Narrowband Light Detection via Internal Quantum Efficiency Manipulation of Organic Photodiodes

Armin, A.; Jansen-van Vuuren, R. D.; Kopidakis, N.; Burn, P. L.; Meredith, P.

doi:10.1038/ncomms7343

Title: Narrowband Light Detection via Internal Quantum Efficiency Manipulation of Organic Photodiodes

Journal Article · Sat Jan 31 23:00:00 EST 2015 · Nature Communications

DOI: https://doi.org/10.1038/ncomms7343 · OSTI ID:1220709

Armin, A. ^[1]; Jansen-van Vuuren, R. D. ^[1]; Kopidakis, N. ^[2]; Burn, P. L. ^[1]; Meredith, P. ^[1]

Univ. of Queensland, Brisbane (Australia). Centre for Organic Photonics & Electronics
National Renewable Energy Lab. (NREL), Golden, CO (United States)

Spectrally selective light detection is vital for full-colour and near-infrared (NIR) imaging and machine vision. This is not possible with traditional broadband-absorbing inorganic semiconductors without input filtering, and is yet to be achieved for narrowband absorbing organic semiconductors. We demonstrate the first sub-100 nm full-width-at-half-maximum visible-blind red and NIR photodetectors with state-of-the-art performance across critical response metrics. These devices are based on organic photodiodes with optically thick junctions. Paradoxically, we use broadband-absorbing organic semiconductors and utilize the electro-optical properties of the junction to create the narrowest NIR-band photoresponses yet demonstrated. In this context, these photodiodes outperform the encumbent technology (input filtered inorganic semiconductor diodes) and emerging technologies such as narrow absorber organic semiconductors or quantum nanocrystals. The design concept allows for response tuning and is generic for other spectral windows. Furthermore, it is materialagnostic and applicable to other disordered and polycrystalline semiconductors.

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Research Organization:: Energy Frontier Research Centers (EFRC) (United States). Molecularly Engineered Energy Materials (MEEM); NREL (National Renewable Energy Laboratory (NREL), Golden, CO (United States))

Sponsoring Organization:: USDOE Office of Science (SC), Basic Energy Sciences (BES) (SC-22); Australian Research Council

Grant/Contract Number:: AC36-08GO28308; SC0001342

OSTI ID:: 1220709

Report Number(s):: NREL/JA-5900-63985

Journal Information:: Nature Communications, Journal Name: Nature Communications Vol. 6

Country of Publication:: United States

Language:: English

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Self-trapped state enabled filterless narrowband photodetections in 2D layered perovskite single crystals Li, Junze; Wang, Jun; Ma, Jiaqi Nature Communications, Vol. 10, Issue 1 https://doi.org/10.1038/s41467-019-08768-z	journal	February 2019
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Revealing the working mechanism of polymer photodetectors with ultra-high external quantum efficiency Li, Lingliang; Zhang, Fujun; Wang, Wenbin Physical Chemistry Chemical Physics, Vol. 17, Issue 45 https://doi.org/10.1039/c5cp05557a	journal	January 2015
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Perovskite photodetectors with both visible-infrared dual-mode response and super-narrowband characteristics towards photo-communication encryption application Wu, Ye; Li, Xiaoming; Wei, Yi Nanoscale, Vol. 10, Issue 1 https://doi.org/10.1039/c7nr06193e	journal	January 2018
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