DOE PAGES title logo U.S. Department of Energy
Office of Scientific and Technical Information

Title: Antineutrino monitoring of thorium reactors

Abstract

Various groups have demonstrated that antineutrino monitoring can be successful in assessing the plutonium content in water-cooled nuclear reactors for nonproliferation applications. New reactor designs and concepts incorporate nontraditional fuel types and chemistry. Understanding how these properties affect the antineutrino emission from a reactor can extend the applicability of antineutrino monitoring. Thorium molten salt reactors breed 233U, that if diverted constitute a direct use material as defined by the International Atomic Energy Agency (IAEA). The antineutrino spectrum from the fission of 233U has been estimated for the first time, and the feasibility of detecting the diversion of 8 kg of 233U, within a 30 day timeliness goal has been evaluated. The antineutrino emission from a thorium reactor operating under normal conditions is compared to a diversion scenario by evaluating the daily antineutrino count rate and the energy spectrum of the detected antineutrinos at a 25 m standoff. It was found that the diversion of a significant quantity of 233U could not be detected within the current IAEA timeliness detection goal using either tests. A rate-time based analysis exceeded the timeliness goal by 23 days, while a spectral based analysis exceeds this goal by 31 days.

Authors:
 [1];  [2];  [1]
  1. Univ. of California, Berkeley, CA (United States)
  2. Lawrence Livermore National Lab. (LLNL), Livermore, CA (United States)
Publication Date:
Research Org.:
Lawrence Livermore National Laboratory (LLNL), Livermore, CA (United States). Nuclear Science and Security Consortium
Sponsoring Org.:
USDOE National Nuclear Security Administration (NNSA)
OSTI Identifier:
1330747
Alternate Identifier(s):
OSTI ID: 1327554; OSTI ID: 1355350
Report Number(s):
LLNL-JRNL-703739
Journal ID: ISSN 0021-8979; JAPIAU; TRN: US1700111
Grant/Contract Number:  
AC52-07NA27344; NA0003180; NA0000979
Resource Type:
Accepted Manuscript
Journal Name:
Journal of Applied Physics
Additional Journal Information:
Journal Volume: 120; Journal Issue: 12; Journal ID: ISSN 0021-8979
Publisher:
American Institute of Physics (AIP)
Country of Publication:
United States
Language:
English
Subject:
11 NUCLEAR FUEL CYCLE AND RUEL MATERIALS; 73 NUCLEAR PHYSICS AND RADIATION PHYSICS; thorium; spectrum analysis; isotopes; beta decay; neutrons

Citation Formats

Akindele, Oluwatomi A., Bernstein, Adam, and Norman, Eric B. Antineutrino monitoring of thorium reactors. United States: N. p., 2016. Web. doi:10.1063/1.4963402.
Akindele, Oluwatomi A., Bernstein, Adam, & Norman, Eric B. Antineutrino monitoring of thorium reactors. United States. https://doi.org/10.1063/1.4963402
Akindele, Oluwatomi A., Bernstein, Adam, and Norman, Eric B. Fri . "Antineutrino monitoring of thorium reactors". United States. https://doi.org/10.1063/1.4963402. https://www.osti.gov/servlets/purl/1330747.
@article{osti_1330747,
title = {Antineutrino monitoring of thorium reactors},
author = {Akindele, Oluwatomi A. and Bernstein, Adam and Norman, Eric B.},
abstractNote = {Various groups have demonstrated that antineutrino monitoring can be successful in assessing the plutonium content in water-cooled nuclear reactors for nonproliferation applications. New reactor designs and concepts incorporate nontraditional fuel types and chemistry. Understanding how these properties affect the antineutrino emission from a reactor can extend the applicability of antineutrino monitoring. Thorium molten salt reactors breed 233U, that if diverted constitute a direct use material as defined by the International Atomic Energy Agency (IAEA). The antineutrino spectrum from the fission of 233U has been estimated for the first time, and the feasibility of detecting the diversion of 8 kg of 233U, within a 30 day timeliness goal has been evaluated. The antineutrino emission from a thorium reactor operating under normal conditions is compared to a diversion scenario by evaluating the daily antineutrino count rate and the energy spectrum of the detected antineutrinos at a 25 m standoff. It was found that the diversion of a significant quantity of 233U could not be detected within the current IAEA timeliness detection goal using either tests. A rate-time based analysis exceeded the timeliness goal by 23 days, while a spectral based analysis exceeds this goal by 31 days.},
doi = {10.1063/1.4963402},
journal = {Journal of Applied Physics},
number = 12,
volume = 120,
place = {United States},
year = {Fri Sep 30 00:00:00 EDT 2016},
month = {Fri Sep 30 00:00:00 EDT 2016}
}

Journal Article:
Free Publicly Available Full Text
Publisher's Version of Record

Citation Metrics:
Cited by: 1 work
Citation information provided by
Web of Science

Save / Share:

Works referenced in this record:

Detection of anomalous reactor activity using antineutrino count evolution over the course of a reactor cycle
journal, June 2011

  • Bulaevskaya, Vera; Bernstein, Adam
  • Journal of Applied Physics, Vol. 109, Issue 11
  • DOI: 10.1063/1.3594247

Development of an advanced antineutrino detector for reactor monitoring
journal, January 2015

  • Classen, T.; Bernstein, A.; Bowden, N. S.
  • Nuclear Instruments and Methods in Physics Research Section A: Accelerators, Spectrometers, Detectors and Associated Equipment, Vol. 771
  • DOI: 10.1016/j.nima.2014.10.022

Determination of antineutrino spectra from nuclear reactors
journal, August 2011


Reactor antineutrino spectra and their application to antineutrino-induced reactions. II
journal, October 1981


Experimental results from an antineutrino detector for cooperative monitoring of nuclear reactors
journal, March 2007

  • Bowden, N. S.; Bernstein, A.; Allen, M.
  • Nuclear Instruments and Methods in Physics Research Section A: Accelerators, Spectrometers, Detectors and Associated Equipment, Vol. 572, Issue 2
  • DOI: 10.1016/j.nima.2006.12.015

Radiative correction to the ν ¯ e ( ν e ) spectrum in β decay
journal, July 2011


Reactor-based neutrino oscillation experiments
journal, March 2002


Evaluated Nuclear Structure Data File (ENSDF)
book, January 1992


Antineutrino Monitoring for Heavy Water Reactors
journal, July 2014


Improved predictions of reactor antineutrino spectra
journal, May 2011


Systematic Uncertainties in the Analysis of the Reactor Neutrino Anomaly
journal, May 2014


Potential of thorium molten salt reactorsdetailed calculations and concept evolution with a view to large scale energy production
journal, January 2005


Experimental Determination of the Antineutrino Spectrum of the Fission Products of U 238
journal, March 2014


Spectral Structure of Electron Antineutrinos from Nuclear Reactors
journal, January 2015


Observation of the isotopic evolution of pressurized water reactor fuel using an antineutrino detector
journal, March 2009

  • Bowden, N. S.; Bernstein, A.; Dazeley, S.
  • Journal of Applied Physics, Vol. 105, Issue 6, Article No. 064902
  • DOI: 10.1063/1.3080251