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Title: A water-based fast integrated mobility spectrometer (WFIMS) with enhanced dynamic size range

We developed a water-based fast integrated mobility spectrometer (WFIMS) with enhanced dynamic size range. The WFIMS builds on two established technologies: the fast integrated mobility spectrometer and laminar flow water-based condensation methodology. Inside WFIMS, particles of differing electrical mobility are separated in a drift tube and subsequently enlarged through water condensation. Particle size and concentration are measured via digital imaging at a frame rate of 10 Hz. When we measure particles of different mobilities simultaneously, the WFIMS resolves particle diameters ranging from 8 to 580 nm within 1 s or less. The performance of WFIMS was characterized with differential mobility analyzer (DMA) classified (NH 4) 2SO 2 particles with diameters ranging from 8 to 265 nm. The mean particle diameters measured by WFIMS were found to be in excellent agreement with DMA centroid diameters. Furthermore, detection efficiency of WFIMS was characterized using a condensation particle counter as a reference and is nearly 100% for particles with diameter greater than 8 nm. In general, measured and simulated WFIMS mobility resolutions are in good agreement. But, some deviations are observed at low particle mobilities, likely due to the non-idealities of the WFIMS electric field.
Authors:
 [1] ;  [2] ;  [2] ;  [1]
  1. Brookhaven National Lab. (BNL), Upton, NY (United States). Environmental and Climate Sciences Dept.
  2. Aerosol Dynamics Inc., Berkeley, CA (United States)
Publication Date:
Report Number(s):
BNL-113991-2017-JA
Journal ID: ISSN 0278-6826; R&D Project: 2016-BNL-EE630EECA-Budg; 87158; KP1701000
Grant/Contract Number:
SC00112704; SC0006312; AC02-98CH10886
Type:
Accepted Manuscript
Journal Name:
Aerosol Science and Technology
Additional Journal Information:
Journal Volume: 51; Journal Issue: 10; Journal ID: ISSN 0278-6826
Publisher:
American Association for Aerosol Research
Research Org:
Brookhaven National Laboratory (BNL), Upton, NY (United States)
Sponsoring Org:
USDOE Office of Science (SC), Biological and Environmental Research (BER) (SC-23)
Country of Publication:
United States
Language:
English
Subject:
54 ENVIRONMENTAL SCIENCES
OSTI Identifier:
1366353