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Title: NMR studies of the incommensurate helical antiferromagnet EuCo 2 P 2 : Determination of antiferromagnetic propagation vector

Journal Article · · Physical Review B
 [1];  [2];  [3];  [2];  [3];  [3];  [3];  [2];  [2]
  1. Ames Lab. and Iowa State Univ., Ames, IA (United States); Univ. of the Ryukyus, Okinawa (Japan)
  2. Ames Lab. and Iowa State Univ., Ames, IA (United States)
  3. Univ. of the Ryukyus, Okinawa (Japan)

Recently, Q.-P. Ding et al. reported that their nuclear magnetic resonance (NMR) study on EuCo2As2 successfully characterized the antiferromagnetic (AFM) propagation vector of the incommensurate helix AFM state, showing that NMR is a unique tool for determination of the spin structures in incommensurate helical AFMs. Motivated by this work, we have carried out 153Eu, 31P, and 59Co NMR measurements on the helical antiferromagnet EuCo2P2 with an AFM ordering temperature TN = 66.5 K. An incommensurate helical AFM structure was clearly confirmed by 153Eu and 31P NMR spectra on single-crystalline EuCo2P2 in zero magnetic field at 1.6 K and its external magnetic field dependence. Furthermore, based on 59Co NMR data in both the paramagnetic and incommensurate AFM states, we have determined the model-independent value of the AFM propagation vector k = (0,0,0.73±0.09)2π/c, where c is the c-axis lattice parameter. As a result, the temperature dependence of k is also discussed.

Research Organization:
Ames Lab. (AMES), Ames, IA (United States)
Sponsoring Organization:
USDOE
Grant/Contract Number:
AC02-07CH11358
OSTI ID:
1374738
Report Number(s):
IS-J--9413
Journal Information:
Physical Review B, Journal Name: Physical Review B Journal Issue: 2 Vol. 96; ISSN 2469-9950; ISSN PRBMDO
Publisher:
American Physical Society (APS)Copyright Statement
Country of Publication:
United States
Language:
English

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Ternary lanthanoid-transition metal pnictides with ThCr2Si2-type structure journal April 1978
A Transition from Localized to Strongly Correlated Electron Behavior and Mixed Valence Driven by Physical or Chemical Pressure in ACo 2 As 2 (A = Eu and Ca) journal February 2016
Effect of pressure on thermopower and resistivity of EuCo 2 P 2 journal January 2010
Electrical resistivity and specific heat of single-crystalline EuFe 2 As 2 : A magnetic homologue of SrFe 2 As 2 journal August 2008
Helical antiferromagnetic ordering in Lu 1 − x Sc x MnSi journal August 2014
Unified molecular field theory for collinear and noncollinear Heisenberg antiferromagnets journal February 2015
Antiferromagnetism in EuCu 2 As 2 and EuCu 1.82 Sb 2 single crystals journal May 2015
Magnetic dipole interactions in crystals journal January 2016
EuCo 2 P 2 : A model molecular-field helical Heisenberg antiferromagnet journal July 2016
Phase diagram of Eu magnetic ordering in Sn-flux-grown Eu ( Fe 1 − x Co x ) 2 As 2 single crystals journal November 2016
NMR determination of an incommensurate helical antiferromagnetic structure in EuCo 2 As 2 journal May 2017
Magnetic Susceptibility of Collinear and Noncollinear Heisenberg Antiferromagnets journal August 2012
Pressure-induced Transition of the Sublattice Magnetization in EuCo 2 P 2 : Change from Local Moment Eu ( 4 f ) to Itinerant Co ( 3 d ) Magnetism journal January 1998
153 Eu and 69,71 Ga Zero-Field NMR Study of Antiferromagnetic State in EuGa 4 journal October 2013

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