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Title: Integrating solids and gases for attosecond pulse generation

Journal Article · · Nature Photonics
 [1];  [2];  [2];  [3];  [4];  [4]; ORCiD logo [4];  [5]
  1. Univ. of Ottawa, Ottawa, ON (Canada); Univ. of Central Florida, Orlando, FL (United States)
  2. Univ. of Ottawa, Ottawa, ON (Canada)
  3. Univ. of Ottawa, Ottawa, ON (Canada); SLAC National Accelerator Lab., Menlo Park, CA (United States)
  4. National Research Council of Canada, Ottawa, ON (Canada)
  5. Univ. of Ottawa, Ottawa, ON (Canada); National Research Council of Canada, Ottawa, ON (Canada)

Here, control of the field of few-cycle optical pulses has had an enormous impact on attosecond science. Subcycle pulses open the potential for non-adiabatic phase matching while concentrating the electric field so it can be used most efficiently. However, subcycle field transients have been difficult to generate. We exploit the perturbative response of a sub-100 µm thick monocrystalline quartz plate irradiated by an intense few-cycle 1.8 µm pulse, which creates a phase-controlled supercontinuum spectrum. Within the quartz, the pulse becomes space–time coupled as it generates a parallel second harmonic. Vacuum propagation naturally leads to a subcycle electric-field transient whose envelope is sculpted by the carrier envelope phase of the incident radiation. We show that a second medium (either gas or solid) can generate isolated attosecond pulses in the extreme ultraviolet region. With no optical elements between the components, the process is scalable to very high energy pulses and allows the use of diverse media.

Research Organization:
SLAC National Accelerator Laboratory (SLAC), Menlo Park, CA (United States)
Sponsoring Organization:
USDOE
Grant/Contract Number:
AC02-76SF00515
OSTI ID:
1394082
Journal Information:
Nature Photonics, Journal Name: Nature Photonics Journal Issue: 9 Vol. 11; ISSN 1749-4885
Publisher:
Nature Publishing GroupCopyright Statement
Country of Publication:
United States
Language:
English

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Cited By (12)

Symmetry of molecular Rydberg states revealed by XUV transient absorption spectroscopy journal November 2019
Measurement of the Berry curvature of solids using high-harmonic spectroscopy text January 2018
Measurement of the Berry curvature of solids using high-harmonic spectroscopy journal March 2018
Symmetry of molecular Rydberg states revealed by XUV transient absorption spectroscopy journal November 2019
Strain-controlled high harmonic generation with Dirac fermions in silicene journal January 2018
Strong-field nonlinear optical properties of monolayer black phosphorus journal January 2019
Near-field imaging for single-shot waveform measurements journal February 2018
Colloquium : Strong-field phenomena in periodic systems journal April 2018
Symmetry of Molecular Rydberg States Revealed by XUV Transient Absorption Spectroscopy conference January 2020
Measurement of the Berry curvature of solids using high-harmonic spectroscopy text January 2018
Strain-controlled high harmonic generation with Dirac fermions in silicene text January 2018
Strong-field nonlinear optical properties of monolayer black phosphorus text January 2019

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