Structural phase transitions in SrTiO3 nanoparticles

Zhang, Han; Liu, Sizhan; Scofield, Megan E.; Wong, Stanislaus S.; Hong, Xinguo; Prakapenka, Vitali B.; Greenberg, Eran; Tyson, Trevor A.

doi:10.1063/1.4997332

Title: Structural phase transitions in SrTiO₃ nanoparticles

Abstract

We present that pressure dependent structural measurements on monodispersed nanoscale SrTiO₃ samples with average diameters of 10 to ~80 nm were conducted to enhance the understanding of the structural phase diagram of nanoscale SrTiO₃. A robust pressure independent polar structure was found in the 10 nm sample for pressures up to 13 GPa, while a size dependent cubic to tetragonal transition occurs (at P = P_c) for larger particle sizes. In conclusion, the results suggest that the growth of ~10 nm STO particles on substrates with significant lattice mismatch may maintain a polar state for a large range of strain values, possibly enabling device use.

Authors:

Zhang, Han ^[1]; Liu, Sizhan ^[1]; Scofield, Megan E. ^[2]; Wong, Stanislaus S. ^[3]; Hong, Xinguo ^[4]; Prakapenka, Vitali B. ^[5];

^[5]; Tyson, Trevor A. ^[1]

New Jersey Inst. of Technology, Newark, NJ (United States). Department of Physics
State University of New York at Stony Brook, Stony Brook, NY (United States). Department of Chemistry
State University of New York at Stony Brook, Stony Brook, NY (United States). Department of Chemistry ; Brookhaven National Lab. (BNL), Upton, NY (United States). Condensed Matter Physics and Materials Science Division
Stony Brook Univ., NY (United States). Mineral Physics Institute; Center for High Pressure Science and Technology Advanced Research, Beijing (China)
Univ. of Chicago, IL (United States). Center for Advanced Radiation Sources

Publication Date:: Fri Aug 04 00:00:00 EDT 2017

Research Org.:: Brookhaven National Laboratory (BNL), Upton, NY (United States)

Sponsoring Org.:: USDOE Office of Science (SC), Basic Energy Sciences (BES)

OSTI Identifier:: 1376161

Report Number(s):: BNL-114120-2017-JA
Journal ID: ISSN 0003-6951; R&D Project: PM037; KC0201030

Grant/Contract Number:: SC0012704; FG02-07ER46402; AC02-98CH10886; FG02-94ER14466

Resource Type:: Accepted Manuscript

Journal Name:: Applied Physics Letters

Additional Journal Information:: Journal Volume: 111; Journal Issue: 5; Journal ID: ISSN 0003-6951

Publisher:: American Institute of Physics (AIP)

Country of Publication:: United States

Language:: English

Subject:: 75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND SUPERFLUIDITY

Citation Formats


                    Zhang, Han, Liu, Sizhan, Scofield, Megan E., Wong, Stanislaus S., Hong, Xinguo, Prakapenka, Vitali B., Greenberg, Eran, and Tyson, Trevor A. Structural phase transitions in SrTiO3 nanoparticles.  United States: N. p., 2017. 
Web.  doi:10.1063/1.4997332.

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                    Zhang, Han, Liu, Sizhan, Scofield, Megan E., Wong, Stanislaus S., Hong, Xinguo, Prakapenka, Vitali B., Greenberg, Eran, & Tyson, Trevor A. Structural phase transitions in SrTiO3 nanoparticles.  United States.  https://doi.org/10.1063/1.4997332

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                    Zhang, Han, Liu, Sizhan, Scofield, Megan E., Wong, Stanislaus S., Hong, Xinguo, Prakapenka, Vitali B., Greenberg, Eran, and Tyson, Trevor A. Fri .  
"Structural phase transitions in SrTiO3 nanoparticles".  United States.  https://doi.org/10.1063/1.4997332.  https://www.osti.gov/servlets/purl/1376161.

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@article{osti_1376161,

  title        = {Structural phase transitions in SrTiO3 nanoparticles},

  author       = {Zhang, Han and Liu, Sizhan and Scofield, Megan E. and Wong, Stanislaus S. and Hong, Xinguo and Prakapenka, Vitali B. and Greenberg, Eran and Tyson, Trevor A.},

  abstractNote = {We present that pressure dependent structural measurements on monodispersed nanoscale SrTiO3 samples with average diameters of 10 to ~80 nm were conducted to enhance the understanding of the structural phase diagram of nanoscale SrTiO3. A robust pressure independent polar structure was found in the 10 nm sample for pressures up to 13 GPa, while a size dependent cubic to tetragonal transition occurs (at P = Pc) for larger particle sizes. In conclusion, the results suggest that the growth of ~10 nm STO particles on substrates with significant lattice mismatch may maintain a polar state for a large range of strain values, possibly enabling device use.},

  doi          = {10.1063/1.4997332},

  journal      = {Applied Physics Letters},

  number       = 5,

  volume       = 111,

  place        = {United States},

  year         = {Fri Aug 04 00:00:00 EDT 2017},

  month        = {Fri Aug 04 00:00:00 EDT 2017}

}

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Polarization rotation transitions in anisotropically strained SrTiO3 thin films
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Works referencing / citing this record:

Size, shape, and orientation dependence of the field-induced behavior in ferroelectric nanoparticles
journal, April 2019

Zhu, Daopei; Mangeri, John; Wang, Ruolin
Journal of Applied Physics, Vol. 125, Issue 13
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Metastable vortex-like polarization textures in ferroelectric nanoparticles of different shapes and sizes
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Mangeri, John; Alpay, S. Pamir; Nakhmanson, Serge
Applied Physics Letters, Vol. 113, Issue 9
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Structural phase transitions in SrTiO ₃ nanoparticles

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Pressure dependent structural measurements on monodispersed nanoscale SrTiO3 samples with average diameters of 10 to ~80 nm were conducted to enhance the understanding of the structural phase diagram of nanoscale SrTiO3. A robust pressure independent polar structure was found in the 10 nm sample for pressures up to 13 GPa, while a size dependent cubic to tetragonal transition occurs (at P = Pc) for larger particle sizes. The results suggest that the growth of ~10 nm STO particles on substrates with significant lattice mismatch may maintain a polar state for a large range of strain values, possibly enabling device use.
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Similar Records

Title: Structural phase transitions in SrTiO3 nanoparticles

Abstract

Citation Formats

Room-temperature ferroelectricity in strained SrTiO3 journal, August 2004

Origin of Anomalous Lattice Expansion in Oxide Nanoparticles journal, October 2000

Pressure-temperature phase diagram of multiferroic EuTiO 3 journal, August 2015

Ferroelectricity Induced by Oxygen Isotope Exchange in Strontium Titanate Perovskite journal, April 1999

Dielectric and X-Ray Studies of Ca x Ba 1 − x Ti O 3 and Ca x Sr 1 − x Ti O 3 journal, December 1961

Theory of ferroelectrics journal, April 1954

Theoretical Study of Antiferrodistortive Phase Transition in Strontium Titanate journal, April 2010

The critical dynamics of SrTiO 3 : a study of neutron- and Raman-determined soft-mode lineshapes journal, February 1983

Electric-Field-Induced Raman Scattering in SrTi O 3 and KTa O 3 journal, October 1968

Emergence of room-temperature ferroelectricity at reduced dimensions journal, September 2015

Polarization rotation transitions in anisotropically strained SrTiO3 thin films journal, May 2008

Pressure-Induced Quenching of the Jahn-Teller Distortion and Insulator-to-Metal Transition in LaMnO 3 journal, August 2001

Grain Size Effect on Dielectric and Piezoelectric Properties of Alkoxy-Derived BaTiO 3 -Based Thin Films journal, September 2004

R factors in Rietveld analysis: How good is good enough? journal, March 2006

Size Dependence of the Pressure-Induced Phase Transition in Nanocrystals journal, February 2008

Ferroelectricity in Strain-Free SrTiO 3 Thin Films journal, May 2010

Pressure-induced disappearance of the local rhombohedral distortion in BaTiO 3 journal, May 2006

EosFit7-GUI : a new graphical user interface for equation of state calculations, analyses and teaching journal, June 2016

Polar state in freestanding strontium titanate nanoparticles journal, September 2014

Murnaghan’s equation of state for the electronic ground state energy journal, December 2006

Structural phase transition of ternary dielectric SmGdO 3 : Evidence from angle dispersive x-ray diffraction and Raman spectroscopic studies journal, March 2015

Prediction of a low-temperature ferroelectric instability in antiphase domain boundaries of strontium titanate journal, November 2001

Temperature Dependence of a Transverse Optic Mode in Strontium Titanate journal, August 1962

E.s.d.'s and estimated probable error obtained in Rietveld refinements with local correlations journal, February 1991

Nanomaterials under high-pressure journal, January 2006

Tetragonal SrTiO3 revisited: The effect of impurities on the Raman spectrum journal, September 1979

Characteristics of Barium Titanate Nanocube Ordered Assembly Thin Films Fabricated by Dip-Coating Method journal, September 2013

Size, shape, and orientation dependence of the field-induced behavior in ferroelectric nanoparticles journal, April 2019

Metastable vortex-like polarization textures in ferroelectric nanoparticles of different shapes and sizes journal, August 2018

Electromechanical control of polarization vortex ordering in an interacting ferroelectric-dielectric composite dimer text, January 2019

Electromechanical control of polarization vortex ordering in an interacting ferroelectric-dielectric composite dimer journal, August 2018

Title: Structural phase transitions in SrTiO₃ nanoparticles

Room-temperature ferroelectricity in strained SrTiO₃
journal, August 2004

Origin of Anomalous Lattice Expansion in Oxide Nanoparticles
journal, October 2000

Pressure-temperature phase diagram of multiferroic ${EuTiO}_{3}$
journal, August 2015

Ferroelectricity Induced by Oxygen Isotope Exchange in Strontium Titanate Perovskite
journal, April 1999

Dielectric and X-Ray Studies of ${Ca}_{x} {Ba}_{1 - x} Ti O_{3}$ and ${Ca}_{x} {Sr}_{1 - x} Ti O_{3}$
journal, December 1961

Theory of ferroelectrics
journal, April 1954

Theoretical Study of Antiferrodistortive Phase Transition in Strontium Titanate
journal, April 2010

The critical dynamics of SrTiO ₃ : a study of neutron- and Raman-determined soft-mode lineshapes
journal, February 1983

Electric-Field-Induced Raman Scattering in SrTi $O_{3}$ and KTa $O_{3}$
journal, October 1968

Emergence of room-temperature ferroelectricity at reduced dimensions
journal, September 2015

Polarization rotation transitions in anisotropically strained SrTiO3 thin films
journal, May 2008

Pressure-Induced Quenching of the Jahn-Teller Distortion and Insulator-to-Metal Transition in ${LaMnO}_{3}$
journal, August 2001

Grain Size Effect on Dielectric and Piezoelectric Properties of Alkoxy-Derived BaTiO ₃ -Based Thin Films
journal, September 2004

R factors in Rietveld analysis: How good is good enough?
journal, March 2006

Size Dependence of the Pressure-Induced Phase Transition in Nanocrystals
journal, February 2008

Ferroelectricity in Strain-Free ${SrTiO}_{3}$ Thin Films
journal, May 2010

Pressure-induced disappearance of the local rhombohedral distortion in BaTiO ₃
journal, May 2006

EosFit7-GUI : a new graphical user interface for equation of state calculations, analyses and teaching
journal, June 2016

Polar state in freestanding strontium titanate nanoparticles
journal, September 2014

Murnaghan’s equation of state for the electronic ground state energy
journal, December 2006

Structural phase transition of ternary dielectric SmGdO ₃ : Evidence from angle dispersive x-ray diffraction and Raman spectroscopic studies
journal, March 2015

Prediction of a low-temperature ferroelectric instability in antiphase domain boundaries of strontium titanate
journal, November 2001

Temperature Dependence of a Transverse Optic Mode in Strontium Titanate
journal, August 1962

E.s.d.'s and estimated probable error obtained in Rietveld refinements with local correlations
journal, February 1991

Nanomaterials under high-pressure
journal, January 2006

Tetragonal SrTiO3 revisited: The effect of impurities on the Raman spectrum
journal, September 1979

Characteristics of Barium Titanate Nanocube Ordered Assembly Thin Films Fabricated by Dip-Coating Method
journal, September 2013

Size, shape, and orientation dependence of the field-induced behavior in ferroelectric nanoparticles
journal, April 2019

Metastable vortex-like polarization textures in ferroelectric nanoparticles of different shapes and sizes
journal, August 2018

Electromechanical control of polarization vortex ordering in an interacting ferroelectric-dielectric composite dimer
text, January 2019

Electromechanical control of polarization vortex ordering in an interacting ferroelectric-dielectric composite dimer
journal, August 2018