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Title: Integrating solids and gases for attosecond pulse generation

Here, control of the field of few-cycle optical pulses has had an enormous impact on attosecond science. Subcycle pulses open the potential for non-adiabatic phase matching while concentrating the electric field so it can be used most efficiently. However, subcycle field transients have been difficult to generate. We exploit the perturbative response of a sub-100 µm thick monocrystalline quartz plate irradiated by an intense few-cycle 1.8 µm pulse, which creates a phase-controlled supercontinuum spectrum. Within the quartz, the pulse becomes space–time coupled as it generates a parallel second harmonic. Vacuum propagation naturally leads to a subcycle electric-field transient whose envelope is sculpted by the carrier envelope phase of the incident radiation. We show that a second medium (either gas or solid) can generate isolated attosecond pulses in the extreme ultraviolet region. With no optical elements between the components, the process is scalable to very high energy pulses and allows the use of diverse media.
Authors:
 [1] ;  [2] ;  [2] ;  [3] ;  [4] ;  [4] ; ORCiD logo [4] ;  [5]
  1. Univ. of Ottawa, Ottawa, ON (Canada); Univ. of Central Florida, Orlando, FL (United States)
  2. Univ. of Ottawa, Ottawa, ON (Canada)
  3. Univ. of Ottawa, Ottawa, ON (Canada); SLAC National Accelerator Lab., Menlo Park, CA (United States)
  4. National Research Council of Canada, Ottawa, ON (Canada)
  5. Univ. of Ottawa, Ottawa, ON (Canada); National Research Council of Canada, Ottawa, ON (Canada)
Publication Date:
Grant/Contract Number:
AC02-76SF00515
Type:
Accepted Manuscript
Journal Name:
Nature Photonics
Additional Journal Information:
Journal Volume: 11; Journal Issue: 9; Journal ID: ISSN 1749-4885
Publisher:
Nature Publishing Group
Research Org:
SLAC National Accelerator Lab., Menlo Park, CA (United States)
Sponsoring Org:
USDOE
Country of Publication:
United States
Language:
English
Subject:
71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSICS
OSTI Identifier:
1394082

Hammond, T. J., Monchoce, Sylvain, Zhang, Chunmei, Vampa, Giulio, Klug, Dennis, Naumov, A. Yu., Villeneuve, D. M., and Corkum, P. B.. Integrating solids and gases for attosecond pulse generation. United States: N. p., Web. doi:10.1038/nphoton.2017.141.
Hammond, T. J., Monchoce, Sylvain, Zhang, Chunmei, Vampa, Giulio, Klug, Dennis, Naumov, A. Yu., Villeneuve, D. M., & Corkum, P. B.. Integrating solids and gases for attosecond pulse generation. United States. doi:10.1038/nphoton.2017.141.
Hammond, T. J., Monchoce, Sylvain, Zhang, Chunmei, Vampa, Giulio, Klug, Dennis, Naumov, A. Yu., Villeneuve, D. M., and Corkum, P. B.. 2017. "Integrating solids and gases for attosecond pulse generation". United States. doi:10.1038/nphoton.2017.141. https://www.osti.gov/servlets/purl/1394082.
@article{osti_1394082,
title = {Integrating solids and gases for attosecond pulse generation},
author = {Hammond, T. J. and Monchoce, Sylvain and Zhang, Chunmei and Vampa, Giulio and Klug, Dennis and Naumov, A. Yu. and Villeneuve, D. M. and Corkum, P. B.},
abstractNote = {Here, control of the field of few-cycle optical pulses has had an enormous impact on attosecond science. Subcycle pulses open the potential for non-adiabatic phase matching while concentrating the electric field so it can be used most efficiently. However, subcycle field transients have been difficult to generate. We exploit the perturbative response of a sub-100 µm thick monocrystalline quartz plate irradiated by an intense few-cycle 1.8 µm pulse, which creates a phase-controlled supercontinuum spectrum. Within the quartz, the pulse becomes space–time coupled as it generates a parallel second harmonic. Vacuum propagation naturally leads to a subcycle electric-field transient whose envelope is sculpted by the carrier envelope phase of the incident radiation. We show that a second medium (either gas or solid) can generate isolated attosecond pulses in the extreme ultraviolet region. With no optical elements between the components, the process is scalable to very high energy pulses and allows the use of diverse media.},
doi = {10.1038/nphoton.2017.141},
journal = {Nature Photonics},
number = 9,
volume = 11,
place = {United States},
year = {2017},
month = {8}
}

Works referenced in this record:

Attosecond control of electronic processes by intense light fields
journal, February 2003
  • Baltuška, A.; Udem, Th.; Uiberacker, M.
  • Nature, Vol. 421, Issue 6923, p. 611-615
  • DOI: 10.1038/nature01414