watts, Justin D., Manno, Michael, Leighton, Chris, Scholl, Andreas, Nisoli, Cristiano, & Schiffer, Peter. Emergent reduced dimensionality by vertex frustration in artificial spin ice. United States. https://doi.org/10.1038/nphys3520
Gilbert, Ian, Lao, Yuyang, Carrasquillo, Isaac, O’Brien, Liam, Watts, Justin D., Manno, Michael, Leighton, Chris, Scholl, Andreas, Nisoli, Cristiano, and Schiffer, Peter. Mon . "Emergent reduced dimensionality by vertex frustration in artificial spin ice". United States. https://doi.org/10.1038/nphys3520. https://www.osti.gov/servlets/purl/1377411.
@article{osti_1377411,
title = {Emergent reduced dimensionality by vertex frustration in artificial spin ice},
author = {Gilbert, Ian and Lao, Yuyang and Carrasquillo, Isaac and O’Brien, Liam and Watts, Justin D. and Manno, Michael and Leighton, Chris and Scholl, Andreas and Nisoli, Cristiano and Schiffer, Peter},
abstractNote = {Reducing the dimensionality of a physical system can have a profound effect on its properties, as in the ordering of low-dimensional magnetic materials, phonon dispersion in mercury chain salts, sliding phases, and the electronic states of graphene. Here we explore the emergence of quasi-one-dimensional behaviour in two-dimensional artificial spin ice, a class of lithographically fabricated nanomagnet arrays used to study geometrical frustration. We extend the implementation of artificial spin ice by fabricating a new array geometry, the so-called tetris lattice. We demonstrate that the ground state of the tetris lattice consists of alternating ordered and disordered bands of nanomagnetic moments. The disordered bands can be mapped onto an emergent thermal one-dimensional Ising model. Furthermore, we show that the level of degeneracy associated with these bands dictates the susceptibility of island moments to thermally induced reversals, thus establishing that vertex frustration can reduce the relevant dimensionality of physical behaviour in a magnetic system.},
doi = {10.1038/nphys3520},
journal = {Nature Physics},
number = 2,
volume = 12,
place = {United States},
year = {Mon Oct 26 00:00:00 EDT 2015},
month = {Mon Oct 26 00:00:00 EDT 2015}
}

Journal Article:
Free Publicly Available Full Text
Publisher's Version of Record

Citation Metrics:
Cited by: 100 works
Citation information provided by
Web of Science

Save / Share:

Works referenced in this record:

The unhappy wanderer
journal, August 2014


Nanoscale structure of the magnetic induction at monopole defects in artificial spin-ice lattices
journal, May 2011


Exploring thermally induced states in square artificial spin-ice arrays
journal, May 2013


Ignoring Your Neighbors: Moment Correlations Dominated by Indirect or Distant Interactions in an Ordered Nanomagnet Array
journal, September 2011


Crystallites of magnetic charges in artificial spin ice
journal, August 2013

  • Zhang, Sheng; Gilbert, Ian; Nisoli, Cristiano
  • Nature, Vol. 500, Issue 7464
  • DOI: 10.1038/nature12399

Direct observation of magnetic monopole defects in an artificial spin-ice system
journal, April 2010

  • Ladak, S.; Read, D. E.; Perkins, G. K.
  • Nature Physics, Vol. 6, Issue 5
  • DOI: 10.1038/nphys1628

Direct entropy determination and application to artificial spin ice
journal, July 2010

  • Lammert, Paul E.; Ke, Xianglin; Li, Jie
  • Nature Physics, Vol. 6, Issue 10
  • DOI: 10.1038/nphys1728

Thermal ground-state ordering and elementary excitations in artificial magnetic square ice
journal, November 2010

  • Morgan, Jason P.; Stein, Aaron; Langridge, Sean
  • Nature Physics, Vol. 7, Issue 1
  • DOI: 10.1038/nphys1853

Studies of nanomagnetism using synchrotron-based x-ray photoemission electron microscopy (X-PEEM)
journal, January 2012


Magnetic recording at 1.5 Pb m−2 using an integrated plasmonic antenna
journal, May 2010

  • Stipe, Barry C.; Strand, Timothy C.; Poon, Chie C.
  • Nature Photonics, Vol. 4, Issue 7
  • DOI: 10.1038/nphoton.2010.90

Real-space observation of emergent magnetic monopoles and associated Dirac strings in artificial kagome spin ice
journal, October 2010

  • Mengotti, Elena; Heyderman, Laura J.; Rodríguez, Arantxa Fraile
  • Nature Physics, Vol. 7, Issue 1
  • DOI: 10.1038/nphys1794

Characterization of domain wall–based traps for magnetic beads separation
journal, April 2012

  • Donolato, M.; Lofink, F.; Hankemeier, S.
  • Journal of Applied Physics, Vol. 111, Issue 7
  • DOI: 10.1063/1.3689009

Emergent ice rule and magnetic charge screening from vertex frustration in artificial spin ice
journal, August 2014

  • Gilbert, Ian; Chern, Gia-Wei; Zhang, Sheng
  • Nature Physics, Vol. 10, Issue 9
  • DOI: 10.1038/nphys3037

Emergent excitations in a geometrically frustrated magnet
journal, August 2002


Artificial ‘spin ice’ in a geometrically frustrated lattice of nanoscale ferromagnetic islands
journal, January 2006

  • Wang, R. F.; Nisoli, C.; Freitas, R. S.
  • Nature, Vol. 439, Issue 7074
  • DOI: 10.1038/nature04447

Thermal fluctuations in artificial spin ice
journal, June 2014

  • Kapaklis, Vassilios; Arnalds, Unnar B.; Farhan, Alan
  • Nature Nanotechnology, Vol. 9, Issue 7, p. 514-519
  • DOI: 10.1038/nnano.2014.104

Near-edge X-ray absorption fine-structure microscopy of organic and magnetic materials
journal, April 2009

  • Ade, Harald; Stoll, Herman
  • Nature Materials, Vol. 8, Issue 4
  • DOI: 10.1038/nmat2399

Propagation of magnetic charge monopoles and Dirac flux strings in an artificial spin-ice lattice
journal, May 2012


One-Dimensional Phonons and "Phase-Ordering" Phase Transition in Hg 3 δ As F 6
journal, December 1977


Colloquium : Artificial spin ice: Designing and imaging magnetic frustration
journal, October 2013

  • Nisoli, Cristiano; Moessner, Roderich; Schiffer, Peter
  • Reviews of Modern Physics, Vol. 85, Issue 4
  • DOI: 10.1103/RevModPhys.85.1473

The electronic properties of graphene
journal, January 2009

  • Castro Neto, A. H.; Guinea, F.; Peres, N. M. R.
  • Reviews of Modern Physics, Vol. 81, Issue 1, p. 109-162
  • DOI: 10.1103/RevModPhys.81.109

Exploring hyper-cubic energy landscapes in thermally active finite artificial spin-ice systems
journal, May 2013

  • Farhan, A.; Derlet, P. M.; Kleibert, A.
  • Nature Physics, Vol. 9, Issue 6
  • DOI: 10.1038/nphys2613

Experiments on simple magnetic model systems
journal, January 1974


Artificial ferroic systems: novel functionality from structure, interactions and dynamics
journal, August 2013


Direct Observation of Thermal Relaxation in Artificial Spin Ice
journal, August 2013


FePd 3 as a material for studying thermally active artificial spin ice systems
journal, June 2015


Unhappy vertices in artificial spin ice: new degeneracies from vertex frustration
journal, April 2013


Sliding Phases in XY Models, Crystals, and Cationic Lipid-DNA Complexes
journal, October 1999


Artificial ‘spin ice’ in a geometrically frustrated lattice of nanoscale ferromagnetic islands
journal, March 2007

  • Wang, R. F.; Nisoli, C.; Freitas, R. S.
  • Nature, Vol. 446, Issue 7131
  • DOI: 10.1038/nature05607

An Information Theory-Inspired Strategy for Design of Re-programmable Encrypted Graphene-based Coding Metasurfaces at Terahertz Frequencies
journal, April 2018


Experiments on simple magnetic model systems
journal, December 2001


The electronic properties of graphene
text, January 2007


Direct entropy determination and application to artificial spin ice
text, January 2012


Colloquium: Artificial spin ice: Designing and imaging magnetic frustration
text, January 2013


Sliding Phases in XY-Models, Crystals, and Cationic Lipid-DNA Complexes
text, January 1999


Works referencing / citing this record:

Photoemission Electron Microscopy
book, January 2019


Deliberate exotic magnetism via frustration and topology
journal, March 2017

  • Nisoli, Cristiano; Kapaklis, Vassilios; Schiffer, Peter
  • Nature Physics, Vol. 13, Issue 3
  • DOI: 10.1038/nphys4059

Ice rule fragility via topological charge transfer in artificial colloidal ice
journal, October 2018


A tunable magnetic metamaterial based on the dipolar four-state Potts model
journal, October 2018


Frustration and thermalization in an artificial magnetic quasicrystal
journal, December 2017


Classical topological order in the kinetics of artificial spin ice
journal, April 2018


Effect of FePd alloy composition on the dynamics of artificial spin ice
journal, March 2018


Direct-write of free-form building blocks for artificial magnetic 3D lattices
journal, April 2018


Thermally and field-driven mobility of emergent magnetic charges in square artificial spin ice
journal, November 2019


Magnetization dynamics of weakly interacting sub-100 nm square artificial spin ices
journal, December 2019


Advances in artificial spin ice
journal, November 2019

  • Skjærvø, Sandra H.; Marrows, Christopher H.; Stamps, Robert L.
  • Nature Reviews Physics, Vol. 2, Issue 1
  • DOI: 10.1038/s42254-019-0118-3

Thermally induced magnetic relaxation in square artificial spin ice
journal, November 2016

  • Andersson, M. S.; Pappas, S. D.; Stopfel, H.
  • Scientific Reports, Vol. 6, Issue 1
  • DOI: 10.1038/srep37097

Tuning magnetic ordering in a dipolar square-kite tessellation
journal, February 2018

  • Petersen, Charlotte F.; Farhan, Alan; Dhuey, Scott
  • Applied Physics Letters, Vol. 112, Issue 9
  • DOI: 10.1063/1.5014041

On the micromagnetic behavior of dipolar-coupled nanomagnets in defective square artificial spin ice systems
journal, December 2019

  • Keswani, Neeti; Das, Pintu
  • Journal of Applied Physics, Vol. 126, Issue 21
  • DOI: 10.1063/1.5127262

Ising-like behaviour of mesoscopic magnetic chains
journal, August 2018

  • Östman, Erik; Arnalds, Unnar B.; Kapaklis, Vassilios
  • Journal of Physics: Condensed Matter, Vol. 30, Issue 36
  • DOI: 10.1088/1361-648x/aad0c1

Nano-Ising
journal, February 2016


Topologically Nontrivial Magnon Bands in Artificial Square Spin Ices with Dzyaloshinskii-Moriya Interaction
journal, September 2017


Intermediate phase and pseudo phase transition in an artificial spin ice model
journal, July 2019


Characterization of switching field distributions in Ising-like magnetic arrays
journal, April 2017


Magnetization reversal in kagome artificial spin ice studied by first-order reversal curves
journal, October 2017


Colloquium : Ice rule and emergent frustration in particle ice and beyond
journal, December 2019

  • Ortiz-Ambriz, Antonio; Nisoli, Cristiano; Reichhardt, Charles
  • Reviews of Modern Physics, Vol. 91, Issue 4
  • DOI: 10.1103/revmodphys.91.041003

Rewritable artificial magnetic charge ice
journal, May 2016


Cooperative magnetic phenomena in artificial spin systems: spin liquids, Coulomb phase and fragmentation of magnetism – a colloquium
journal, March 2019


Magnetic Characterization of Direct-Write Free-Form Building Blocks for Artificial Magnetic 3D Lattices
journal, February 2018

  • Al Mamoori, Mohanad; Keller, Lukas; Pieper, Jonathan
  • Materials, Vol. 11, Issue 2
  • DOI: 10.3390/ma11020289

Ice Rule Fragility via Topological Charge Transfer in Artificial Colloidal Ice
text, January 2018


Characterization of switching field distributions in Ising-like magnetic arrays
text, January 2016


Thermally induced magnetic relaxation in square artificial spin ice
text, January 2016


Thermally and field-driven mobility of emergent magnetic charges in square artificial spin ice
text, January 2018


Nanoscale control of competing interactions and geometrical frustration in a dipolar trident lattice
journal, October 2017


Ice rule fragility via topological charge transfer in artificial colloidal ice
journal, October 2018


Thermally and field-driven mobility of emergent magnetic charges in square artificial spin ice
journal, November 2019


Magnetization dynamics of weakly interacting sub-100 nm square artificial spin ices
journal, December 2019


Magnetic Characterization of Direct-Write Free-Form Building Blocks for Artificial Magnetic 3D Lattices
journal, February 2018

  • Al Mamoori, Mohanad; Keller, Lukas; Pieper, Jonathan
  • Materials, Vol. 11, Issue 2
  • DOI: 10.3390/ma11020289