Nuclear magnetic resonance studies of pseudospin fluctuations in URu2Si2

Shirer, K. R.; Haraldsen, J. T.; Dioguardi, A. P.; Crocker, J.; apRoberts-Warren, N.; Shockley, A. C.; Lin, C. -H.; Nisson, D. M.; Cooley, J. C.; Janoschek, M.; Huang, K.; Kanchanavatee, N.; Maple, M. B.; Graf, M. J.; Balatsky, A. V.; Curro, N. J.

doi:10.1103/PhysRevB.88.094436

Title: Nuclear magnetic resonance studies of pseudospin fluctuations in URu $_{2}$ Si $_{2}$

Abstract

Here, we report ²⁹Si nuclear magnetic resonance measurements in single crystals and aligned powders of URu₂Si₂ in the hidden order and paramagnetic phases. The spin-lattice relaxation data reveal evidence of pseudospin fluctuations of U moments in the paramagnetic phase. We find evidence for partial suppression of the density of states below 30 K and analyze the data in terms of a two-component spin-fermion model. We propose that this behavior is a realization of a pseudogap between the hidden-order transition T_HO and 30 K. This behavior is then compared to other materials that demonstrate precursor fluctuations in a pseudogap regime above a ground state with long-range order.

Authors:

Shirer, K. R. ^[1]; Haraldsen, J. T. ^[2]; Dioguardi, A. P. ^[1]; Crocker, J. ^[1]; apRoberts-Warren, N. ^[1]; Shockley, A. C. ^[1]; Lin, C. -H. ^[1]; Nisson, D. M. ^[1]; Cooley, J. C. ^[2]; Janoschek, M. ^[3]; Huang, K. ^[3]; Kanchanavatee, N. ^[3]; Maple, M. B. ^[3]; Graf, M. J. ^[2]; Balatsky, A. V. ^[4]; Curro, N. J. ^[1]

Univ. of California, Davis, CA (United States)
Los Alamos National Lab. (LANL), Los Alamos, NM (United States)
Univ. of California, San Diego, La Jolla, CA (United States)
Los Alamos National Lab. (LANL), Los Alamos, NM (United States); NORDITA, Stockholm (Sweden)

Publication Date:: Thu Sep 26 00:00:00 EDT 2013

Research Org.:: Univ. of California, Davis, CA (United States)

Sponsoring Org.:: USDOE

OSTI Identifier:: 1329380

Grant/Contract Number:: FG52-09NA29464

Resource Type:: Accepted Manuscript

Journal Name:: Physical Review. B, Condensed Matter and Materials Physics

Additional Journal Information:: Journal Volume: 88; Journal Issue: 9; Journal ID: ISSN 1098-0121

Publisher:: American Physical Society (APS)

Country of Publication:: United States

Language:: English

Subject:: 75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND SUPERFLUIDITY

Citation Formats


                    Shirer, K. R., Haraldsen, J. T., Dioguardi, A. P., Crocker, J., apRoberts-Warren, N., Shockley, A. C., Lin, C. -H., Nisson, D. M., Cooley, J. C., Janoschek, M., Huang, K., Kanchanavatee, N., Maple, M. B., Graf, M. J., Balatsky, A. V., and Curro, N. J. Nuclear magnetic resonance studies of pseudospin fluctuations in URu2Si2.  United States: N. p., 2013. 
Web.  doi:10.1103/PhysRevB.88.094436.

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                    Shirer, K. R., Haraldsen, J. T., Dioguardi, A. P., Crocker, J., apRoberts-Warren, N., Shockley, A. C., Lin, C. -H., Nisson, D. M., Cooley, J. C., Janoschek, M., Huang, K., Kanchanavatee, N., Maple, M. B., Graf, M. J., Balatsky, A. V., & Curro, N. J. Nuclear magnetic resonance studies of pseudospin fluctuations in URu2Si2.  United States.  https://doi.org/10.1103/PhysRevB.88.094436

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                    Shirer, K. R., Haraldsen, J. T., Dioguardi, A. P., Crocker, J., apRoberts-Warren, N., Shockley, A. C., Lin, C. -H., Nisson, D. M., Cooley, J. C., Janoschek, M., Huang, K., Kanchanavatee, N., Maple, M. B., Graf, M. J., Balatsky, A. V., and Curro, N. J. Thu .  
"Nuclear magnetic resonance studies of pseudospin fluctuations in URu2Si2".  United States.  https://doi.org/10.1103/PhysRevB.88.094436.  https://www.osti.gov/servlets/purl/1329380.

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@article{osti_1329380,

  title        = {Nuclear magnetic resonance studies of pseudospin fluctuations in URu2Si2},

  author       = {Shirer, K. R. and Haraldsen, J. T. and Dioguardi, A. P. and Crocker, J. and apRoberts-Warren, N. and Shockley, A. C. and Lin, C. -H. and Nisson, D. M. and Cooley, J. C. and Janoschek, M. and Huang, K. and Kanchanavatee, N. and Maple, M. B. and Graf, M. J. and Balatsky, A. V. and Curro, N. J.},

  abstractNote = {Here, we report 29Si nuclear magnetic resonance measurements in single crystals and aligned powders of URu2Si2 in the hidden order and paramagnetic phases. The spin-lattice relaxation data reveal evidence of pseudospin fluctuations of U moments in the paramagnetic phase. We find evidence for partial suppression of the density of states below 30 K and analyze the data in terms of a two-component spin-fermion model. We propose that this behavior is a realization of a pseudogap between the hidden-order transition THO and 30 K. This behavior is then compared to other materials that demonstrate precursor fluctuations in a pseudogap regime above a ground state with long-range order.},

  doi          = {10.1103/PhysRevB.88.094436},

  journal      = {Physical Review. B, Condensed Matter and Materials Physics},

  number       = 9,

  volume       = 88,

  place        = {United States},

  year         = {Thu Sep 26 00:00:00 EDT 2013},

  month        = {Thu Sep 26 00:00:00 EDT 2013}

}

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Works referencing / citing this record:

Evidence for a nematic component to the hidden-order parameter in URu2Si2 from differential elastoresistance measurements
journal, March 2015

Riggs, Scott C.; Shapiro, M. C.; Maharaj, Akash V.
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Evidence for a nematic component to the Hidden Order parameter in URu2Si2 from differential elastoresistance measurements
text, January 2014

Riggs, Scott C.; Shapiro, M. C.; Maharaj, Akash V.
arXiv
DOI: 10.48550/arxiv.1405.7403

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Title: Nuclear magnetic resonance studies of pseudospin fluctuations in URu 2 Si 2

Abstract

Citation Formats

Colloquium : Hidden order, superconductivity, and magnetism: The unsolved case of URu 2 Si 2 journal, November 2011

Exotic Superconducting Properties in the Electron-Hole-Compensated Heavy-Fermion “Semimetal” URu 2 Si 2 journal, September 2007

Magnetic excitations and ordering in the heavy-electron superconductor URu 2 Si 2 journal, April 1987

Analysis of Si NMR line-width in journal, March 2007

Partially gapped Fermi surface in the heavy-electron superconductor URu 2 Si 2 journal, January 1986

Hidden orbital order in the heavy fermion metal URu2Si2 journal, June 2002

Interplay between spin-density wave and induced local moments in URu 2 Si 2 journal, July 2005

Spin-orbit density wave induced hidden topological order in URu2Si2 journal, August 2012

Phase transition arising from the underscreened Anderson lattice model: A candidate concept for explaining hidden order in URu 2 Si 2 journal, April 2012

Hidden order in URu2Si2 originates from Fermi surface gapping induced by dynamic symmetry breaking journal, February 2009

Hastatic order in the heavy-fermion compound URu2Si2 journal, January 2013

Hybridization Wave as the “Hidden Order” in URu 2 Si 2 journal, February 2011

Gapped itinerant spin excitations account for missing entropy in the hidden-order state of URu2Si2 journal, January 2007

Precise Study of the Resonance at Q 0 =(1,0,0) in URu 2 Si 2 journal, June 2010

Anomalous femtosecond quasiparticle dynamics of hidden order state in URu 2 Si 2 journal, October 2011

Formation of the Coherent Heavy Fermion Liquid at the Hidden Order Transition in URu 2 Si 2 journal, May 2013

Momentum-Resolved Evolution of the Kondo Lattice into “Hidden Order” in URu 2 Si 2 journal, April 2013

The Kondo Problem to Heavy Fermions book, January 1993

Arrested Kondo effect and hidden order in URu2Si2 journal, September 2009

Imaging the Fano lattice to ‘hidden order’ transition in URu2Si2 journal, June 2010

Visualizing the formation of the Kondo lattice and the hidden order in URu2Si2 journal, May 2010

Hidden-order pseudogap in URu 2 Si 2 journal, December 2011

Point-contact spectroscopy of superconducting URu 2 Si 2 journal, September 1992

Itinerant spin excitations near the hidden order transition in URu 2 Si 2 journal, April 2009

Specific heat of heavy-fermion URu 2 Si 2 in high magnetic fields journal, December 1997

Thermal expansion and specific heat of monocrystalline U Ru 2 Si 2 journal, December 1986

Elastic properties of the heavy fermion superconductor URu2Si2 journal, February 1994

Far-Infrared Properties of URu 2 Si 2 journal, September 1988

Evidence of a hidden-order pseudogap state in URu 2 Si 2 using ultrafast optical spectroscopy journal, October 2011

Hybridization gap and anisotropic far-infrared optical conductivity of URu 2 Si 2 journal, November 2011

Observation of the Hybridization Gap and Fano Resonance in the Kondo Lattice URu 2 Si 2 journal, June 2012

Point-contact spectroscopy on URu 2 Si 2 journal, June 1997

Temperature dependence of the antiferromagnetic state in URu 2 Si 2 by point-contact spectroscopy journal, June 1994

Magnetic state in URu2Si2, UPd2Al3, and UNi2Al3 probed by point contacts journal, June 2001

Anisotropy of the gapped Fermi surface of URu2Si2 in the antiferromagnetic state studied by point contact spectroscopy journal, February 1996

Point-contact study of the heavy-fermion system URu2Si2 journal, October 1992

Pressure-tuned point-contact spectroscopy of URu 2 Si 2 from hidden order to antiferromagnetic states: Similarity of the Fermi surface gapping journal, January 2012

Long range order and two-fluid behavior in heavy electron materials journal, September 2012

Reentrant Hidden Order at a Metamagnetic Quantum Critical End Point journal, March 2003

29 Si NMR Study of Antiferromagnetic Superconductor URu 2 Si 2 journal, April 1996

Antiferromagnetic patches and hidden order in URu 2 Si 2 by impurity doping journal, April 2010

Construction of a microscopic model for f -electron systems on the basis of a j − j coupling scheme journal, March 2003

Pressure–temperature phase diagram of the heavy-electron superconductor journal, March 2007

Two-Dimensional Fluctuations at the Quantum-Critical Point of CeCu 6 − x Au x journal, June 1998

Quantum criticality in heavy-fermion metals journal, March 2008

Nuclear spin-lattice relaxation rate in Pu M Ga 5 ( M = Rh , Co ) : A two-component spin-fermion model journal, August 2006

Two-dimensional quantum Heisenberg antiferromagnet at low temperatures journal, February 1989

Optical spectroscopy shows that the normal state of URu2Si2 is an anomalous Fermi liquid journal, October 2012

Cu 63 (2) nuclear quadrupole and nuclear magnetic resonance studies of Y Ba 2 Cu 4 O 8 in the normal and superconducting states journal, March 1996

Unconventional superconductivity in PuCoGa5 journal, March 2005

Evidence for a nematic component to the hidden-order parameter in URu2Si2 from differential elastoresistance measurements journal, March 2015

Hidden order behaviour in URu 2 Si 2 (A critical review of the status of hidden order in 2014) journal, May 2014

Hidden Order Behaviour in URu2Si2 (A Critical Review of the Status of Hidden Order in 2014) text, January 2014

Evidence for a nematic component to the Hidden Order parameter in URu2Si2 from differential elastoresistance measurements text, January 2014

Title: Nuclear magnetic resonance studies of pseudospin fluctuations in URu $_{2}$ Si $_{2}$

Colloquium : Hidden order, superconductivity, and magnetism: The unsolved case of ${URu}_{2} {Si}_{2}$
journal, November 2011

Exotic Superconducting Properties in the Electron-Hole-Compensated Heavy-Fermion “Semimetal” ${URu}_{2} {Si}_{2}$
journal, September 2007

Magnetic excitations and ordering in the heavy-electron superconductor ${URu}_{2}$ ${Si}_{2}$
journal, April 1987

Analysis of Si NMR line-width in
journal, March 2007

Partially gapped Fermi surface in the heavy-electron superconductor ${URu}_{2}$ ${Si}_{2}$
journal, January 1986

Hidden orbital order in the heavy fermion metal URu2Si2
journal, June 2002

Interplay between spin-density wave and induced local moments in ${URu}_{2} {Si}_{2}$
journal, July 2005

Spin-orbit density wave induced hidden topological order in URu2Si2
journal, August 2012

Phase transition arising from the underscreened Anderson lattice model: A candidate concept for explaining hidden order in URu $_{2}$ Si $_{2}$
journal, April 2012

Hidden order in URu2Si2 originates from Fermi surface gapping induced by dynamic symmetry breaking
journal, February 2009

Hastatic order in the heavy-fermion compound URu2Si2
journal, January 2013

Hybridization Wave as the “Hidden Order” in ${URu}_{2} {Si}_{2}$
journal, February 2011

Gapped itinerant spin excitations account for missing entropy in the hidden-order state of URu2Si2
journal, January 2007

Precise Study of the Resonance at Q ₀ =(1,0,0) in URu ₂ Si ₂
journal, June 2010

Anomalous femtosecond quasiparticle dynamics of hidden order state in URu $_{2}$ Si $_{2}$
journal, October 2011

Formation of the Coherent Heavy Fermion Liquid at the Hidden Order Transition in ${URu}_{2} {Si}_{2}$
journal, May 2013

Momentum-Resolved Evolution of the Kondo Lattice into “Hidden Order” in ${URu}_{2} {Si}_{2}$
journal, April 2013

The Kondo Problem to Heavy Fermions
book, January 1993

Arrested Kondo effect and hidden order in URu2Si2
journal, September 2009

Imaging the Fano lattice to ‘hidden order’ transition in URu2Si2
journal, June 2010

Visualizing the formation of the Kondo lattice and the hidden order in URu2Si2
journal, May 2010

Hidden-order pseudogap in URu $_{2}$ Si $_{2}$
journal, December 2011

Point-contact spectroscopy of superconducting ${URu}_{2}$ ${Si}_{2}$
journal, September 1992

Itinerant spin excitations near the hidden order transition in URu ₂ Si ₂
journal, April 2009

Specific heat of heavy-fermion ${URu}_{2} {Si}_{2}$ in high magnetic fields
journal, December 1997

Thermal expansion and specific heat of monocrystalline U ${Ru}_{2}$ ${Si}_{2}$
journal, December 1986

Elastic properties of the heavy fermion superconductor URu2Si2
journal, February 1994

Far-Infrared Properties of ${URu}_{2}$ ${Si}_{2}$
journal, September 1988

Evidence of a hidden-order pseudogap state in URu $_{2}$ Si $_{2}$ using ultrafast optical spectroscopy
journal, October 2011

Hybridization gap and anisotropic far-infrared optical conductivity of URu $_{2}$ Si $_{2}$
journal, November 2011

Observation of the Hybridization Gap and Fano Resonance in the Kondo Lattice ${URu}_{2} {Si}_{2}$
journal, June 2012

Point-contact spectroscopy on ${URu}_{2}$ ${Si}_{2}$
journal, June 1997

Temperature dependence of the antiferromagnetic state in ${URu}_{2}$ ${Si}_{2}$ by point-contact spectroscopy
journal, June 1994

Magnetic state in URu2Si2, UPd2Al3, and UNi2Al3 probed by point contacts
journal, June 2001

Anisotropy of the gapped Fermi surface of URu2Si2 in the antiferromagnetic state studied by point contact spectroscopy
journal, February 1996

Point-contact study of the heavy-fermion system URu2Si2
journal, October 1992

Pressure-tuned point-contact spectroscopy of URu $_{2}$ Si $_{2}$ from hidden order to antiferromagnetic states: Similarity of the Fermi surface gapping
journal, January 2012

Long range order and two-fluid behavior in heavy electron materials
journal, September 2012

Reentrant Hidden Order at a Metamagnetic Quantum Critical End Point
journal, March 2003

²⁹ Si NMR Study of Antiferromagnetic Superconductor URu ₂ Si ₂
journal, April 1996

Antiferromagnetic patches and hidden order in ${URu}_{2} {Si}_{2}$ by impurity doping
journal, April 2010

Construction of a microscopic model for f -electron systems on the basis of a $j - j$ coupling scheme
journal, March 2003

Pressure–temperature phase diagram of the heavy-electron superconductor
journal, March 2007

Two-Dimensional Fluctuations at the Quantum-Critical Point of ${CeCu}_{6 - x} {Au}_{x}$
journal, June 1998

Quantum criticality in heavy-fermion metals
journal, March 2008

Nuclear spin-lattice relaxation rate in $Pu M {Ga}_{5}$ $(M = Rh, Co)$ : A two-component spin-fermion model
journal, August 2006

Two-dimensional quantum Heisenberg antiferromagnet at low temperatures
journal, February 1989

Optical spectroscopy shows that the normal state of URu2Si2 is an anomalous Fermi liquid
journal, October 2012

${}^{63}{Cu}$ (2) nuclear quadrupole and nuclear magnetic resonance studies of Y ${Ba}_{2}$ ${Cu}_{4}$ $O_{8}$ in the normal and superconducting states
journal, March 1996

Unconventional superconductivity in PuCoGa5
journal, March 2005

Evidence for a nematic component to the hidden-order parameter in URu2Si2 from differential elastoresistance measurements
journal, March 2015

Hidden order behaviour in URu ₂ Si ₂ (A critical review of the status of hidden order in 2014)
journal, May 2014

Hidden Order Behaviour in URu2Si2 (A Critical Review of the Status of Hidden Order in 2014)
text, January 2014

Evidence for a nematic component to the Hidden Order parameter in URu2Si2 from differential elastoresistance measurements
text, January 2014