Progress in the analysis of complex atmospheric particles

Journal Article · Wed Jun 01 00:00:00 EDT 2016 · Annual Review of Analytical Chemistry

DOI: https://doi.org/10.1146/annurev-anchem-071015-041521 · OSTI ID:1311631

Laskin, Alexander ^[1]; Gilles, Mary K. ^[2]; Knopf, Daniel A. ^[3]; Wang, Bingbing ^[1]; China, Swarup ^[1]

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1. Pacific Northwest National Lab. (PNNL), Richland, WA (United States)
2. Lawrence Berkeley National Lab. (LBNL), Berkeley, CA (United States)
3. Stony Brook Univ., Stony Brook, NY (United States)

This study presents an overview of recent advances in field and laboratory studies of atmospheric particles formed in processes of environmental air-surface interactions. The overarching goal of these studies is to advance predictive understanding of atmospheric particle composition, particle chemistry during aging, and their environmental impacts. The diversity between chemical constituents and lateral heterogeneity within individual particles adds to the chemical complexity of particles and their surfaces. Once emitted, particles undergo transformation via atmospheric aging processes that further modify their complex composition. We highlight a range of modern analytical approaches that enable multimodal chemical characterization of particles with both molecular and lateral specificity. When combined, these approaches provide a comprehensive arsenal of tools for understanding the nature of particles at air-surface interactions and their reactivity and transformations with atmospheric aging. We discuss applications of these novel approaches in recent studies and highlight additional research areas to explore the environmental effects of air-surface interactions.

• Research Organization: Lawrence Berkeley National Laboratory (LBNL), Berkeley, CA (United States)
• Sponsoring Organization: USDOE Office of Science (SC), Basic Energy Sciences (BES) (SC-22); USDOE Office of Science (SC), Biological and Environmental Research (BER) (SC-23); National Science Foundation (NSF)
• Grant/Contract Number: AC02-05CH11231; SC0008613
• OSTI ID: 1311631
• Report Number(s): LBNL--1006038; ir:1006038
• Journal Information: Annual Review of Analytical Chemistry, Journal Name: Annual Review of Analytical Chemistry Journal Issue: 1 Vol. 9; ISSN 1936-1327
• Publisher: Annual ReviewsCopyright Statement
• Country of Publication: United States
• Language: English

Related Subjects

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CHEMISTRY
54 ENVIRONMENTAL SCIENCES
aerosol
atmospheric aging
chemical imaging
environmental interfaces
molecular-level
multi-phase chemistry