Multifunctional magnetoelectric materials for device applications

Ortega, N.; Kumar, Ashok; Scott, J. F.; Katiyar, Ram S.

doi:10.1088/0953-8984/27/50/504002

Title: Multifunctional magnetoelectric materials for device applications

Authors:: Ortega, N.; Kumar, Ashok; Scott, J. F.; Katiyar, Ram S.

Publication Date:: 2015-11-27

Sponsoring Org.:: USDOE Advanced Research Projects Agency - Energy (ARPA-E)

OSTI Identifier:: 1238940

Grant/Contract Number:: FG02-08ER46526

Resource Type:: Publisher's Accepted Manuscript

Journal Name:: Journal of Physics. Condensed Matter

Additional Journal Information:: Journal Name: Journal of Physics. Condensed Matter Journal Volume: 27 Journal Issue: 50; Journal ID: ISSN 0953-8984

Publisher:: IOP Publishing

Country of Publication:: United Kingdom

Language:: English

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                    Ortega, N., Kumar, Ashok, Scott, J. F., and Katiyar, Ram S. Multifunctional magnetoelectric materials for device applications.  United Kingdom: N. p., 2015. 
Web.  doi:10.1088/0953-8984/27/50/504002.

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                    Ortega, N., Kumar, Ashok, Scott, J. F., & Katiyar, Ram S. Multifunctional magnetoelectric materials for device applications.  United Kingdom.  https://doi.org/10.1088/0953-8984/27/50/504002

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                    Ortega, N., Kumar, Ashok, Scott, J. F., and Katiyar, Ram S. Fri .  
"Multifunctional magnetoelectric materials for device applications".  United Kingdom.  https://doi.org/10.1088/0953-8984/27/50/504002.

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@article{osti_1238940,

  title        = {Multifunctional magnetoelectric materials for device applications},

  author       = {Ortega, N. and Kumar, Ashok and Scott, J. F. and Katiyar, Ram S.},

  abstractNote = {},

  doi          = {10.1088/0953-8984/27/50/504002},

  journal      = {Journal of Physics. Condensed Matter},

  number       = 50,

  volume       = 27,

  place        = {United Kingdom},

  year         = {2015},

  month        = {11}

}

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Liu, Xian-Ming; Fu, Shao-Yun; Huang, Chuan-Jun
Materials Science and Engineering: B, Vol. 121, Issue 3
DOI: 10.1016/j.mseb.2005.04.009

Magnetic effects on dielectric and polarization behavior of multiferroic heterostructures
journal, February 2010

Dussan, Sandra; Kumar, Ashok; Scott, J. F.
Applied Physics Letters, Vol. 96, Issue 7
DOI: 10.1063/1.3327889

Enhanced multiferroic properties of the high-valence Pr doped BiFeO3 thin film
journal, November 2008

Yu, Benfang; Li, Meiya; Hu, Zhongqiang
Applied Physics Letters, Vol. 93, Issue 18
DOI: 10.1063/1.3020296

Magnetoelectric effect of TmMn ₂ O ₅
journal, November 1998

Uga, Masanori; Iwata, Nobuyuki; Kohn, Kay
Ferroelectrics, Vol. 219, Issue 1
DOI: 10.1080/00150199808213498

Is CdCr2S4 a multiferroic relaxor?
journal, August 2007

Catalan, Gustau; Scott, James F.
Nature, Vol. 448, Issue 7156
DOI: 10.1038/nature06156

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Room-temperature magnetoelectric multiferroic thin films and applications thereof

Patent Katiyar, Ram S ; Kuman, Ashok ; Scott, James F.

The invention provides a novel class of room-temperature, single-phase, magnetoelectric multiferroic (PbFe.sub.0.67W.sub.0.33O.sub.3).sub.x (PbZr.sub.0.53Ti.sub.0.47O.sub.3).sub.1-x (0.2.ltoreq.x.ltoreq.0.8) (PFW.sub.x-PZT.sub.1-x) thin films that exhibit high dielectric constants, high polarization, weak saturation magnetization, broad dielectric temperature peak, high-frequency dispersion, low dielectric loss and low leakage current. These properties render them to be suitable candidates for room-temperature multiferroic devices. Methods of preparation are also provided.
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Title: Multifunctional magnetoelectric materials for device applications

Citation Formats

Strain-mediated magnetoelectric coupling in BaTiO3-Co nanocomposite thin films journal, February 2008

Magnetoelectricity in piezoelectric-magnetostrictive composites journal, January 1976

Enhanced mangnetoelectric voltage in multiferroic particulate Ni0.83Co0.15Cu0.02Fe1.9O4−δ/PbZr0.52Ti0.48O3 composites – dielectric, piezoelectric and magnetic properties journal, September 2009

Large high-frequency magnetoelectric response in laminated composites of piezoelectric ceramics, rare-earth iron alloys and polymer journal, May 2004

Multiferroic magnetoelectric composite nanostructures journal, April 2010

Magnetoelectric effect of Pb(Zr,Ti)O3 rod arrays in a (Tb,Dy)Fe2∕epoxy medium journal, July 2005

Microstructure control of YMnO3 thin films on Si (100) substrates journal, September 2002

Symmetries and multiferroic properties of novel room-temperature magnetoelectrics: Lead iron tantalate – lead zirconate titanate (PFT/PZT) journal, December 2011

Dependence of breakdown field on dielectric (interelectrode) thickness in base-metal electroded multilayer capacitors journal, March 2007

A simple method for direct observation of the converse magnetoelectric effect in magnetic/ferroelectric composite thin films journal, November 2011

Trends in Electromechanical Transduction journal, July 1998

Ferroelectric transition in Y Mn O 3 from first principles journal, September 2005

Raman spectroscopy of multiferroic trigonal boracite Co 3 B 7 O 13 Cl journal, December 2007

Multiferroic composite ferroelectric-ferromagnetic films journal, December 2005

Controlling magnetism with multiferroics journal, October 2007

Observation of the Magnetically Induced Magnetoelectric Effect and Evidence for Antiferromagnetic Domains journal, October 1961

An in situ grown eutectic magnetoelectric composite material: Part 2 Physical properties journal, October 1974

Recent progress in first-principles studies of magnetoelectric multiferroics journal, June 2005

Magnetoelectric coupling in CoFe2O4∕SrRuO3∕Pb(Zr0.52Ti0.48)O3 heteroepitaxial thin film structure journal, January 2008

Strain-induced artificial multiferroicity in Pb(Zr0.53Ti0.47)O3/Pb(Fe0.66W0.33)O3 layered nanostructure at ambient temperature journal, October 2009

Insulating Ferromagnetic Spinels journal, September 1965

Magnetoelectric CoFe2O4–Pb(Zr,Ti)O3 composite thin films derived by a sol-gel process journal, March 2005

Ferroelectricity and structure in the YMnO 3 family journal, July 2001

Magnetodielectric effect in BaTiO3−LaMnO3 composites journal, July 2007

Room temperature multiferroic effects in superlattice nanocapacitors journal, December 2010

Magnetic-field-induced transition of thulium manganese oxide TmMn 2 O 5 journal, December 1997

The effects of drying temperature on the crystallization of YMnO3 thin films prepared by sol-gel method using alkoxides journal, August 2004

Low-temperature phase transition in ErMn 2 O 5 journal, December 1997

Prominent ferroelectricity of BiFeO3 thin films prepared by pulsed-laser deposition journal, November 2003

Thickness and coupling effects in bilayered multiferroic CoFe2O4/Pb(Zr0.52Ti0.48)O3 thin films journal, June 2008

Observation of strong magnetoelectric effects in Ba 0.7 Sr 0.3 TiO 3 /La 0.7 Sr 0.3 MnO 3 thin film heterostructures journal, May 2012

Magnetic structure of TbMnO 3 by neutron diffraction journal, July 2004

BiFeO3 film deposited on Si substrate buffered with La0.7Sr0.3MnO3 electrode journal, October 2006

Electric and Magnetic Low-Temperature Phase Transitions of Y b M n 2 O 5 journal, May 1996

Coupled magnetodielectric properties of laminated PbZr0.53Ti0.47O3/NiFe2O4 ceramics journal, May 2004

Influence of strain and oxygen vacancies on the magnetoelectric properties of multiferroic bismuth ferrite journal, June 2005

Colossal Magnetodielectric Effects in D y M n 2 O 5 journal, September 2004

Magnetoelectric effect in cobalt ferrite-barium titanate composites and their electrical properties journal, May 2002

Harvesting magnetic energy using extensional vibration of laminated magnetoelectric plates journal, July 2009

Multiferroic and magnetoelectric materials journal, August 2006

Memory window of highly c -axis oriented ferroelectric YMnO3 thin films journal, June 1999

Room temperature ferroelectric properties of Mn-substituted BiFeO3 thin films deposited on Pt electrodes using chemical solution deposition journal, June 2006

Near-room temperature relaxor multiferroic journal, November 2010

Magnetoelectric CoFe2O4∕Pb(Zr0.52Ti0.48)O3 double-layer thin film prepared by pulsed-laser deposition journal, January 2006

Internal friction study on CuFe2O4∕PbZr0.53Ti0.47O3 composites journal, November 2004

Multiferroic Pb(Fe0.66W0.33)0.80Ti0.20O3 thin films: A room-temperature relaxor ferroelectric and weak ferromagnetic journal, March 2008

Dielectric, ferroelectric, magnetic, and magnetoelectric properties of multiferroic laminated composites journal, December 2003

Room-temperature Multiferroic Properties of Pb(Zr0.57Ti0.43)O3-Pb(Fe0.67W0.33)O3 Solid-solution Epitaxial Thin Films journal, December 2010

Magnetic phase diagram of magnetoelectric CuFeO 2 in high magnetic fields journal, August 2009

Origin of ferroelectricity in the multiferroic barium fluorides Ba M F 4 : A first principles study journal, July 2006

Maxwell-Wagner space charge effects on the Pb(Zr,Ti)O3–CoFe2O4 multilayers journal, September 2007

Inversion-symmetry breaking in the noncollinear magnetic phase of the triangular-lattice antiferromagnet Cu Fe O 2 journal, June 2006

Structural, ferroelectric, dielectric, and magnetic properties of BiFeO3∕Pb(Zr0.5,Ti0.5)O3 multilayer films derived by chemical solution deposition journal, October 2005

Dramatically enhanced polarization in (001), (101), and (111) BiFeO3 thin films due to epitiaxial-induced transitions journal, June 2004

Large bulk polarization and regular domain structure in ceramic BiFeO3 journal, April 2007

Spin-phonon coupling in Zn Cr 2 Se 4 journal, February 2007

Large magnetoelectric coupling coefficient in poly(vinylidene fluoride-hexafluoropropylene)/Metglas laminates journal, November 2011

Spin-lattice coupling in multiferroic Pb(Fe1/2Nb1/2)O3 thin films journal, January 2009

Nanoscale ordering and multiferroic behavior in Pb ( Fe 1 / 2 Ta 1 / 2 ) O 3 journal, October 2010

The role of ferroelectric-ferromagnetic layers on the properties of superlattice-based multiferroics journal, May 2005

Dielectric, magnetic, and magnetoelectric properties of laminated PbZr0.52Ti0.48O3∕CoFe2O4 composite ceramics journal, November 2006

Magnetic-Field-Induced Electric Polarization in Multiferroic Nanostructures journal, May 2005

Revival of the magnetoelectric effect journal, April 2005

Preparation and multiferroic properties of 2-2 type CoFe2O4/Pb(Zr,Ti)O3 composite films with different structures journal, August 2014

Electric-field-switchable magnets: The case of BaNiF 4 journal, July 2006

Mechanisms of dielectric anomalies in BaMn F 4 journal, September 1977

Conductivity, dielectric behaviour and magnetoelectric effect in copper ferrite-barium titanate composites journal, August 2000

Giant room-temperature magnetoresistance in single-crystal Fe/MgO/Fe magnetic tunnel junctions journal, October 2004

Exploration of artificial multiferroic thin-film heterostructures using composition spreads journal, April 2004

Magnetoelectric Properties in Piezoelectric and Magnetostrictive Laminate Composites journal, August 2001

Ferroelectric domains in epitaxial PbZr0.65Ti0.35O3/La0.5Sr0.5CoO3 heterostructures journal, August 2010

Magnetic field induced polarization and magnetoelectric effect of Ba 0.8 Ca 0.2 TiO 3 -Ni 0.2 Cu 0.3 Zn 0.5 Fe 2 O 4 nanomultiferroic journal, May 2013

Dielectric and Magnetoelectric Characterization of CoFe2O4∕Sr0.5Ba0.5Nb2O6 Composites journal, December 2004

Multiferroic properties and dielectric relaxation of BiFeO3∕Bi3.25La0.75Ti3O12 double-layered thin films journal, June 2007

Ferroelectric BiFeO3 X-ray and neutron diffraction study journal, January 1971

Preparation and electrical properties of high-Curie temperature ferroelectrics journal, January 2009

Magneto-electric anomalies in bamnf 4 journal, November 1994

Effect of Microstructure on Magnetoelectric Properties of 0.9Pb(Zr 0.52 Ti 0.48 )O 3 –0.1Pb(Zn 1/3 Nb 2/3 )O 3 and Ni 0.8 Zn 0.2 Fe 2 O 4 Particulate Composites journal, November 2011

Strain-mediated magnetoelectric coupling in BaTiO3-Co nanocomposite thin films
journal, February 2008

Magnetoelectricity in piezoelectric-magnetostrictive composites
journal, January 1976

Enhanced mangnetoelectric voltage in multiferroic particulate Ni0.83Co0.15Cu0.02Fe1.9O4−δ/PbZr0.52Ti0.48O3 composites – dielectric, piezoelectric and magnetic properties
journal, September 2009

Large high-frequency magnetoelectric response in laminated composites of piezoelectric ceramics, rare-earth iron alloys and polymer
journal, May 2004

Multiferroic magnetoelectric composite nanostructures
journal, April 2010

Magnetoelectric effect of Pb(Zr,Ti)O3 rod arrays in a (Tb,Dy)Fe2∕epoxy medium
journal, July 2005

Microstructure control of YMnO3 thin films on Si (100) substrates
journal, September 2002

Symmetries and multiferroic properties of novel room-temperature magnetoelectrics: Lead iron tantalate – lead zirconate titanate (PFT/PZT)
journal, December 2011

Dependence of breakdown field on dielectric (interelectrode) thickness in base-metal electroded multilayer capacitors
journal, March 2007

A simple method for direct observation of the converse magnetoelectric effect in magnetic/ferroelectric composite thin films
journal, November 2011

Trends in Electromechanical Transduction
journal, July 1998

Ferroelectric transition in $Y Mn O_{3}$ from first principles
journal, September 2005

Raman spectroscopy of multiferroic trigonal boracite ${Co}_{3} B_{7} O_{13} Cl$
journal, December 2007

Multiferroic composite ferroelectric-ferromagnetic films
journal, December 2005

Controlling magnetism with multiferroics
journal, October 2007

Observation of the Magnetically Induced Magnetoelectric Effect and Evidence for Antiferromagnetic Domains
journal, October 1961

An in situ grown eutectic magnetoelectric composite material: Part 2 Physical properties
journal, October 1974

Recent progress in first-principles studies of magnetoelectric multiferroics
journal, June 2005

Magnetoelectric coupling in CoFe2O4∕SrRuO3∕Pb(Zr0.52Ti0.48)O3 heteroepitaxial thin film structure
journal, January 2008

Strain-induced artificial multiferroicity in Pb(Zr0.53Ti0.47)O3/Pb(Fe0.66W0.33)O3 layered nanostructure at ambient temperature
journal, October 2009

Insulating Ferromagnetic Spinels
journal, September 1965

Magnetoelectric CoFe2O4–Pb(Zr,Ti)O3 composite thin films derived by a sol-gel process
journal, March 2005

Ferroelectricity and structure in the YMnO ₃ family
journal, July 2001

Magnetodielectric effect in BaTiO3−LaMnO3 composites
journal, July 2007

Room temperature multiferroic effects in superlattice nanocapacitors
journal, December 2010

Magnetic-field-induced transition of thulium manganese oxide TmMn ₂ O ₅
journal, December 1997

The effects of drying temperature on the crystallization of YMnO3 thin films prepared by sol-gel method using alkoxides
journal, August 2004

Low-temperature phase transition in ErMn ₂ O ₅
journal, December 1997

Prominent ferroelectricity of BiFeO3 thin films prepared by pulsed-laser deposition
journal, November 2003

Thickness and coupling effects in bilayered multiferroic CoFe2O4/Pb(Zr0.52Ti0.48)O3 thin films
journal, June 2008

Observation of strong magnetoelectric effects in Ba _0.7 Sr _0.3 TiO ₃ /La _0.7 Sr _0.3 MnO ₃ thin film heterostructures
journal, May 2012

Magnetic structure of ${TbMnO}_{3}$ by neutron diffraction
journal, July 2004

BiFeO3 film deposited on Si substrate buffered with La0.7Sr0.3MnO3 electrode
journal, October 2006

Electric and Magnetic Low-Temperature Phase Transitions of Y b M n ₂ O ₅
journal, May 1996

Coupled magnetodielectric properties of laminated PbZr0.53Ti0.47O3/NiFe2O4 ceramics
journal, May 2004

Influence of strain and oxygen vacancies on the magnetoelectric properties of multiferroic bismuth ferrite
journal, June 2005

Colossal Magnetodielectric Effects in ${D y M n}_{2} O_{5}$
journal, September 2004

Magnetoelectric effect in cobalt ferrite-barium titanate composites and their electrical properties
journal, May 2002

Harvesting magnetic energy using extensional vibration of laminated magnetoelectric plates
journal, July 2009

Multiferroic and magnetoelectric materials
journal, August 2006

Memory window of highly c -axis oriented ferroelectric YMnO3 thin films
journal, June 1999

Room temperature ferroelectric properties of Mn-substituted BiFeO3 thin films deposited on Pt electrodes using chemical solution deposition
journal, June 2006

Near-room temperature relaxor multiferroic
journal, November 2010

Magnetoelectric CoFe2O4∕Pb(Zr0.52Ti0.48)O3 double-layer thin film prepared by pulsed-laser deposition
journal, January 2006

Internal friction study on CuFe2O4∕PbZr0.53Ti0.47O3 composites
journal, November 2004

Multiferroic Pb(Fe0.66W0.33)0.80Ti0.20O3 thin films: A room-temperature relaxor ferroelectric and weak ferromagnetic
journal, March 2008

Dielectric, ferroelectric, magnetic, and magnetoelectric properties of multiferroic laminated composites
journal, December 2003

Room-temperature Multiferroic Properties of Pb(Zr0.57Ti0.43)O3-Pb(Fe0.67W0.33)O3 Solid-solution Epitaxial Thin Films
journal, December 2010

Magnetic phase diagram of magnetoelectric ${CuFeO}_{2}$ in high magnetic fields
journal, August 2009

Origin of ferroelectricity in the multiferroic barium fluorides $Ba M F_{4}$ : A first principles study
journal, July 2006

Maxwell-Wagner space charge effects on the Pb(Zr,Ti)O3–CoFe2O4 multilayers
journal, September 2007

Inversion-symmetry breaking in the noncollinear magnetic phase of the triangular-lattice antiferromagnet $Cu Fe O_{2}$
journal, June 2006

Structural, ferroelectric, dielectric, and magnetic properties of BiFeO3∕Pb(Zr0.5,Ti0.5)O3 multilayer films derived by chemical solution deposition
journal, October 2005

Dramatically enhanced polarization in (001), (101), and (111) BiFeO3 thin films due to epitiaxial-induced transitions
journal, June 2004

Large bulk polarization and regular domain structure in ceramic BiFeO3
journal, April 2007

Spin-phonon coupling in $Zn {Cr}_{2} {Se}_{4}$
journal, February 2007

Large magnetoelectric coupling coefficient in poly(vinylidene fluoride-hexafluoropropylene)/Metglas laminates
journal, November 2011

Spin-lattice coupling in multiferroic Pb(Fe1/2Nb1/2)O3 thin films
journal, January 2009

Nanoscale ordering and multiferroic behavior in $Pb ({Fe}_{1 / 2} {Ta}_{1 / 2}) O_{3}$
journal, October 2010

The role of ferroelectric-ferromagnetic layers on the properties of superlattice-based multiferroics
journal, May 2005

Dielectric, magnetic, and magnetoelectric properties of laminated PbZr0.52Ti0.48O3∕CoFe2O4 composite ceramics
journal, November 2006

Magnetic-Field-Induced Electric Polarization in Multiferroic Nanostructures
journal, May 2005

Revival of the magnetoelectric effect
journal, April 2005

Preparation and multiferroic properties of 2-2 type CoFe2O4/Pb(Zr,Ti)O3 composite films with different structures
journal, August 2014

Electric-field-switchable magnets: The case of ${BaNiF}_{4}$
journal, July 2006

Mechanisms of dielectric anomalies in BaMn $F_{4}$
journal, September 1977

Conductivity, dielectric behaviour and magnetoelectric effect in copper ferrite-barium titanate composites
journal, August 2000

Giant room-temperature magnetoresistance in single-crystal Fe/MgO/Fe magnetic tunnel junctions
journal, October 2004

Exploration of artificial multiferroic thin-film heterostructures using composition spreads
journal, April 2004

Magnetoelectric Properties in Piezoelectric and Magnetostrictive Laminate Composites
journal, August 2001

Ferroelectric domains in epitaxial PbZr0.65Ti0.35O3/La0.5Sr0.5CoO3 heterostructures
journal, August 2010

Magnetic field induced polarization and magnetoelectric effect of Ba _0.8 Ca _0.2 TiO ₃ -Ni _0.2 Cu _0.3 Zn _0.5 Fe ₂ O ₄ nanomultiferroic
journal, May 2013

Dielectric and Magnetoelectric Characterization of CoFe2O4∕Sr0.5Ba0.5Nb2O6 Composites
journal, December 2004

Multiferroic properties and dielectric relaxation of BiFeO3∕Bi3.25La0.75Ti3O12 double-layered thin films
journal, June 2007

Ferroelectric BiFeO3 X-ray and neutron diffraction study
journal, January 1971

Preparation and electrical properties of high-Curie temperature ferroelectrics
journal, January 2009

Magneto-electric anomalies in bamnf ₄
journal, November 1994

Effect of Microstructure on Magnetoelectric Properties of 0.9Pb(Zr _0.52 Ti _0.48 )O ₃ –0.1Pb(Zn _1/3 Nb _2/3 )O ₃ and Ni _0.8 Zn _0.2 Fe ₂ O ₄ Particulate Composites
journal, November 2011

Multiferroics progress and prospects in thin films
journal, January 2007

Multiferroics: a magnetic twist for ferroelectricity
journal, January 2007