Mesoscopic structural phase progression in photo-excited VO2 revealed by time-resolved x-ray diffraction microscopy

Zhu, Yi; Cai, Zhonghou; Chen, Pice; Zhang, Qingteng; Highland, Matthew J.; Jung, II Woong; Walko, Donald A.; Dufresne, Eric M.; Jaewoo, Jeong; Samant, Mahesh G.; Parkin, Stuart S. P.; Freeland, John W.; Evans, Paul G.; Wen, Haidan

doi:10.1038/srep21999

Title: Mesoscopic structural phase progression in photo-excited VO₂ revealed by time-resolved x-ray diffraction microscopy

Journal Article · Fri Feb 26 04:00:00 UTC 2016 · Scientific Reports

DOI: https://doi.org/10.1038/srep21999 · OSTI ID:1245469

Zhu, Yi ^[1]; Cai, Zhonghou ^[1]; Chen, Pice ^[2]; Zhang, Qingteng ^[3]; Highland, Matthew J. ^[1]; Jung, II Woong ^[1]; Walko, Donald A. ^[1]; Dufresne, Eric M. ^[1]; Jaewoo, Jeong ^[4]; Samant, Mahesh G. ^[4]; Parkin, Stuart S. P. ^[5]; Freeland, John W. ^[1]; Evans, Paul G. ^[6]; Wen, Haidan ^[1]

Argonne National Lab. (ANL), Argonne, IL (United States)
Univ. of Wisconsin, Madison, WI (United States); Northwestern Univ., Evanston, IL (United States)
Univ. of Wisconsin, Madison, WI (United States); Argonne National Lab. (ANL), Lemont, IL (United States)
IBM Almaden Research Center, San Jose, CA (United States)
IBM Almaden Research Center, San Jose, CA (United States); Max Planck Institute for Microstructure Physics, Halle (Germany)
Univ. of Wisconsin, Madison, WI (United States)

Dynamical phase separation during a solid-solid phase transition poses a challenge for understanding the fundamental processes in correlated materials. Critical information underlying a phase transition, such as localized phase competition, is difficult to reveal by measurements that are spatially averaged over many phase seperated regions. The ability to simultanousely track the spatial and temporal evolution of such systems is essential to understanding mesoscopic processes during a phase transition. Using state-of- the-art time-resolved hard x-ray diffraction microscopy, we directly visualize the structural phase progression in a VO₂ film upon photoexcitation. Following a homogenous in-plane optical excitation, the phase transformation is initiated at discrete sites and completed by the growth of one lattice structure into the other, instead of a simultaneous isotropic lattice symmetry change. The time-dependent x-ray diffraction spatial maps show that the in-plane phase progression in laser-superheated VO₂ is via a displacive lattice transformation as a result of relaxation from an excited monoclinic phase into a rutile phase. The speed of the phase front progression is quantitatively measured, which is faster than the process driven by in-plane thermal diffusion but slower than the sound speed in VO₂. Lastly, the direct visualization of localized structural changes in the time domain opens a new avenue to study mesoscopic processes in driven systems.

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Research Organization:: Argonne National Lab. (ANL), Argonne, IL (United States)

Sponsoring Organization:: USDOE Office of Science (SC), Basic Energy Sciences (BES) (SC-22)

Grant/Contract Number:: AC02-06CH11357

OSTI ID:: 1245469

Journal Information:: Scientific Reports, Journal Name: Scientific Reports Vol. 6; ISSN 2045-2322

Publisher:: Nature Publishing GroupCopyright Statement

Country of Publication:: United States

Language:: English

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Photoinduced Strain Release and Phase Transition Dynamics of Solid-Supported Ultrathin Vanadium Dioxide He, Xing; Punpongjareorn, Napat; Liang, Weizheng Scientific Reports, Vol. 7, Issue 1 https://doi.org/10.1038/s41598-017-10217-0	journal	August 2017
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Strain Induced Orbital Dynamics Across the Metal Insulator Transition in Thin VO2/TiO2 (001) Films D’Elia, A.; Rezvani, S. J.; Cossaro, A. Journal of Superconductivity and Novel Magnetism, Vol. 33, Issue 8 https://doi.org/10.1007/s10948-019-05378-0	journal	January 2020
Ultrafast terahertz field control of electronic and structural interactions in vanadium dioxide Gray, A. X.; Hoffmann, M. C.; Jeong, J. Physical Review B, Vol. 98, Issue 4 https://doi.org/10.1103/physrevb.98.045104	journal	July 2018
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Giant impact of self-photothermal on light-induced ultrafast insulator-to-metal transition in VO ₂ nanofilms at terahertz frequency Zhai, Zhao-Hui; Chen, Si-Chao; Du, Liang-Hui Optics Express, Vol. 26, Issue 21 https://doi.org/10.1364/oe.26.028051	journal	January 2018
Ultrafast THz Field Control of Electronic and Structural Interactions in Vanadium Dioxide Gray, A. X.; Hoffmann, M. C.; Jeong, J. arXiv https://doi.org/10.48550/arxiv.1601.07490	text	January 2016
Strain induced orbital dynamics across the Metal Insulator transition in thin VO2/TiO2(001) films D'Elia, A.; Rezvani, S. J.; Cossaro, A. arXiv https://doi.org/10.48550/arxiv.2001.03890	text	January 2020

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Title: Mesoscopic structural phase progression in photo-excited VO₂ revealed by time-resolved x-ray diffraction microscopy