Composition-matched molecular “solders” for semiconductors

Dolzhnikov, Dmitriy S.; Zhang, Hao; Jang, Jaeyoung; Son, Jae Sung; Panthani, Matthew G.; Shibata, Tomohiro; Chattopadhyay, Soma; Talapin, Dmitri V.

doi:10.1126/science.1260501

Title: Composition-matched molecular “solders” for semiconductors

Abstract

Soldering semiconductor nanoparticles The optical and electronic properties of semiconductor nanoparticles can be tuned through changes in their size and composition. However, poor contact between interfaces can degrade nanoparticle performance in devices. Dolzhnikov et al. report the synthesis of a gel-like “solder” for metal chalcogenide nanoparticles, such as cadmium selenide and lead telluride, by cross-linking molecular wires of these materials. Science , this issue p. 425

Authors:

Dolzhnikov, Dmitriy S. ^[1]; Zhang, Hao ^[1]; Jang, Jaeyoung ^[1]; Son, Jae Sung ^[1]; Panthani, Matthew G. ^[1]; Shibata, Tomohiro ^[2]; Chattopadhyay, Soma ^[2]; Talapin, Dmitri V. ^[3]

Department of Chemistry, University of Chicago, Chicago, IL 60637, USA., James Franck Institute, University of Chicago, Chicago, IL 60637, USA.
Materials Research Collaborative Access Team (MRCAT) Sector 10 Advanced Photon Source, Argonne National Laboratory, Argonne, IL 60439, USA., Department of Physics, Advanced Materials Group, Illinois Institute of Technology, Chicago, IL 60616, USA.
Department of Chemistry, University of Chicago, Chicago, IL 60637, USA., James Franck Institute, University of Chicago, Chicago, IL 60637, USA., Center for Nanoscale Materials, Argonne National Laboratory, Argonne, IL 60439, USA.

Publication Date:: Fri Jan 23 00:00:00 EST 2015

Sponsoring Org.:: USDOE

OSTI Identifier:: 1353291

Grant/Contract Number:: EE0005312

Resource Type:: Published Article

Journal Name:: Science

Additional Journal Information:: Journal Name: Science Journal Volume: 347 Journal Issue: 6220; Journal ID: ISSN 0036-8075

Publisher:: American Association for the Advancement of Science (AAAS)

Country of Publication:: United States

Language:: English

Citation Formats


                    Dolzhnikov, Dmitriy S., Zhang, Hao, Jang, Jaeyoung, Son, Jae Sung, Panthani, Matthew G., Shibata, Tomohiro, Chattopadhyay, Soma, and Talapin, Dmitri V. Composition-matched molecular “solders” for semiconductors.  United States: N. p., 2015. 
Web.  doi:10.1126/science.1260501.

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                    Dolzhnikov, Dmitriy S., Zhang, Hao, Jang, Jaeyoung, Son, Jae Sung, Panthani, Matthew G., Shibata, Tomohiro, Chattopadhyay, Soma, & Talapin, Dmitri V. Composition-matched molecular “solders” for semiconductors.  United States.  https://doi.org/10.1126/science.1260501

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                    Dolzhnikov, Dmitriy S., Zhang, Hao, Jang, Jaeyoung, Son, Jae Sung, Panthani, Matthew G., Shibata, Tomohiro, Chattopadhyay, Soma, and Talapin, Dmitri V. Fri .  
"Composition-matched molecular “solders” for semiconductors".  United States.  https://doi.org/10.1126/science.1260501.

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@article{osti_1353291,

  title        = {Composition-matched molecular “solders” for semiconductors},

  author       = {Dolzhnikov, Dmitriy S. and Zhang, Hao and Jang, Jaeyoung and Son, Jae Sung and Panthani, Matthew G. and Shibata, Tomohiro and Chattopadhyay, Soma and Talapin, Dmitri V.},

  abstractNote = {Soldering semiconductor nanoparticles The optical and electronic properties of semiconductor nanoparticles can be tuned through changes in their size and composition. However, poor contact between interfaces can degrade nanoparticle performance in devices. Dolzhnikov et al. report the synthesis of a gel-like “solder” for metal chalcogenide nanoparticles, such as cadmium selenide and lead telluride, by cross-linking molecular wires of these materials. Science , this issue p. 425},

  doi          = {10.1126/science.1260501},

  journal      = {Science},

  number       = 6220,

  volume       = 347,

  place        = {United States},

  year         = {Fri Jan 23 00:00:00 EST 2015},

  month        = {Fri Jan 23 00:00:00 EST 2015}

}

Copy to clipboard

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Title: Composition-matched molecular “solders” for semiconductors

Abstract

Citation Formats

PbSe Nanocrystal Solids for n- and p-Channel Thin Film Field-Effect Transistors journal, October 2005

ATHENA , ARTEMIS , HEPHAESTUS : data analysis for X-ray absorption spectroscopy using IFEFFIT journal, June 2005

Solution-processed silicon films and transistors journal, April 2006

PbSe Quantum Dot Field-Effect Transistors with Air-Stable Electron Mobilities above 7 cm 2 V –1 s –1 journal, March 2013

n-Type Conducting CdSe Nanocrystal Solids journal, May 2003

Dependence of Carrier Mobility on Nanocrystal Size and Ligand Length in PbSe Nanocrystal Solids journal, May 2010

Porous Semiconducting Gels and Aerogels from Chalcogenide Clusters journal, July 2007

Type conversion, contacts, and surface effects in electroplated CdTe films journal, November 1985

Universal and Solution-Processable Precursor to Bismuth Chalcogenide Thermoelectrics journal, March 2010

Ultra-high mobility transparent organic thin film transistors grown by an off-centre spin-coating method journal, January 2014

A High-Efficiency Solution-Deposited Thin-Film Photovoltaic Device journal, October 2008

Colloidal Nanocrystals with Molecular Metal Chalcogenide Surface Ligands journal, June 2009

High-mobility ultrathin semiconducting films prepared by spin coating journal, March 2004

Preparation and multinuclear magnetic resonance study of the Zintl anions, HgCh22-, CdCh22-, SnCh32-, TlCh33-, SnCh44-, and Tl2Ch22- (Ch = Se and/or Te). Chemical shift and coupling constant correlations journal, August 1985

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Low-Voltage Organic Transistors on Plastic Comprising High-Dielectric Constant Gate Insulators journal, February 1999

High-performance bulk thermoelectrics with all-scale hierarchical architectures journal, September 2012

Low Voltage, Hysteresis Free, and High Mobility Transistors from All-Inorganic Colloidal Nanocrystals journal, January 2012

Plastic and Moldable Metals by Self-Assembly of Sticky Nanoparticle Aggregates journal, April 2007

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Hole and electron drift velocity in CdSe at room temperature journal, July 1972

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Designing High-Performance PbS and PbSe Nanocrystal Electronic Devices through Stepwise, Post-Synthesis, Colloidal Atomic Layer Deposition journal, February 2014

Synthesis and Micrometer-Scale Assembly of Colloidal CdSe/CdS Nanorods Prepared by a Seeded Growth Approach journal, October 2007

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PbSe Nanocrystal Solids for n- and p-Channel Thin Film Field-Effect Transistors
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Solution-processed silicon films and transistors
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journal, March 2013

n-Type Conducting CdSe Nanocrystal Solids
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