Materials for the Recovery of Uranium from Seawater

Abney, Carter W.; Mayes, Richard T.; Saito, Tomonori; Dai, Sheng

doi:10.1021/acs.chemrev.7b00355

Title: Materials for the Recovery of Uranium from Seawater

Journal Article · Wed Nov 22 04:00:00 UTC 2017 · Chemical Reviews

DOI: https://doi.org/10.1021/acs.chemrev.7b00355 · OSTI ID:1412046

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Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States)

More than 1000× uranium exists in the oceans than exists in terrestrial ores. With nuclear power generation expected to increase over the coming decades, access to this unconventional reserve is a matter of energy security. With origins in the mid-1950’s, materials have been developed for the selective recovery of seawater uranium for more than six decades, with a renewed interest in particular since 2010. This review comprehensively surveys materials developed from 2000 – 2016 for recovery of seawater uranium, in particular including recent developments in inorganic materials, polymer adsorbents and related research pertaining to amidoxime, and nanostructured materials such as metal-organic frameworks, porous-organic polymers, and mesoporous carbons. In conclusion, challenges of performing reliable and reproducible uranium adsorption studies are also discussed, as well as the standardization of parameters necessary to ensure valid comparisons between different adsorbents.

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Research Organization:: Oak Ridge National Laboratory (ORNL), Oak Ridge, TN (United States)

Sponsoring Organization:: USDOE Office of Nuclear Energy (NE), Fuel Cycle Technologies (NE-5)

Grant/Contract Number:: AC05-00OR22725

OSTI ID:: 1412046

Journal Information:: Chemical Reviews, Journal Name: Chemical Reviews Journal Issue: 23 Vol. 117; ISSN 0009-2665

Publisher:: American Chemical SocietyCopyright Statement

Country of Publication:: United States

Language:: English

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A uranium capture strategy based on self-assembly in a hydroxyl-functionalized ionic liquid extraction system Chen, Baihua; Wu, Kaige; Yang, Yanqiu Chemical Communications, Vol. 55, Issue 48 https://doi.org/10.1039/c9cc02823d	journal	January 2019
Complexation of UO ₂ (CO ₃ ) ₃ ⁴⁻ with Mg ²⁺ at varying temperatures and its effect on U( vi ) speciation in groundwater and seawater Jo, Yongheum; Kim, Hee-Kyung; Yun, Jong-Il Dalton Transactions, Vol. 48, Issue 39 https://doi.org/10.1039/c9dt03313k	journal	January 2019
A highly efficient uranium grabber derived from acrylic fiber for extracting uranium from seawater Pan, Horng-Bin; Wai, Chien M.; Kuo, Li-Jung Dalton Transactions, Vol. 49, Issue 9 https://doi.org/10.1039/c9dt04562g	journal	January 2020
3D hierarchical porous amidoxime fibers speed up uranium extraction from seawater Xu, Xiao; Zhang, Hongjun; Ao, Junxuan Energy & Environmental Science, Vol. 12, Issue 6 https://doi.org/10.1039/c9ee00626e	journal	January 2019
Metal–organic framework-based materials for the recovery of uranium from aqueous solutions Yang, Weiting; Pan, Qinhe; Song, Shuyan Inorganic Chemistry Frontiers, Vol. 6, Issue 8 https://doi.org/10.1039/c9qi00386j	journal	January 2019
Structural and computational characterization of a bridging zwitterionic-amidoxime uranyl complex Decato, Daniel A.; Berryman, Orion B. Organic Chemistry Frontiers, Vol. 6, Issue 7 https://doi.org/10.1039/c9qo00267g	journal	January 2019
Water-stable 2-D Zr MOFs with exceptional UO ₂ ²⁺ sorption capability Panagiotou, Nikos; Liatsou, Ioanna; Pournara, Anastasia Journal of Materials Chemistry A, Vol. 8, Issue 4 https://doi.org/10.1039/c9ta10701k	journal	January 2020
Detailed characterization of dioxouranium( vi ) complexes with a symmetrical tetradentate N ₂ O ₂ -benzil bis(isonicotinoyl hydrazone) ligand Sethi, Sipun; Panigrahi, Rachita; Paul, Avijit Kumar Dalton Transactions, Vol. 49, Issue 30 https://doi.org/10.1039/d0dt02014a	journal	January 2020
A water-stable cyano-functionalized metal-organic framework as an efficient adsorbent of uranyl ion Peng, Ying; Zhang, Xiaowen; Wu, Xiaoyan Materials Research Express, Vol. 6, Issue 12 https://doi.org/10.1088/2053-1591/ab5415	journal	November 2019
Oligonuclear Actinoid Complexes with Schiff Bases as Ligands—Older Achievements and Recent Progress Tsantis, Sokratis T.; Tzimopoulos, Demetrios I.; Holynska, Malgorzata International Journal of Molecular Sciences, Vol. 21, Issue 2 https://doi.org/10.3390/ijms21020555	journal	January 2020
Symbiotic Aerogel Fibers Made via In-Situ Gelation of Aramid Nanofibers with Polyamidoxime for Uranium Extraction Li, Juan; Wang, Jin; Wang, Wei Molecules, Vol. 24, Issue 9 https://doi.org/10.3390/molecules24091821	journal	May 2019

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