Van der Waals engineering of ferromagnetic semiconductor heterostructures for spin and valleytronics

Zhong, Ding; Seyler, Kyle L.; Linpeng, Xiayu; Cheng, Ran; Sivadas, Nikhil; Huang, Bevin; Schmidgall, Emma; Taniguchi, Takashi; Wantanabe, Kenji; McGuire, Michael A.; Yao, Wang; Xiao, Di; Fu, Kai-Mei C.; Xu, Xiaodong

doi:10.1126/sciadv.1603113

Title: Van der Waals engineering of ferromagnetic semiconductor heterostructures for spin and valleytronics

Journal Article · Wed May 31 00:00:00 EDT 2017 · Science Advances

DOI: https://doi.org/10.1126/sciadv.1603113 · OSTI ID:1376521

Zhong, Ding ^[1]; Seyler, Kyle L. ^[1]; Linpeng, Xiayu ^[1]; Cheng, Ran ^[2]; Sivadas, Nikhil ^[2]; Huang, Bevin ^[1]; Schmidgall, Emma ^[1]; Taniguchi, Takashi ^[3]; Wantanabe, Kenji ^[3]; McGuire, Michael A. ^[4]; Yao, Wang ^[5]; Xiao, Di ^[5]; Fu, Kai-Mei C. ^[1]; Xu, Xiaodong ^[1]

Univ. of Washington, Seattle, WA (United States)
Carnegie Mellon Univ., Pittsburgh, PA (United States)
National Inst. for Materials Science (NIMS), Tsukuba (Japan)
Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States)
Univ. of Hong Kong (China)

The integration of magnetic material with semiconductors has been fertile ground for fundamental science as well as of great practical interest toward the seamless integration of information processing and storage. We create van der Waals heterostructures formed by an ultrathin ferromagnetic semiconductor CrI₃ and a monolayer of WSe₂. We observe unprecedented control of the spin and valley pseudospin in WSe₂, where we detect a large magnetic exchange field of nearly 13 T and rapid switching of the WSe₂ valley splitting and polarization via flipping of the CrI₃ magnetization. The WSe2 photoluminescence intensity strongly depends on the relative alignment between photoexcited spins in WSe₂ and the CrI₃ magnetization, because of ultrafast spin-dependent charge hopping across the heterostructure interface. The photoluminescence detection of valley pseudospin provides a simple and sensitive method to probe the intriguing domain dynamics in the ultrathin magnet, as well as the rich spin interactions within the heterostructure.

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Research Organization:: Oak Ridge National Laboratory (ORNL), Oak Ridge, TN (United States)

Sponsoring Organization:: USDOE Office of Science (SC), Basic Energy Sciences (BES) (SC-22)

Grant/Contract Number:: AC05-00OR22725

OSTI ID:: 1376521

Journal Information:: Science Advances, Journal Name: Science Advances Journal Issue: 5 Vol. 3; ISSN 2375-2548

Publisher:: AAASCopyright Statement

Country of Publication:: United States

Language:: English

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Physical origin of giant excitonic and magneto-optical responses in two-dimensional ferromagnetic insulators Wu, Meng; Li, Zhenglu; Cao, Ting arXiv https://doi.org/10.48550/arxiv.1903.07787	text	January 2019
Magneto-optical Kerr effect in spin split two-dimensional massive Dirac materials Catarina, G.; Peres, N. M. R.; Fernández-Rossier, J. arXiv https://doi.org/10.48550/arxiv.1910.13371	text	January 2019
Marrying Excitons and Plasmons in Monolayer Transition-Metal Dichalcogenides Van Tuan, Dinh; Scharf, Benedikt; Žutić, Igor Universität Regensburg https://doi.org/10.5283/epub.39560	text	January 2017
Strain-tunable orbital, spin-orbit, and optical properties of monolayer transition-metal dichalcogenides Zollner, Klaus; Faria Junior, Paulo E.; Fabian, Jaroslav Universität Regensburg https://doi.org/10.5283/epub.41297	text	January 2019
Magnetic proximity in a van der Waals heterostructure of magnetic insulator and graphene Karpiak, Bogdan; Cummings, Aron W.; Zollner, Klaus Universität Regensburg https://doi.org/10.5283/epub.41300	text	January 2019

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