Surface engineering of hierarchical platinum-cobalt nanowires for efficient electrocatalysis

Bu, Lingzheng; Guo, Shaojun; Zhang, Xu; Shen, Xuan; Su, Dong; Lu, Gang; Zhu, Xing; Yao, Jianlin; Guo, Jun; Huang, Xiaoqing

doi:10.1038/ncomms11850

Title: Surface engineering of hierarchical platinum-cobalt nanowires for efficient electrocatalysis

Journal Article · Wed Jun 29 04:00:00 UTC 2016 · Nature Communications

DOI: https://doi.org/10.1038/ncomms11850 · OSTI ID:1307420

Bu, Lingzheng ^[1]; Guo, Shaojun ^[2]; Zhang, Xu ^[3]; Shen, Xuan ^[4]; Su, Dong ^[4]; Lu, Gang ^[3]; Zhu, Xing ^[5]; Yao, Jianlin ^[5]; Guo, Jun ^[5]; Huang, Xiaoqing ^[5]

Soochow Univ., Jiangsu (China); Peking University, China
Peking Univ., Beijing (China)
California State Univ. (CalState), Northridge, CA (United States)
Brookhaven National Lab. (BNL), Upton, NY (United States)
Soochow Univ., Jiangsu (China)

Despite intense research in past decades, the lack of high-performance catalysts for fuel cell reactions remains a challenge in realizing fuel cell technologies for transportation applications. Here we report a facile strategy for synthesizing hierarchical platinum-cobalt nanowires with high-index, platinum-rich facets and ordered intermetallic structure. These structural features enable unprecedented performance for the oxygen reduction and alcohol oxidation reactions. The specific/mass activities of the platinum-cobalt nanowires for oxygen reduction reaction are 39.6/33.7 times higher than commercial Pt/C catalyst, respectively. Density functional theory simulations reveal that the active threefold hollow sites on the platinum-rich high-index facets provide an additional factor in enhancing oxygen reduction reaction activities. The nanowires are stable in the electrochemical conditions and also thermally stable. Furthermore, this work may represent a key step towards scalable production of high performance platinum-based nanowires for applications in catalysis and energy conversion.

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Research Organization:: Brookhaven Science Associates, LLC, Upton, NY (United States)

Sponsoring Organization:: USDOE Office of Science (SC), Basic Energy Sciences (BES) (SC-22)

Grant/Contract Number:: SC0012704

OSTI ID:: 1307420

Journal Information:: Nature Communications, Journal Name: Nature Communications Vol. 7; ISSN 2041-1723

Publisher:: Nature Publishing GroupCopyright Statement

Country of Publication:: United States

Language:: English

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Tungsten‐Doped L1 ₀ ‐PtCo Ultrasmall Nanoparticles as a High‐Performance Fuel Cell Cathode Liang, Jiashun; Li, Na; Zhao, Zhonglong Angewandte Chemie, Vol. 131, Issue 43 https://doi.org/10.1002/ange.201908824	journal	September 2019
Crystallinity-Modulated Electrocatalytic Activity of a Nickel(II) Borate Thin Layer on Ni ₃ B for Efficient Water Oxidation Jiang, Wen-Jie; Niu, Shuai; Tang, Tang Angewandte Chemie International Edition, Vol. 56, Issue 23 https://doi.org/10.1002/anie.201703183	journal	May 2017
General π-Electron-Assisted Strategy for Ir, Pt, Ru, Pd, Fe, Ni Single-Atom Electrocatalysts with Bifunctional Active Sites for Highly Efficient Water Splitting Lai, Wei-Hong; Zhang, Li-Fu; Hua, Wei-Bo Angewandte Chemie International Edition, Vol. 58, Issue 34 https://doi.org/10.1002/anie.201904614	journal	July 2019
Tungsten‐Doped L1 ₀ ‐PtCo Ultrasmall Nanoparticles as a High‐Performance Fuel Cell Cathode Liang, Jiashun; Li, Na; Zhao, Zhonglong Angewandte Chemie International Edition, Vol. 58, Issue 43 https://doi.org/10.1002/anie.201908824	journal	October 2019
Design and Application of Foams for Electrocatalysis Zhu, Wenxin; Zhang, Rong; Qu, Fengli ChemCatChem, Vol. 9, Issue 10 https://doi.org/10.1002/cctc.201601607	journal	May 2017
Constructing an Atomic Layer Pt Electrocatalyst with a Concave Curved Surface for the Oxygen Reduction Reaction Li, Jian; Gao, Yong-Fu; Yin, Hui-Ming ChemElectroChem, Vol. 4, Issue 10 https://doi.org/10.1002/celc.201700442	journal	July 2017
Facile Solvothermal Synthesis of Pt ₄ Co Multi-dendrites: An Effective Electrocatalyst for Oxygen Reduction and Glycerol Oxidation Jiang, Liu-Ying; Wang, Ai-Jun; Li, Xin-Sheng ChemElectroChem, Vol. 4, Issue 11 https://doi.org/10.1002/celc.201700640	journal	September 2017
In Situ Incorporation Strategy for Bimetallic FeCo-Doped Carbon as Highly Efficient Bifunctional Oxygen Electrocatalysts Shui, Hengxin; Jin, Tian; Hu, Jun ChemElectroChem, Vol. 5, Issue 10 https://doi.org/10.1002/celc.201800013	journal	April 2018
Ternary PtPdCu Multicubes as a Highly Active and Durable Catalyst toward the Oxygen Reduction Reaction An, Hong Ming; Zhao, Zhi Liang; Wang, Qi ChemElectroChem, Vol. 5, Issue 10 https://doi.org/10.1002/celc.201800202	journal	March 2018
Phase Modulating of Cu–Ni Nanowires Enables Active and Stable Electrocatalysts for the Methanol Oxidation Reaction Tong, Wu; Shao, Qi; Wang, Pengtang Chemistry – A European Journal, Vol. 25, Issue 29 https://doi.org/10.1002/chem.201901064	journal	April 2019
2D Metal–Organic Framework Derived CuCo Alloy Nanoparticles Encapsulated by Nitrogen‐Doped Carbonaceous Nanoleaves for Efficient Bifunctional Oxygen Electrocatalyst and Zinc–Air Batteries Huo, Meiling; Wang, Bin; Zhang, Chaochao Chemistry – A European Journal, Vol. 25, Issue 55 https://doi.org/10.1002/chem.201902389	journal	September 2019
Hollow PtFe Alloy Nanoparticles Derived from Pt‐Fe ₃ O ₄ Dimers through a Silica‐Protection Reduction Strategy as Efficient Oxygen Reduction Electrocatalysts Yang, Zhaojun; Shang, Lu; Xiong, Xuyang Chemistry – A European Journal https://doi.org/10.1002/chem.201904208	journal	January 2020
Pt Islands on 3 D Nut-like PtAg Nanocrystals for Efficient Formic Acid Oxidation Electrocatalysis Xu, Hui; Song, Pingping; Yan, Bo ChemSusChem, Vol. 11, Issue 6 https://doi.org/10.1002/cssc.201702409	journal	February 2018
Gold-Copper Aerogels with Intriguing Surface Electronic Modulation as Highly Active and Stable Electrocatalysts for Oxygen Reduction and Borohydride Oxidation Wang, Jiali; Chen, Fuyi; Jin, Yachao ChemSusChem, Vol. 11, Issue 8 https://doi.org/10.1002/cssc.201800052	journal	March 2018
Nanocatalysts for Electrocatalytic Oxidation of Ethanol Bai, Juan; Liu, Danye; Yang, Jun ChemSusChem, Vol. 12, Issue 10 https://doi.org/10.1002/cssc.201803063	journal	April 2019
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Hollow PtNi Nanochains as Highly Efficient and Stable Oxygen Reduction Reaction Catalysts Li, Wenping; Li, Chuang; Qi, Ji ChemistrySelect, Vol. 4, Issue 3 https://doi.org/10.1002/slct.201803697	journal	January 2019
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The OH ⁻ -driven synthesis of Pt–Ni nanocatalysts with atomic segregation for alkaline hydrogen evolution reaction Zhang, Cong; Chen, Biaohua; Mei, Donghai Journal of Materials Chemistry A, Vol. 7, Issue 10 https://doi.org/10.1039/c8ta12250d	journal	January 2019
Multidimensional nanostructured membrane electrode assemblies for proton exchange membrane fuel cell applications Wang, Guoliang; Zou, Liangliang; Huang, Qinghong Journal of Materials Chemistry A, Vol. 7, Issue 16 https://doi.org/10.1039/c8ta12382a	journal	January 2019
Localized surface plasmon enhanced electrocatalytic methanol oxidation of AgPt bimetallic nanoparticles with an ultra-thin shell Bi, Jinglei; Cai, Hairui; Wang, Bin Chemical Communications, Vol. 55, Issue 27 https://doi.org/10.1039/c9cc00331b	journal	January 2019
Synthesis of ammonia via electrochemical nitrogen reduction on high-index faceted Au nanoparticles with a high faradaic efficiency Tan, Lianqiao; Yang, Na; Huang, Xun Chemical Communications, Vol. 55, Issue 96 https://doi.org/10.1039/c9cc06132k	journal	January 2019
Regulating locations of active sites: a novel strategy to greatly improve the stability of PtAu electrocatalysts Xu, Suying; Hou, Wenjie; Jiang, Rui Chemical Communications, Vol. 55, Issue 90 https://doi.org/10.1039/c9cc07275f	journal	January 2019
Concave PtCo nanooctahedra with high-energy {110} facets for the oxygen reduction reaction Li, Zhijuan; Wang, Xiaoru; Zhang, Zhenbo CrystEngComm, Vol. 22, Issue 9 https://doi.org/10.1039/c9ce01488h	journal	January 2020
Preparation of Ni@Pt core@shell conformal nanofibre oxygen reduction electrocatalysts via microwave-assisted galvanic displacement Ercolano, Giorgio; Farina, Filippo; Stievano, Lorenzo Catalysis Science & Technology, Vol. 9, Issue 24 https://doi.org/10.1039/c9cy01514k	journal	January 2019
Atomically dispersed metal catalysts for the oxygen reduction reaction: synthesis, characterization, reaction mechanisms and electrochemical energy applications Liu, Minmin; Wang, Linlin; Zhao, Kangning Energy & Environmental Science, Vol. 12, Issue 10 https://doi.org/10.1039/c9ee01722d	journal	January 2019
Ultra-small intermetallic NiZn nanoparticles: a non-precious metal catalyst for efficient electrocatalysis Samanta, Arnab; Das, Sankar; Jana, Subhra Nanoscale Advances, Vol. 2, Issue 1 https://doi.org/10.1039/c9na00611g	journal	January 2020
One-pot synthesis of PtIn/3D-GNs composites with high alloying degree for electro-photo synergistic catalysis Ye, Yixiang; Wang, Yanli; Li, Zhongshui New Journal of Chemistry, Vol. 43, Issue 43 https://doi.org/10.1039/c9nj04367e	journal	January 2019
In situ high-potential-driven surface restructuring of ternary AgPd–Pt _dilute aerogels with record-high performance improvement for formate oxidation electrocatalysis Wang, Jiali; Chen, Fuyi; Jin, Yachao Nanoscale, Vol. 11, Issue 30 https://doi.org/10.1039/c9nr03266e	journal	January 2019
Cyanogel auto-reduction induced synthesis of PdCo nanocubes on carbon nanobowls: a highly active electrocatalyst for ethanol electrooxidation Xu, Guang-Rui; Zhai, Ya-Nan; Li, Fu-min Nanoscale, Vol. 11, Issue 28 https://doi.org/10.1039/c9nr04767k	journal	January 2019
Nanoscale engineering of porous Fe-doped Pd nanosheet assemblies for efficient methanol and ethanol electrocatalyses Xu, Hui; Shang, Hongyuan; Wang, Cheng Nanoscale, Vol. 12, Issue 3 https://doi.org/10.1039/c9nr09755d	journal	January 2020
Shaping well-defined noble-metal-based nanostructures for fabricating high-performance electrocatalysts: advances and perspectives Yin, Hai-Jing; Zhou, Jun-Hao; Zhang, Ya-Wen Inorganic Chemistry Frontiers, Vol. 6, Issue 10 https://doi.org/10.1039/c9qi00689c	journal	January 2019
Understanding the roles of amorphous domains and oxygen-containing groups of nitrogen-doped carbon in oxygen reduction catalysis: toward superior activity Biemolt, Jasper; Rothenberg, Gadi; Yan, Ning Inorganic Chemistry Frontiers, Vol. 7, Issue 1 https://doi.org/10.1039/c9qi00983c	journal	January 2020
Transition metal-doped ultrathin RuO ₂ networked nanowires for efficient overall water splitting across a broad pH range Wang, Juan; Ji, Yujin; Yin, Rongguan Journal of Materials Chemistry A, Vol. 7, Issue 11 https://doi.org/10.1039/c9ta00598f	journal	January 2019
Morphology controllable synthesis of PtNi concave nanocubes enclosed by high-index facets supported on porous graphene for enhanced hydrogen evolution reaction Yang, Juntao; Ning, Guoqing; Yu, Lei Journal of Materials Chemistry A, Vol. 7, Issue 30 https://doi.org/10.1039/c9ta03442k	journal	January 2019
Facile synthesis of ultrathin Pt–Pd nanosheets for enhanced formic acid oxidation and oxygen reduction reaction Yang, Qian; Shi, Lijie; Yu, Beibei Journal of Materials Chemistry A, Vol. 7, Issue 32 https://doi.org/10.1039/c9ta03945g	journal	January 2019
One-step solid-phase boronation to fabricate self-supported porous FeNiB/FeNi foam for efficient electrocatalytic oxygen evolution and overall water splitting Yuan, Hefeng; Wang, Shumin; Gu, Xundi Journal of Materials Chemistry A, Vol. 7, Issue 33 https://doi.org/10.1039/c9ta04076e	journal	January 2019
Advanced engineering of core/shell nanostructures for electrochemical carbon dioxide reduction Shao, Qi; Wang, Pengtang; Liu, Shangheng Journal of Materials Chemistry A, Vol. 7, Issue 36 https://doi.org/10.1039/c9ta07016h	journal	January 2019
Interfacial synergy of ultralong jagged Pt ₈₅ Mo ₁₅ –S nanowires with abundant active sites on enhanced hydrogen evolution in an alkaline solution Wang, Yao; Zhuo, Hongying; Zhang, Xin Journal of Materials Chemistry A, Vol. 7, Issue 42 https://doi.org/10.1039/c9ta09285d	journal	January 2019
SnO ₂ patched ultrathin PtRh nanowires as efficient catalysts for ethanol electrooxidation Fan, Xiaokun; Tang, Min; Wu, Xiaotong Journal of Materials Chemistry A, Vol. 7, Issue 48 https://doi.org/10.1039/c9ta10941b	journal	January 2019
Asymmetric PdPtCu mesoporous hemispheres on nitrogen-functionalized graphene for methanol oxidation electrocatalysis Sun, Lizhi; Lv, Hao; Xu, Dongdong Journal of Materials Chemistry A, Vol. 8, Issue 31 https://doi.org/10.1039/c9ta13478f	journal	January 2020
Cobalt-platinum nanomotors for local gas generation Szkudlarek, Aleksandra; Hnida-Gut, Katarzyna E.; Kollbek, Kamila Nanotechnology, Vol. 31, Issue 7 https://doi.org/10.1088/1361-6528/ab53bd	journal	November 2019
Monatomic Co, CoO 2 , and CoO 3 nanowires on Ir(100) and Pt(100) surfaces: Formation, structure, and energetics Ferstl, P.; Mittendorfer, F.; Redinger, J. Physical Review B, Vol. 96, Issue 8 https://doi.org/10.1103/physrevb.96.085407	journal	August 2017
Design of ultrathin Pt-Mo-Ni nanowire catalysts for ethanol electrooxidation Mao, Junjie; Chen, Wenxing; He, Dongsheng Science Advances, Vol. 3, Issue 8 https://doi.org/10.1126/sciadv.1603068	journal	August 2017
Surface-modulated palladium-nickel icosahedra as high-performance non-platinum oxygen reduction electrocatalysts Feng, Yonggang; Shao, Qi; Ji, Yujin Science Advances, Vol. 4, Issue 7 https://doi.org/10.1126/sciadv.aap8817	journal	July 2018
Semiconductor nanowire plasmonic lasers Li, Chun; Liu, Zhen; Chen, Jie Nanophotonics, Vol. 8, Issue 12 https://doi.org/10.1515/nanoph-2019-0206	journal	October 2019
Annealing Behaviour of Pt and PtNi Nanowires for Proton Exchange Membrane Fuel Cells Mardle, Peter; Du, Shangfeng Materials, Vol. 11, Issue 8 https://doi.org/10.3390/ma11081473	journal	August 2018

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