Diffuse Scattering from Lead-Containing Ferroelectric Perovskite Oxides
Abstract
Ferroelectric materials rely on some type of non-centrosymmetric displacement correlations to give rise to a macroscopic polarisation. These displacements can show short-range order (SRO) that is reflective of the local chemistry, and so studying it reveals important information about how the structure gives rise to the technologically useful properties. A key means of exploring this SRO is diffuse scattering. Conventional structural studies use Bragg peak intensitiesto determine the average structure. In a single crystal diffuse scattering (SCDS) experiment, the coherent scattered intensity is measured at non-integer Miller indices, and can be used to examine the population of local configurations. This is because the diffuse scattering is sensitive to two-body averages, whereas the Bragg intensity gives single-body averages. This review outlines key results of SCDS studies on several materials and explores the similarities and differences in their diffuse scattering. Random strains are considered, as are models based on a phonon-like picture or a more local-chemistry oriented picture. Limitations of the technique are discussed.
- Authors:
-
- Research School of Chemistry, Australian National University, Canberra ACT 0200, Australia
- Publication Date:
- Sponsoring Org.:
- USDOE
- OSTI Identifier:
- 1198291
- Grant/Contract Number:
- AC02-06CH11357
- Resource Type:
- Published Article
- Journal Name:
- ISRN Materials Science
- Additional Journal Information:
- Journal Name: ISRN Materials Science Journal Volume: 2013; Journal ID: ISSN 2090-6099
- Publisher:
- Hindawi Publishing Corporation
- Country of Publication:
- Country unknown/Code not available
- Language:
- English
Citation Formats
Goossens, D. J. Diffuse Scattering from Lead-Containing Ferroelectric Perovskite Oxides. Country unknown/Code not available: N. p., 2013.
Web. doi:10.1155/2013/107178.
Goossens, D. J. Diffuse Scattering from Lead-Containing Ferroelectric Perovskite Oxides. Country unknown/Code not available. https://doi.org/10.1155/2013/107178
Goossens, D. J. Sun .
"Diffuse Scattering from Lead-Containing Ferroelectric Perovskite Oxides". Country unknown/Code not available. https://doi.org/10.1155/2013/107178.
@article{osti_1198291,
title = {Diffuse Scattering from Lead-Containing Ferroelectric Perovskite Oxides},
author = {Goossens, D. J.},
abstractNote = {Ferroelectric materials rely on some type of non-centrosymmetric displacement correlations to give rise to a macroscopic polarisation. These displacements can show short-range order (SRO) that is reflective of the local chemistry, and so studying it reveals important information about how the structure gives rise to the technologically useful properties. A key means of exploring this SRO is diffuse scattering. Conventional structural studies use Bragg peak intensitiesto determine the average structure. In a single crystal diffuse scattering (SCDS) experiment, the coherent scattered intensity is measured at non-integer Miller indices, and can be used to examine the population of local configurations. This is because the diffuse scattering is sensitive to two-body averages, whereas the Bragg intensity gives single-body averages. This review outlines key results of SCDS studies on several materials and explores the similarities and differences in their diffuse scattering. Random strains are considered, as are models based on a phonon-like picture or a more local-chemistry oriented picture. Limitations of the technique are discussed.},
doi = {10.1155/2013/107178},
journal = {ISRN Materials Science},
number = ,
volume = 2013,
place = {Country unknown/Code not available},
year = {Sun Jul 07 00:00:00 EDT 2013},
month = {Sun Jul 07 00:00:00 EDT 2013}
}
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