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Title: Controlling the Topological Sector of Magnetic Solitons in Exfoliated Cr 1 / 3 NbS 2 Crystals

Journal Article · · Physical Review Letters
 [1];  [2];  [3];  [4]; ORCiD logo [5]; ORCiD logo [5];  [6];  [7];  [2];  [8];  [9];  [3]
  1. Univ. of Geneva (Switzerland). Dept. of Quantum Matter Physics and Group of Applied Physics; Nanjing Tech Univ. (China). Key Lab. of Flexible Electronics (KLOFE) and Inst. of Advanced Materials (IAM)
  2. Ecole Polytechnique Federale Lausanne (Switzlerland). Inst. of Physics
  3. Univ. of Geneva (Switzerland). Dept. of Quantum Matter Physics and Group of Applied Physics
  4. Univ. of Tennessee, Knoxville, TN (United States). Dept. of Materials Science and Engineering
  5. Los Alamos National Lab. (LANL), Los Alamos, NM (United States). Theoretical Division T-4 and CNLS
  6. Univ. of Tokyo (Japan). Dept. of Applied Physics
  7. Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States). Center for Nanophase Materials Science
  8. Argonne National Lab. (ANL), Argonne, IL (United States). Materials Science Division
  9. Univ. of Tennessee, Knoxville, TN (United States). Dept. of Materials Science and Engineering and Dept. of Physics and Astronomy; Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States). Materials Science and Technology Division

Here, we investigate manifestations of topological order in monoaxial helimagnet Cr1/3NbS2 by performing transport measurements on ultrathin crystals. Upon sweeping the magnetic field perpendicularly to the helical axis, crystals thicker than one helix pitch (48 nm) but much thinner than the magnetic domain size (similar to 1 mu m) are found to exhibit sharp and hysteretic resistance jumps. We also show that these phenomena originate from transitions between topological sectors with a different number of magnetic solitons. This is confirmed by measurements on crystals thinner than 48 nm-in which the topological sector cannot change-that do not exhibit any jump or hysteresis. These results show the ability to deterministically control the topological sector of finite-size Cr1/3NbS2 and to detect intersector transitions by transport measurements.

Research Organization:
Argonne National Lab. (ANL), Argonne, IL (United States)
Sponsoring Organization:
USDOE Office of Science (SC), Basic Energy Sciences (BES); Swiss National Science Foundation (SNSF); National Science Foundation (NSF)
Grant/Contract Number:
AC02-06CH11357; AC05-00OR22725
OSTI ID:
1374539
Journal Information:
Physical Review Letters, Journal Name: Physical Review Letters Journal Issue: 25 Vol. 118; ISSN 0031-9007; ISSN PRLTAO
Publisher:
American Physical Society (APS)Copyright Statement
Country of Publication:
United States
Language:
English

References (28)

A thermodynamic theory of “weak” ferromagnetism of antiferromagnetics journal January 1958
Evidence for the helical spin structure due to antisymmetric exchange interaction in Cr13NbS2 journal April 1982
Magnetic and transport properties of 3d transition metal intercalates of some group Va transition metal dichalcogenides journal January 1980
Chiral helimagnetism in T1/3NbS2 (T=Cr and Mn)
  • Kousaka, Y.; Nakao, Y.; Kishine, J.
  • Nuclear Instruments and Methods in Physics Research Section A: Accelerators, Spectrometers, Detectors and Associated Equipment, Vol. 600, Issue 1 https://doi.org/10.1016/j.nima.2008.11.040
journal February 2009
Condensed Matter Field Theory book August 2010
Field Theories of Condensed Matter Physics book January 2013
Condensed Matter Field Theory book January 2006
Spin structure of the anisotropic helimagnet Cr 1∕3 NbS 2 in a magnetic field journal August 2014
Size dependence of discrete change in magnetization in single crystal of chiral magnet Cr 1/3 NbS 2 journal October 2016
Modulated, or long-periodic, magnetic structures of crystals journal November 1984
3 d transition-metal intercalates of the niobium and tantalum dichalcogenides. I. Magnetic properties journal January 1980
Theory of helical magnetic structures and phase transitions in MnSi and FeGe journal November 1980
Anisotropic Superexchange Interaction and Weak Ferromagnetism journal October 1960
Magnetic soliton transport over topological spin texture in chiral helimagnet with strong easy-plane anisotropy journal April 2009
Chiral modulations and reorientation effects in MnSi thin films journal March 2012
Magnetic phase transition in single crystals of the chiral helimagnet Cr 1 / 3 NbS 2 journal March 2013
Discrete helicoidal states in chiral magnetic thin films journal December 2013
Topological magnetization jumps in a confined chiral soliton lattice journal January 2014
Out-of-plane spin-orientation dependent magnetotransport properties in the anisotropic helimagnet Cr 1 / 3 NbS 2 journal May 2015
Magnetic soliton confinement and discretization effects arising from macroscopic coherence in a chiral spin soliton lattice journal December 2015
Phase diagram of the chiral magnet Cr 1 / 3 NbS 2 in a magnetic field journal March 2016
Tuning Magnetotransport through a Magnetic Kink Crystal in a Chiral Helimagnet journal July 2011
Chiral Magnetic Soliton Lattice on a Chiral Helimagnet journal March 2012
Interlayer Magnetoresistance due to Chiral Soliton Lattice Formation in Hexagonal Chiral Magnet CrNb 3 S 6 journal November 2013
Topological insulators and superconductors journal October 2011
Magnetic Properties of Cr 1/3 NbS 2 journal April 1983
Modulated, or long-periodic, magnetic structures of crystals [Modulirovannye, ili dlinnoperiodicheskie, magnitnye struktury kristallov] journal January 1984
Discrete Change in Magnetization by Chiral Soliton Lattice Formation in the Chiral Magnet Cr 1/3 NbS 2 journal January 2016

Cited By (9)

Surface-size and shape dependencies of change in chiral soliton number in submillimeter-scale crystals of chiral magnet CrNb 3 S 6 journal July 2019
Spin-current diode with a monoaxial chiral magnet journal July 2019
Theory of standing spin waves in a finite-size chiral spin soliton lattice journal July 2019
Magnetic solitons and magnetic phase diagram of the hexagonal chiral crystal CrNb 3 S 6 in oblique magnetic fields journal November 2017
Geometrical protection of topological magnetic solitons in microprocessed chiral magnets journal January 2018
Intrinsic hysteresis due to the surface barrier for chiral solitons in monoaxial chiral helimagnets journal June 2018
Magnetic field dependence of nonlinear magnetic response and tricritical point in the monoaxial chiral helimagnet Cr 1 / 3 Nb S 2 journal June 2018
Anomalous Temperature Behavior of the Chiral Spin Helix in CrNb 3 S 6 Thin Lamellae journal January 2019
Spin-current diode with a monoaxial chiral magnet text January 2019