Time resolved 3D momentum imaging of ultrafast dynamics by coherent VUV-XUV radiation
Abstract
Have we present a new experimental setup for measuring ultrafast nuclear and electron dynamics of molecules after photo-excitation and ionization. We combine a high flux femtosecond vacuum ultraviolet (VUV) and extreme ultraviolet (XUV) source with an internally cold molecular beam and a 3D momentum imaging particle spectrometer to measure electrons and ions in coincidence. We describe a variety of tools developed to perform pump-probe studies in the VUV-XUV spectrum and to modify and characterize the photon beam. First benchmark experiments are presented to demonstrate the capabilities of the system.
- Authors:
-
[2];
[2];
- Lawrence Berkeley National Lab. (LBNL), Berkeley, CA (United States). Ultrafast X-Ray Science Lab.; Univ. Frankfurt (Germany). Inst. fur Kernphysik
- Lawrence Berkeley National Lab. (LBNL), Berkeley, CA (United States). Ultrafast X-Ray Science Lab.
- Lawrence Berkeley National Lab. (LBNL), Berkeley, CA (United States). Ultrafast X-Ray Science Lab.; Extreme Light Infrastructure Attosecond Light Pulse Source (ELI-ALPS), Szeged (Hungary)
- Publication Date:
- Research Org.:
- Lawrence Berkeley National Laboratory (LBNL), Berkeley, CA (United States)
- Sponsoring Org.:
- USDOE Office of Science (SC), Basic Energy Sciences (BES)
- OSTI Identifier:
- 1379368
- Alternate Identifier(s):
- OSTI ID: 1257000
- Grant/Contract Number:
- AC02-05CH11231
- Resource Type:
- Accepted Manuscript
- Journal Name:
- Review of Scientific Instruments
- Additional Journal Information:
- Journal Volume: 87; Journal Issue: 6; Journal ID: ISSN 0034-6748
- Publisher:
- American Institute of Physics (AIP)
- Country of Publication:
- United States
- Language:
- English
- Subject:
- 46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND TECHNOLOGY; Photons; Mirrors; Ionization; Fluid jets; Laser beams
Citation Formats
Sturm, F. P., Wright, T. W., Ray, D., Zalyubovskaya, I., Shivaram, N., Slaughter, D. S., Ranitovic, P., Belkacem, A., and Weber, Th. Time resolved 3D momentum imaging of ultrafast dynamics by coherent VUV-XUV radiation. United States: N. p., 2016.
Web. doi:10.1063/1.4953441.
Sturm, F. P., Wright, T. W., Ray, D., Zalyubovskaya, I., Shivaram, N., Slaughter, D. S., Ranitovic, P., Belkacem, A., & Weber, Th. Time resolved 3D momentum imaging of ultrafast dynamics by coherent VUV-XUV radiation. United States. https://doi.org/10.1063/1.4953441
Sturm, F. P., Wright, T. W., Ray, D., Zalyubovskaya, I., Shivaram, N., Slaughter, D. S., Ranitovic, P., Belkacem, A., and Weber, Th. Tue .
"Time resolved 3D momentum imaging of ultrafast dynamics by coherent VUV-XUV radiation". United States. https://doi.org/10.1063/1.4953441. https://www.osti.gov/servlets/purl/1379368.
@article{osti_1379368,
title = {Time resolved 3D momentum imaging of ultrafast dynamics by coherent VUV-XUV radiation},
author = {Sturm, F. P. and Wright, T. W. and Ray, D. and Zalyubovskaya, I. and Shivaram, N. and Slaughter, D. S. and Ranitovic, P. and Belkacem, A. and Weber, Th.},
abstractNote = {Have we present a new experimental setup for measuring ultrafast nuclear and electron dynamics of molecules after photo-excitation and ionization. We combine a high flux femtosecond vacuum ultraviolet (VUV) and extreme ultraviolet (XUV) source with an internally cold molecular beam and a 3D momentum imaging particle spectrometer to measure electrons and ions in coincidence. We describe a variety of tools developed to perform pump-probe studies in the VUV-XUV spectrum and to modify and characterize the photon beam. First benchmark experiments are presented to demonstrate the capabilities of the system.},
doi = {10.1063/1.4953441},
journal = {Review of Scientific Instruments},
number = 6,
volume = 87,
place = {United States},
year = {Tue Jun 14 00:00:00 EDT 2016},
month = {Tue Jun 14 00:00:00 EDT 2016}
}
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Works referencing / citing this record:
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