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Title: Single shot speckle and coherence analysis of the hard X-ray free electron laser LCLS

Abstract

The single shot based coherence properties of hard x-ray pulses from the Linac Coherent Light Source (LCLS) were measured by analyzing coherent diffraction patterns from nano-particles and gold nanopowder. The intensity histogram of the small angle x-ray scattering ring from nano-particles reveals the fully transversely coherent nature of the LCLS beam with a number of transverse mode $$\langle$$Ms$$\rangle$$ = 1.1. On the other hand, the speckle contrasts measured at a large wavevector yields information about the longitudinal coherence of the LCLS radiation after a silicon (111) monochromator. The quantitative agreement between our data and the simulation confirms a mean coherence time of 2.2 fs and a x-ray pulse duration of 29 fs. Lastly the observed reduction of the speckle contrast generated by x-rays with pulse duration longer than 30 fs indicates ultrafast dynamics taking place at an atomic length scale prior to the permanent sample damage.

Authors:
 [1];  [2];  [2];  [2];  [2];  [2];  [2];  [3];  [3];  [3];  [3];  [4];  [4];  [5];  [5];  [5];  [2];  [3]
+ Show Author Affiliations
  1. Korea Research Inst. of Standards and Science (KRISS), Daejeon (Korea); Deutsches Elektronen-Synchrotron (DESY), Hamburg (Germany). Hasylab; SLAC National Accelerator Lab., Menlo Park, CA (United States). Linac Coherent Light Source (LCLS)
  2. Deutsches Elektronen-Synchrotron (DESY), Hamburg (Germany). Hasylab
  3. SLAC National Accelerator Lab., Menlo Park, CA (United States). Linac Coherent Light Source (LCLS)
  4. Max Planck Inst. for Intelligent Systems, Stuttgart (Germany)
  5. Argonne National Lab. (ANL), Argonne, IL (United States). Materials Science Division
Publication Date:
Research Org.:
Argonne National Laboratory (ANL), Argonne, IL (United States); SLAC National Accelerator Laboratory (SLAC), Menlo Park, CA (United States)
Sponsoring Org.:
USDOE Office of Science (SC), Basic Energy Sciences (BES); Ministry of Science, ICT and Future Planning, Korea; German Research Foundation (DFG)
OSTI Identifier:
1396050
Grant/Contract Number:  
AC02-06CH11357
Resource Type:
Accepted Manuscript
Journal Name:
Optics Express
Additional Journal Information:
Journal Volume: 21; Journal Issue: 21; Journal ID: ISSN 1094-4087
Publisher:
Optical Society of America (OSA)
Country of Publication:
United States
Language:
English
Subject:
46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND TECHNOLOGY; Free-electron lasers; Spectroscopy; Speckle

Citation Formats

Lee, Sooheyong, Roseker, W., Gutt, C., Fischer, B., Conrad, H., Lehmkühler, F., Steinke, I., Zhu, D., Lemke, H., Cammarata, M., Fritz, D. M., Wochner, P., Castro-Colin, M., Hruszkewycz, S. O., Fuoss, P. H., Stephenson, G. B., Grübel, G., and Robert, A. Single shot speckle and coherence analysis of the hard X-ray free electron laser LCLS. United States: N. p., 2013. Web. doi:10.1364/OE.21.024647.
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Lee, Sooheyong, Roseker, W., Gutt, C., Fischer, B., Conrad, H., Lehmkühler, F., Steinke, I., Zhu, D., Lemke, H., Cammarata, M., Fritz, D. M., Wochner, P., Castro-Colin, M., Hruszkewycz, S. O., Fuoss, P. H., Stephenson, G. B., Grübel, G., & Robert, A. Single shot speckle and coherence analysis of the hard X-ray free electron laser LCLS. United States. https://doi.org/10.1364/OE.21.024647
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Lee, Sooheyong, Roseker, W., Gutt, C., Fischer, B., Conrad, H., Lehmkühler, F., Steinke, I., Zhu, D., Lemke, H., Cammarata, M., Fritz, D. M., Wochner, P., Castro-Colin, M., Hruszkewycz, S. O., Fuoss, P. H., Stephenson, G. B., Grübel, G., and Robert, A. Tue . "Single shot speckle and coherence analysis of the hard X-ray free electron laser LCLS". United States. https://doi.org/10.1364/OE.21.024647. https://www.osti.gov/servlets/purl/1396050.
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@article{osti_1396050,
title = {Single shot speckle and coherence analysis of the hard X-ray free electron laser LCLS},
author = {Lee, Sooheyong and Roseker, W. and Gutt, C. and Fischer, B. and Conrad, H. and Lehmkühler, F. and Steinke, I. and Zhu, D. and Lemke, H. and Cammarata, M. and Fritz, D. M. and Wochner, P. and Castro-Colin, M. and Hruszkewycz, S. O. and Fuoss, P. H. and Stephenson, G. B. and Grübel, G. and Robert, A.},
abstractNote = {The single shot based coherence properties of hard x-ray pulses from the Linac Coherent Light Source (LCLS) were measured by analyzing coherent diffraction patterns from nano-particles and gold nanopowder. The intensity histogram of the small angle x-ray scattering ring from nano-particles reveals the fully transversely coherent nature of the LCLS beam with a number of transverse mode $\langle$Ms$\rangle$ = 1.1. On the other hand, the speckle contrasts measured at a large wavevector yields information about the longitudinal coherence of the LCLS radiation after a silicon (111) monochromator. The quantitative agreement between our data and the simulation confirms a mean coherence time of 2.2 fs and a x-ray pulse duration of 29 fs. Lastly the observed reduction of the speckle contrast generated by x-rays with pulse duration longer than 30 fs indicates ultrafast dynamics taking place at an atomic length scale prior to the permanent sample damage.},
doi = {10.1364/OE.21.024647},
journal = {Optics Express},
number = 21,
volume = 21,
place = {United States},
year = {Tue Oct 08 00:00:00 EDT 2013},
month = {Tue Oct 08 00:00:00 EDT 2013}
}
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https://doi.org/10.1364/OE.21.024647
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    Works referencing / citing this record:

    Coherent X-rays reveal the influence of cage effects on ultrafast water dynamics
    journal, May 2018

    Diffraction based Hanbury Brown and Twiss interferometry at a hard x-ray free-electron laser
    journal, February 2018

    Coherence and pulse duration characterization of the PAL-XFEL in the hard X-ray regime
    journal, March 2019

    Double-pulse speckle contrast correlations with near Fourier transform limited free-electron laser light using hard X-ray split-and-delay
    journal, March 2020

    Single Shot Coherence Properties of the Free-Electron Laser SACLA in the Hard X-ray Regime
    journal, June 2014

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    • Scientific Reports, Vol. 4, Issue 1
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    Spatial and temporal pre-alignment of an X-ray split-and-delay unit by laser light interferometry
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    Characterizing the intrinsic properties of individual XFEL pulses via single-particle diffraction
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    Spatial and temporal pre-alignment of an X-ray split-and-delay unit by laser light interferometry
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    Coherent X-rays reveal the influence of cage effects on ultrafast water dynamics
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    Double-pulse speckle contrast correlations with near Fourier transform limited free-electron laser light using hard split-and-delay
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    • Roseker, Wojciech; Lee, Sooheyong; Walther, Michael
    • Deutsches Elektronen-Synchrotron, DESY, Hamburg
    • DOI: 10.3204/pubdb-2020-01030
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