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Ion energy dependence of atomic bonding state in CN-molecular negative ion beam deposition

Abstract

We have investigated CN negative-ion beam deposited films with respect dependencies of a nitrogen atom content and interatomic bonding state upon the ion energy. The CN negative ions extracted from a sputter-type negative ion source were deposited on a silicon substrate n-Si(100) at various ion energies in a range 25 - 500 eV. The film with a maximum nitrogen content was obtained at an ion energy of 75 eV, and its N/C ratio was evaluated to be 0.60 from RBS spectroscopy. From X-ray Photoelectron Spectroscopy (XPS) analysis, nitrogen atoms in the film were found to be mostly combined with carbon atoms, dominantly in bonding states C=N and C{identical_to}N. The C-N bond fraction increased with an increase in ion energy, and reached 11% of nitrogen atoms at maxim at an energy of 500 eV. In Raman spectroscopy, CN{sub x} films showed similar Raman bands to those of the diamond like carbon (DLC) film. (author)
Authors:
Yoshihara, Takaaki; Tsuji, Hiroshi; Gotoh, Yasuhito; Ishikawa, Junzo [1] 
  1. Kyoto Univ., Kyoto (Japan). Dept. of Electronic Science and Engineering
Publication Date:
Nov 01, 1998
Product Type:
Conference
Report Number:
CONF-981172-
Reference Number:
SCA: 665200; PA: JPN-99:011186; EDB-99:067548; SN: 99002110629
Resource Relation:
Conference: BEAMS 1998: 9. symposium on beam engineering of advanced material syntheses, Tokyo (Japan), 25-26 Nov 1998; Other Information: PBD: Nov 1998; Related Information: Is Part Of Proceedings of the ninth symposium on beam engineering of advanced material syntheses; Ishikawa, Junzo [ed.] [Kyoto Univ., Kyoto (Japan)]; PB: 195 p.; Dai-9-kai ryushisen no sentanteki oyo gijutsu ni kansuru shinpojiumu
Subject:
66 PHYSICS; ION BEAMS; CYANIDES; DEPOSITION; THIN FILMS; BINDING ENERGY; ENERGY DEPENDENCE; RAMAN SPECTRA; BOND LENGTHS; PHOTOELECTRON SPECTROSCOPY
OSTI ID:
355189
Research Organizations:
The Beam Engineering Research Society of Japan, Kyoto (Japan)
Country of Origin:
Japan
Language:
Japanese
Other Identifying Numbers:
TRN: JP9911186
Submitting Site:
JPN
Size:
pp. 119-122
Announcement Date:
Jan 25, 2004

Citation Formats

Yoshihara, Takaaki, Tsuji, Hiroshi, Gotoh, Yasuhito, and Ishikawa, Junzo. Ion energy dependence of atomic bonding state in CN-molecular negative ion beam deposition. Japan: N. p., 1998. Web.
Yoshihara, Takaaki, Tsuji, Hiroshi, Gotoh, Yasuhito, & Ishikawa, Junzo. Ion energy dependence of atomic bonding state in CN-molecular negative ion beam deposition. Japan.
Yoshihara, Takaaki, Tsuji, Hiroshi, Gotoh, Yasuhito, and Ishikawa, Junzo. 1998. "Ion energy dependence of atomic bonding state in CN-molecular negative ion beam deposition." Japan.
@misc{etde_355189,
title = {Ion energy dependence of atomic bonding state in CN-molecular negative ion beam deposition}
author = {Yoshihara, Takaaki, Tsuji, Hiroshi, Gotoh, Yasuhito, and Ishikawa, Junzo}
abstractNote = {We have investigated CN negative-ion beam deposited films with respect dependencies of a nitrogen atom content and interatomic bonding state upon the ion energy. The CN negative ions extracted from a sputter-type negative ion source were deposited on a silicon substrate n-Si(100) at various ion energies in a range 25 - 500 eV. The film with a maximum nitrogen content was obtained at an ion energy of 75 eV, and its N/C ratio was evaluated to be 0.60 from RBS spectroscopy. From X-ray Photoelectron Spectroscopy (XPS) analysis, nitrogen atoms in the film were found to be mostly combined with carbon atoms, dominantly in bonding states C=N and C{identical_to}N. The C-N bond fraction increased with an increase in ion energy, and reached 11% of nitrogen atoms at maxim at an energy of 500 eV. In Raman spectroscopy, CN{sub x} films showed similar Raman bands to those of the diamond like carbon (DLC) film. (author)}
place = {Japan}
year = {1998}
month = {Nov}
}