Concealed d -wave pairs in the s ± condensate of iron-based superconductors
Abstract
A central question in iron-based superconductivity is the mechanism by which the paired electrons minimize their strong mutual Coulomb repulsion. In most unconventional superconductors, Coulomb repulsion is minimized through the formation of higher angular momentum Cooper pairs, with Fermi surface nodes in the pair wavefunction. The apparent absence of such nodes in the iron-based superconductors has led to a belief they form an s-wave (s±) singlet state, which changes sign between the electron and hole pockets. However, the multiorbital nature of these systems opens an alternative possibility. In this paper, we propose a new class of s± state containing a condensate of d-wave Cooper pairs, concealed by their entanglement with the iron orbitals. By combining the d-wave (L=2) motion of the pairs with the internal angular momenta I =2 of the iron orbitals to make a singlet (J =L+I =0), an s± superconductor with a nontrivial topology is formed. This scenario allows us to understand the development of octet nodes in potassium-doped Ba1$$-$$xKXFe2As2 as a reconfiguration of the orbital and internal angular momentum into a high spin (J =L+I =4) state; the reverse transition under pressure into a fully gapped state can then be interpreted as a return to the low-spin singlet. Finally, the formation of orbitally entangled pairs is predicted to give rise to a shift in the orbital content at the Fermi surface, which can be tested via laser-based angle-resolved photoemission spectroscopy.
- Authors:
-
- Center for Materials Theory, Department of Physics and Astronomy, Rutgers University, Piscataway, NJ 08854,
- Center for Materials Theory, Department of Physics and Astronomy, Rutgers University, Piscataway, NJ 08854,, Department of Physics, Royal Holloway University of London, Egham TW20 0EX, United Kingdom,
- Institute for Theory of Condensed Matter, Karlsruhe Institute of Technology, 76131 Karlsruhe, Germany,, DFG Center for Functional Nanostructures, Karlsruhe Institute of Technology, 76128 Karlsruhe, Germany
- Publication Date:
- Research Org.:
- Rutgers Univ., Piscataway, NJ (United States)
- Sponsoring Org.:
- USDOE Office of Science (SC), Basic Energy Sciences (BES)
- OSTI Identifier:
- 1250546
- Alternate Identifier(s):
- OSTI ID: 1347954
- Grant/Contract Number:
- FG02-99ER45790
- Resource Type:
- Published Article
- Journal Name:
- Proceedings of the National Academy of Sciences of the United States of America
- Additional Journal Information:
- Journal Name: Proceedings of the National Academy of Sciences of the United States of America Journal Volume: 113 Journal Issue: 20; Journal ID: ISSN 0027-8424
- Publisher:
- Proceedings of the National Academy of Sciences
- Country of Publication:
- United States
- Language:
- English
- Subject:
- 75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND SUPERFLUIDITY; superconductivity; iron-based superconductors; unconventional superconductivity; strongly correlated electrons
Citation Formats
Ong, Tzen, Coleman, Piers, and Schmalian, Jörg. Concealed d -wave pairs in the s ± condensate of iron-based superconductors. United States: N. p., 2016.
Web. doi:10.1073/pnas.1523064113.
Ong, Tzen, Coleman, Piers, & Schmalian, Jörg. Concealed d -wave pairs in the s ± condensate of iron-based superconductors. United States. https://doi.org/10.1073/pnas.1523064113
Ong, Tzen, Coleman, Piers, and Schmalian, Jörg. Mon .
"Concealed d -wave pairs in the s ± condensate of iron-based superconductors". United States. https://doi.org/10.1073/pnas.1523064113.
@article{osti_1250546,
title = {Concealed d -wave pairs in the s ± condensate of iron-based superconductors},
author = {Ong, Tzen and Coleman, Piers and Schmalian, Jörg},
abstractNote = {A central question in iron-based superconductivity is the mechanism by which the paired electrons minimize their strong mutual Coulomb repulsion. In most unconventional superconductors, Coulomb repulsion is minimized through the formation of higher angular momentum Cooper pairs, with Fermi surface nodes in the pair wavefunction. The apparent absence of such nodes in the iron-based superconductors has led to a belief they form an s-wave (s±) singlet state, which changes sign between the electron and hole pockets. However, the multiorbital nature of these systems opens an alternative possibility. In this paper, we propose a new class of s± state containing a condensate of d-wave Cooper pairs, concealed by their entanglement with the iron orbitals. By combining the d-wave (L=2) motion of the pairs with the internal angular momenta I =2 of the iron orbitals to make a singlet (J =L+I =0), an s± superconductor with a nontrivial topology is formed. This scenario allows us to understand the development of octet nodes in potassium-doped Ba1$-$xKXFe2As2 as a reconfiguration of the orbital and internal angular momentum into a high spin (J =L+I =4) state; the reverse transition under pressure into a fully gapped state can then be interpreted as a return to the low-spin singlet. Finally, the formation of orbitally entangled pairs is predicted to give rise to a shift in the orbital content at the Fermi surface, which can be tested via laser-based angle-resolved photoemission spectroscopy.},
doi = {10.1073/pnas.1523064113},
journal = {Proceedings of the National Academy of Sciences of the United States of America},
number = 20,
volume = 113,
place = {United States},
year = {Mon May 02 00:00:00 EDT 2016},
month = {Mon May 02 00:00:00 EDT 2016}
}
https://doi.org/10.1073/pnas.1523064113
Web of Science
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