Attosecond transient absorption of a bound wave packet coupled to a smooth continuum
Abstract
Here, we investigate the possibility of using transient absorption of a coherent bound electron wave packet in hydrogen as an attosecond pulse characterization technique. In a recent work, we have shown that photoionization of such a coherent bound electron wave packet opens up for pulse characterization with unprecedented temporal accuracy—independent of the atomic structure—with maximal photoemission at all kinetic energies given a wave packet with zero relative phase. Here, we perform numerical propagation of the time-dependent Schrödinger equation and analytical calculations based on perturbation theory to show that the energy-resolved maximal absorption of photons from the attosecond pulse does not uniquely occur at a zero relative phase of the initial wave packet. Instead, maximal absorption occurs at different relative wave packet phases, distributed as a non-monotonous function with a smooth $$-\pi /2$$ shift across the central photon energy (given a Fourier-limited Gaussian pulse). Similar results are also found in helium. Our finding is surprising, because it implies that the energy-resolved photoelectrons are not mapped one-to-one with the energy-resolved absorbed photons of the attosecond pulse.
- Authors:
-
- Lund Univ., Lund (Sweden); Stockholm Univ., Stockholm (Sweden)
- Harvard-Smithsonian Center for Astrophysics, Cambridge, MA (United States); SLAC National Accelerator Lab., Menlo Park, CA (United States)
- Stockholm Univ., Stockholm (Sweden)
- Publication Date:
- Research Org.:
- SLAC National Accelerator Laboratory (SLAC), Menlo Park, CA (United States)
- Sponsoring Org.:
- USDOE
- OSTI Identifier:
- 1410602
- Grant/Contract Number:
- AC02-76SF00515; 2014-3724; 2016-03789
- Resource Type:
- Accepted Manuscript
- Journal Name:
- Journal of Optics
- Additional Journal Information:
- Journal Volume: 19; Journal Issue: 11; Journal ID: ISSN 2040-8978
- Publisher:
- IOP Publishing
- Country of Publication:
- United States
- Language:
- English
- Subject:
- 37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CHEMISTRY; 72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS; attosecond; transient absorption; ATAS; pulse characterization; continuum transition
Citation Formats
Dahlström, Jan Marcus, Pabst, Stefan, and Lindroth, Eva. Attosecond transient absorption of a bound wave packet coupled to a smooth continuum. United States: N. p., 2017.
Web. doi:10.1088/2040-8986/aa8a93.
Dahlström, Jan Marcus, Pabst, Stefan, & Lindroth, Eva. Attosecond transient absorption of a bound wave packet coupled to a smooth continuum. United States. https://doi.org/10.1088/2040-8986/aa8a93
Dahlström, Jan Marcus, Pabst, Stefan, and Lindroth, Eva. Mon .
"Attosecond transient absorption of a bound wave packet coupled to a smooth continuum". United States. https://doi.org/10.1088/2040-8986/aa8a93. https://www.osti.gov/servlets/purl/1410602.
@article{osti_1410602,
title = {Attosecond transient absorption of a bound wave packet coupled to a smooth continuum},
author = {Dahlström, Jan Marcus and Pabst, Stefan and Lindroth, Eva},
abstractNote = {Here, we investigate the possibility of using transient absorption of a coherent bound electron wave packet in hydrogen as an attosecond pulse characterization technique. In a recent work, we have shown that photoionization of such a coherent bound electron wave packet opens up for pulse characterization with unprecedented temporal accuracy—independent of the atomic structure—with maximal photoemission at all kinetic energies given a wave packet with zero relative phase. Here, we perform numerical propagation of the time-dependent Schrödinger equation and analytical calculations based on perturbation theory to show that the energy-resolved maximal absorption of photons from the attosecond pulse does not uniquely occur at a zero relative phase of the initial wave packet. Instead, maximal absorption occurs at different relative wave packet phases, distributed as a non-monotonous function with a smooth $-\pi /2$ shift across the central photon energy (given a Fourier-limited Gaussian pulse). Similar results are also found in helium. Our finding is surprising, because it implies that the energy-resolved photoelectrons are not mapped one-to-one with the energy-resolved absorbed photons of the attosecond pulse.},
doi = {10.1088/2040-8986/aa8a93},
journal = {Journal of Optics},
number = 11,
volume = 19,
place = {United States},
year = {Mon Oct 16 00:00:00 EDT 2017},
month = {Mon Oct 16 00:00:00 EDT 2017}
}
Web of Science
Works referenced in this record:
Femtochemistry: Atomic-Scale Dynamics of the Chemical Bond †
journal, June 2000
- Zewail, Ahmed H.
- The Journal of Physical Chemistry A, Vol. 104, Issue 24
Attosecond physics
journal, February 2009
- Krausz, Ferenc; Ivanov, Misha
- Reviews of Modern Physics, Vol. 81, Issue 1
Real-time observation of valence electron motion
journal, August 2010
- Goulielmakis, Eleftherios; Loh, Zhi-Heng; Wirth, Adrian
- Nature, Vol. 466, Issue 7307
Synthesized Light Transients
journal, September 2011
- Wirth, A.; Hassan, M. T.; Grguras, I.
- Science, Vol. 334, Issue 6053
State-resolved attosecond reversible and irreversible dynamics in strong optical fields
journal, February 2017
- Sabbar, Mazyar; Timmers, Henry; Chen, Yi-Jen
- Nature Physics, Vol. 13, Issue 5
Time-resolved x-ray absorption spectroscopy with a water window high-harmonic source
journal, January 2017
- Pertot, Yoann; Schmidt, Cédric; Matthews, Mary
- Science, Vol. 355, Issue 6322
Attosecond Time-Resolved Autoionization of Argon
journal, October 2010
- Wang, He; Chini, Michael; Chen, Shouyuan
- Physical Review Letters, Vol. 105, Issue 14
Lorentz Meets Fano in Spectral Line Shapes: A Universal Phase and Its Laser Control
journal, May 2013
- Ott, C.; Kaldun, A.; Raith, P.
- Science, Vol. 340, Issue 6133
Reconstruction and control of a time-dependent two-electron wave packet
journal, December 2014
- Ott, Christian; Kaldun, Andreas; Argenti, Luca
- Nature, Vol. 516, Issue 7531
Attosecond counter-rotating-wave effect in xenon driven by strong fields
journal, May 2017
- Anand, M.; Pabst, Stefan; Kwon, Ojoon
- Physical Review A, Vol. 95, Issue 5
Probing ultrafast dynamics with attosecond transient absorption
journal, March 2015
- Beck, Annelise R.; Neumark, Daniel M.; Leone, Stephen R.
- Chemical Physics Letters, Vol. 624
Absorption and emission of single attosecond light pulses in an autoionizing gaseous medium dressed by a time-delayed control field
journal, January 2013
- Chu, Wei-Chun; Lin, C. D.
- Physical Review A, Vol. 87, Issue 1
Theory of attosecond transient-absorption spectroscopy of krypton for overlapping pump and probe pulses
journal, December 2012
- Pabst, Stefan; Sytcheva, Arina; Moulet, Antoine
- Physical Review A, Vol. 86, Issue 6
Infinite-range exterior complex scaling as a perfect absorber in time-dependent problems
journal, May 2010
- Scrinzi, Armin
- Physical Review A, Vol. 81, Issue 5
A Practical Guide to Splines.
journal, January 1980
- R., J.; de Boor, Carl
- Mathematics of Computation, Vol. 34, Issue 149
Diagrammatic approach to attosecond delays in photoionization
journal, December 2012
- Dahlström, J. M.; Carette, T.; Lindroth, E.
- Physical Review A, Vol. 86, Issue 6
The definition of molecular resonance curves by the method of exterior complex scaling
journal, April 1979
- Simon, Barry
- Physics Letters A, Vol. 71, Issue 2-3
Solving the time-dependent Schrödinger equation using complex-coordinate contours
journal, June 1991
- McCurdy, C. William; Stroud, Carrie K.; Wisinski, Matthew K.
- Physical Review A, Vol. 43, Issue 11
Modern Quantum Mechanics
journal, July 1986
- Sakurai, J. J.; Liboff, Richard L.
- American Journal of Physics, Vol. 54, Issue 7
Ionization delays in few-cycle-pulse multiphoton quantum-beat spectroscopy in helium
journal, February 2016
- Pazourek, Renate; Reduzzi, Maurizio; Carpeggiani, Paolo A.
- Physical Review A, Vol. 93, Issue 2
Observation of a Train of Attosecond Pulses from High Harmonic Generation
journal, June 2001
- Paul, P. M.
- Science, Vol. 292, Issue 5522
Study of attosecond delays using perturbation diagrams and exterior complex scaling
text, January 2014
- Dahlström, J. M.; Lindroth, E.
- arXiv
Works referencing / citing this record:
Pulse analysis by delayed absorption from a coherently excited atom
journal, January 2019
- Dahlström, Jan Marcus; Pabst, Stefan; Lindroth, Eva
- APL Photonics, Vol. 4, Issue 1
Emerging attosecond technologies
journal, October 2018
- Mauritsson, Johan; Vampa, Giulio; Vozzi, Caterina
- Journal of Optics, Vol. 20, Issue 11
Attosecond precision in delay measurements using transient absorption spectroscopy
journal, January 2019
- Hartmann, Maximilian; Stooß, Veit; Birk, Paul
- Optics Letters, Vol. 44, Issue 19
Pulse analysis by delayed absorption from a coherently excited atom
preprint, January 2018
- Dahlström, Jan Marcus; Pabst, Stefan; Lindroth, Eva
- arXiv