Reply to “Comment on `Rapid chemical and topological ordering in supercooled liquid Cu46Zr54”’

Wessels, V.; Gangopadhyay, A. K.; Sahu, K. K.; Hyers, R. W.; Canepari, S. M.; Rogers, J. R.; Kramer, M. J.; Goldman, A. I.; Robinson, D.; Lee, J. W.; Morris, J. R.; Kelton, K. F.

doi:10.1103/PhysRevB.85.066102

Title: Reply to “Comment on `Rapid chemical and topological ordering in supercooled liquid Cu₄₆Zr₅₄”’

Authors:: Wessels, V.; Gangopadhyay, A. K.; Sahu, K. K.; Hyers, R. W.; Canepari, S. M.; Rogers, J. R.; Kramer, M. J.; Goldman, A. I.; Robinson, D.; Lee, J. W.; Morris, J. R.; Kelton, K. F.

Publication Date:: Fri Feb 10 00:00:00 EST 2012

Sponsoring Org.:: USDOE

OSTI Identifier:: 1099143

Resource Type:: Publisher's Accepted Manuscript

Journal Name:: Physical Review. B, Condensed Matter and Materials Physics

Additional Journal Information:: Journal Name: Physical Review. B, Condensed Matter and Materials Physics Journal Volume: 85 Journal Issue: 6; Journal ID: ISSN 1098-0121

Publisher:: American Physical Society

Country of Publication:: United States

Language:: English

Citation Formats


                    Wessels, V., Gangopadhyay, A. K., Sahu, K. K., Hyers, R. W., Canepari, S. M., Rogers, J. R., Kramer, M. J., Goldman, A. I., Robinson, D., Lee, J. W., Morris, J. R., and Kelton, K. F. Reply to “Comment on `Rapid chemical and topological ordering in supercooled liquid Cu46Zr54”’.  United States: N. p., 2012. 
Web.  doi:10.1103/PhysRevB.85.066102.

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                    Wessels, V., Gangopadhyay, A. K., Sahu, K. K., Hyers, R. W., Canepari, S. M., Rogers, J. R., Kramer, M. J., Goldman, A. I., Robinson, D., Lee, J. W., Morris, J. R., & Kelton, K. F. Reply to “Comment on `Rapid chemical and topological ordering in supercooled liquid Cu46Zr54”’.  United States.  https://doi.org/10.1103/PhysRevB.85.066102

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                    Wessels, V., Gangopadhyay, A. K., Sahu, K. K., Hyers, R. W., Canepari, S. M., Rogers, J. R., Kramer, M. J., Goldman, A. I., Robinson, D., Lee, J. W., Morris, J. R., and Kelton, K. F. Fri .  
"Reply to “Comment on `Rapid chemical and topological ordering in supercooled liquid Cu46Zr54”’".  United States.  https://doi.org/10.1103/PhysRevB.85.066102.

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@article{osti_1099143,

  title        = {Reply to “Comment on `Rapid chemical and topological ordering in supercooled liquid Cu46Zr54”’},

  author       = {Wessels, V. and Gangopadhyay, A. K. and Sahu, K. K. and Hyers, R. W. and Canepari, S. M. and Rogers, J. R. and Kramer, M. J. and Goldman, A. I. and Robinson, D. and Lee, J. W. and Morris, J. R. and Kelton, K. F.},

  abstractNote = {},

  doi          = {10.1103/PhysRevB.85.066102},

  journal      = {Physical Review. B, Condensed Matter and Materials Physics},

  number       = 6,

  volume       = 85,

  place        = {United States},

  year         = {Fri Feb 10 00:00:00 EST 2012},

  month        = {Fri Feb 10 00:00:00 EST 2012}

}

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https://doi.org/10.1103/PhysRevB.85.066102

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Rapid chemical and topological ordering in supercooled liquid Cu $_{46}$ Zr $_{54}$

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The criticisms of Harvey and Gheribi (HG) are directed towards supporting evidence for ordering in supercooled Cu46Zr54 liquid from specific heat measurements and molecular dynamics simulations, not on the direct evidence that came from x-ray diffraction studies. In this reply, we demonstrate that the unique features observed in the specific heat [Cp(T)] are not artifacts of any specific assumptions, as suggested by HG. We have furnished additional details of theMDsimulations and clarified related issues raised by HG. The basic conclusions, however, remain unchanged.
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Similar Records

Title: Reply to “Comment on `Rapid chemical and topological ordering in supercooled liquid Cu46Zr54”’

Citation Formats

Nearest-neighbor coordination and chemical ordering in multicomponent bulk metallic glasses journal, May 2007

Rapid chemical and topological ordering in supercooled liquid Cu 46 Zr 54 journal, March 2011

Microscopic origin of slow dynamics at the good glass forming composition range in Zr1−xCux metallic liquids journal, March 2010

Thermodynamics of Cu47Ti34Zr11Ni8, Zr52.5Cu17.9Ni14.6Al10Ti5 and Zr57Cu15.4Ni12.6Al10Nb5 bulk metallic glass forming alloys journal, May 2000

Relationship between structure, dynamics, and mechanical properties in metallic glass-forming alloys journal, July 2008

Effect of local structures and atomic packing on glass forming ability in CuxZr100−x metallic glasses journal, January 2010

Thermophysical Properties by a Pulse-Heating Reflectometric Technique: Niobium, 1100 to 2700 K journal, January 1999

Experimental and computer simulation determination of the structural changes occurring through the liquid–glass transition in Cu–Zr alloys journal, October 2010

Thermophysical Properties of Bulk Metallic Glass Forming Alloys in the Stable and Undercooled Liquid — A Microgravity Investigation journal, January 2001

Icosahedral Ordering in the Lennard-Jones Liquid and Glass journal, May 1988

Comment on “Rapid chemical and topological ordering in supercooled liquid Cu 46 Zr 54 ” journal, February 2012

Noncontact Measurements of Thermophysical Properties of Molybdenum at High Temperatures journal, January 2002

The total hemispherical emissivity of copper journal, January 1978

EXAFS study of amorphous Cu33Zr66 alloy journal, January 1984

Development of suitable interatomic potentials for simulation of liquid and amorphous Cu–Zr alloys journal, April 2009

Thermodynamics and kinetics of the Mg65Cu25Y10 bulk metallic glass forming liquid journal, April 1998

Supercooled liquids and the glass transition journal, March 2001

Significant Liquid Structures, vi. the Vacancy Theory of Liquids journal, April 1961

Hemispherical total emissivity and specific heat capacity of deeply undercooled Zr 41.2 Ti 13.8 Cu 12.5 Ni 10.0 Be 22.5 melts journal, June 1995

Thermodynamics, kinetics, and crystallization of Pt57.3Cu14.6Ni5.3P22.8 bulk metallic glass journal, February 2007

Thermodynamic properties of undercooled liquid metals journal, January 1984

Local order and dynamic properties of liquid and undercooled Cu x Zr 1 − x alloys by ab initio molecular dynamics journal, December 2008

Thermophysical and elastic properties of Cu50Zr50 and (Cu50Zr50)95Al5 bulk-metallic-glass-forming alloys journal, December 2006

Thermodynamics and Kinetics of Bulk Metallic Glass journal, August 2007

Thermodynamics and kinetics of the undercooled liquid and the glass transition of the Zr 41.2 Ti 13.8 Cu 12.5 Ni 10.0 Be 22.5 alloy journal, April 1995

Thermal radiation from metal surfaces journal, January 1978

Deriving thermophysical properties of liquid Nb by containerless electrostatic levitation journal, December 2002

Thermophysical and Thermal Optical Properties of Vanadium by Millisecond Calorimetry Between 300 and 1900 K journal, January 1999

Density-of-States Monte Carlo Simulation of a Binary Glass journal, June 2004

The embedded-atom method: a review of theory and applications journal, March 1993

Erratum: Rapid chemical and topological ordering in supercooled liquid Cu 46 Zr 54 [Phys. Rev. B 83 , 094116 (2011)] journal, January 2012

The influence of shear rate and temperature on the viscosity and fragility of the Zr41.2Ti13.8Cu12.5Ni10.0Be22.5 metallic-glass-forming liquid journal, May 2007

Using atomistic computer simulations to analyze x-ray diffraction data from metallic glasses journal, August 2007

Title: Reply to “Comment on `Rapid chemical and topological ordering in supercooled liquid Cu₄₆Zr₅₄”’

Nearest-neighbor coordination and chemical ordering in multicomponent bulk metallic glasses
journal, May 2007

Rapid chemical and topological ordering in supercooled liquid Cu $_{46}$ Zr $_{54}$
journal, March 2011

Microscopic origin of slow dynamics at the good glass forming composition range in Zr1−xCux metallic liquids
journal, March 2010

Thermodynamics of Cu47Ti34Zr11Ni8, Zr52.5Cu17.9Ni14.6Al10Ti5 and Zr57Cu15.4Ni12.6Al10Nb5 bulk metallic glass forming alloys
journal, May 2000

Relationship between structure, dynamics, and mechanical properties in metallic glass-forming alloys
journal, July 2008

Effect of local structures and atomic packing on glass forming ability in CuxZr100−x metallic glasses
journal, January 2010

Thermophysical Properties by a Pulse-Heating Reflectometric Technique: Niobium, 1100 to 2700 K
journal, January 1999

Experimental and computer simulation determination of the structural changes occurring through the liquid–glass transition in Cu–Zr alloys
journal, October 2010

Thermophysical Properties of Bulk Metallic Glass Forming Alloys in the Stable and Undercooled Liquid — A Microgravity Investigation
journal, January 2001

Icosahedral Ordering in the Lennard-Jones Liquid and Glass
journal, May 1988

Comment on “Rapid chemical and topological ordering in supercooled liquid Cu $_{46}$ Zr $_{54}$ ”
journal, February 2012

Noncontact Measurements of Thermophysical Properties of Molybdenum at High Temperatures
journal, January 2002

The total hemispherical emissivity of copper
journal, January 1978

EXAFS study of amorphous Cu33Zr66 alloy
journal, January 1984

Development of suitable interatomic potentials for simulation of liquid and amorphous Cu–Zr alloys
journal, April 2009

Thermodynamics and kinetics of the Mg65Cu25Y10 bulk metallic glass forming liquid
journal, April 1998

Supercooled liquids and the glass transition
journal, March 2001

Significant Liquid Structures, vi. the Vacancy Theory of Liquids
journal, April 1961

Hemispherical total emissivity and specific heat capacity of deeply undercooled Zr _41.2 Ti _13.8 Cu _12.5 Ni _10.0 Be _22.5 melts
journal, June 1995

Thermodynamics, kinetics, and crystallization of Pt57.3Cu14.6Ni5.3P22.8 bulk metallic glass
journal, February 2007

Thermodynamic properties of undercooled liquid metals
journal, January 1984

Local order and dynamic properties of liquid and undercooled ${Cu}_{x} {Zr}_{1 - x}$ alloys by ab initio molecular dynamics
journal, December 2008

Thermophysical and elastic properties of Cu50Zr50 and (Cu50Zr50)95Al5 bulk-metallic-glass-forming alloys
journal, December 2006

Thermodynamics and Kinetics of Bulk Metallic Glass
journal, August 2007

Thermodynamics and kinetics of the undercooled liquid and the glass transition of the Zr _41.2 Ti _13.8 Cu _12.5 Ni _10.0 Be _22.5 alloy
journal, April 1995

Thermal radiation from metal surfaces
journal, January 1978

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journal, December 2002

Thermophysical and Thermal Optical Properties of Vanadium by Millisecond Calorimetry Between 300 and 1900 K
journal, January 1999

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journal, June 2004

The embedded-atom method: a review of theory and applications
journal, March 1993

Erratum: Rapid chemical and topological ordering in supercooled liquid Cu $_{46}$ Zr $_{54}$ [Phys. Rev. B 83 , 094116 (2011)]
journal, January 2012

The influence of shear rate and temperature on the viscosity and fragility of the Zr41.2Ti13.8Cu12.5Ni10.0Be22.5 metallic-glass-forming liquid
journal, May 2007

Using atomistic computer simulations to analyze x-ray diffraction data from metallic glasses
journal, August 2007