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Title: Correlated Perovskites as a New Platform for Super-Broadband-Tunable Photonics

The electron-doping-induced phase transition of a prototypical perovskite SmNiO 3 induces a large and non-volatile optical refractive-index change and has great potential for active-photonic-device applications. Strong optical modulation from the visible to the mid-infrared is demonstrated using thin-film SmNiO 3. Finally, modulation of a narrow band of light is demonstrated in this paper using plasmonic metasurfaces integrated with SmNiO 3.
Authors:
 [1] ;  [2] ;  [3] ;  [3] ;  [4] ;  [1] ;  [5] ;  [5] ;  [3] ;  [4] ;  [1]
  1. Columbia Univ., New York, NY (United States). Dept. of Applied Physics and Applied Mathematics
  2. Harvard Univ., Cambridge, MA (United States). Dept. of Chemistry and Chemical Biology
  3. Drexel Univ., Philadelphia, PA (United States). Dept. of Materials Science and Engineering
  4. Purdue Univ., West Lafayette, IN (United States). School of Materials Engineering
  5. Brookhaven National Lab. (BNL), Upton, NY (United States). Center for Functional Nanomaterials
Publication Date:
Report Number(s):
BNL-113987-2017-JA
Journal ID: ISSN 0935-9648; KC0403020
Grant/Contract Number:
SC0012704; D15AP00111; N00014-16-1-2442; FA9550-14-1-0389; FA9550-12-1-0189; ECCS-1307948; W911NF-16-1-0042; W911NF-14-1-0669
Type:
Accepted Manuscript
Journal Name:
Advanced Materials
Additional Journal Information:
Journal Volume: 28; Journal Issue: 41; Journal ID: ISSN 0935-9648
Publisher:
Wiley
Research Org:
Brookhaven National Lab. (BNL), Upton, NY (United States); Purdue Univ., West Lafayette, IN (United States); Columbia Univ., New York, NY (United States)
Sponsoring Org:
USDOE Office of Science (SC), Basic Energy Sciences (BES) (SC-22); Defense Advanced Research Projects Agency (DARPA) (United States); Office of Naval Research (ONR) (United States); US Air Force Office of Scientific Research (AFOSR); National Science Foundation (NSF); US Army Research Office (ARO)
Contributing Orgs:
Harvard Univ., Cambridge, MA (United States); Drexel Univ., Philadelphia, PA (United States)
Country of Publication:
United States
Language:
English
Subject:
77 NANOSCIENCE AND NANOTECHNOLOGY; correlated oxides; metamaterials; optical modulation; perovskites; phase-transition materials
OSTI Identifier:
1368665