Dynamic nuclear polarization solid-state NMR in heterogeneous catalysis research
Abstract
In this study, a revolution in solid-state nuclear magnetic resonance (SSNMR) spectroscopy is taking place, attributable to the rapid development of high-field dynamic nuclear polarization (DNP), a technique yielding sensitivity improvements of 2–3 orders of magnitude. This higher sensitivity in SSNMR has already impacted materials research, and the implications of new methods on catalytic sciences are expected to be profound.
- Authors:
-
- Ames Lab., Ames, IA (United States)
- Ames Lab., Ames, IA (United States); Iowa State Univ., Ames, IA (United States)
- Publication Date:
- Research Org.:
- Ames Laboratory (AMES), Ames, IA (United States)
- Sponsoring Org.:
- USDOE Office of Science (SC), Basic Energy Sciences (BES)
- OSTI Identifier:
- 1227432
- Report Number(s):
- IS-J-8825
Journal ID: ISSN 2155-5435
- Grant/Contract Number:
- AC02-07CH11358
- Resource Type:
- Accepted Manuscript
- Journal Name:
- ACS Catalysis
- Additional Journal Information:
- Journal Name: ACS Catalysis; Journal ID: ISSN 2155-5435
- Publisher:
- American Chemical Society
- Country of Publication:
- United States
- Language:
- English
- Subject:
- 75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND SUPERFLUIDITY; solid-state NMR spectroscopy; DNP; hyperpolarization of spins; heterogeneous catalysis; surface-enhanced NMR spectroscopy
Citation Formats
Kobayashi, Takeshi, Perras, Frédéric A., Slowing, Igor I., Sadow, Aaron D., and Pruski, Marek. Dynamic nuclear polarization solid-state NMR in heterogeneous catalysis research. United States: N. p., 2015.
Web. doi:10.1021/acscatal.5b02039.
Kobayashi, Takeshi, Perras, Frédéric A., Slowing, Igor I., Sadow, Aaron D., & Pruski, Marek. Dynamic nuclear polarization solid-state NMR in heterogeneous catalysis research. United States. https://doi.org/10.1021/acscatal.5b02039
Kobayashi, Takeshi, Perras, Frédéric A., Slowing, Igor I., Sadow, Aaron D., and Pruski, Marek. Tue .
"Dynamic nuclear polarization solid-state NMR in heterogeneous catalysis research". United States. https://doi.org/10.1021/acscatal.5b02039. https://www.osti.gov/servlets/purl/1227432.
@article{osti_1227432,
title = {Dynamic nuclear polarization solid-state NMR in heterogeneous catalysis research},
author = {Kobayashi, Takeshi and Perras, Frédéric A. and Slowing, Igor I. and Sadow, Aaron D. and Pruski, Marek},
abstractNote = {In this study, a revolution in solid-state nuclear magnetic resonance (SSNMR) spectroscopy is taking place, attributable to the rapid development of high-field dynamic nuclear polarization (DNP), a technique yielding sensitivity improvements of 2–3 orders of magnitude. This higher sensitivity in SSNMR has already impacted materials research, and the implications of new methods on catalytic sciences are expected to be profound.},
doi = {10.1021/acscatal.5b02039},
journal = {ACS Catalysis},
number = ,
volume = ,
place = {United States},
year = {Tue Oct 20 00:00:00 EDT 2015},
month = {Tue Oct 20 00:00:00 EDT 2015}
}
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