Title: EPCAPE-PT-LANL Measurements: Wideband Integrated Bioaerosol Sensor

Abstract

Coastal cities offer a unique environment for studying aerosol-cloud interactions and the effects of urban emissions on cloud properties. As part of the Eastern Pacific Cloud Aerosol Precipitation Experiment (EPCAPE), the Partitioning Thrust by Los Alamos National Laboratory (EPCAPE-PT-LANL) was conducted. Our campaign focused on measuring the optical and chemical properties of aerosols and their interactions within marine stratocumulus clouds in La Jolla, California. EPCAPE-PT-LANL enhances the primary goals of EPCAPE through innovative observations of vapor-phase transitions between aerosols and cloud droplets, the impact of black carbon on aerosol-cloud dynamics, and the effects of cloud processing on aerosol optical properties. Instrument: Wideband Integrated Bioaerosol Sensor (Droplet Measurements Technology)Data Notes: The WIBS is an online single-particle measurement that detects FBAPs (within a size range of 0.5 - 30 microns in diameter) based on the excitation and emission wavelengths of the individual particles. Using two xenon lamps, the WIBS excites FBAPs at 280 nm and 370 nm. Their emission is detected across two wavebands of 310-400 nm and 420-650 nm. We classified the FBAPs into seven different categories (A, B, C, AB, BC, AC, and ABC) using the classification scheme in Perring et. al. (2015) [1].Averaged number concentration of FBAPs (total and bymore » category) and particles that non-fluorescent bioaerosols particles (NFBAPs). In separate files, we also present one-minute-averaged size distributions and the asymmetry factor (AF, a surrogate for shape) of all FBAPs and NFBAPs. The logarithmic bin width of the size bins are the same as the average bin width of the AOS's optical particle counter (OPC, Grimm) for the range of sizes in which they overlap (26 bins from 0.5 - 30 microns). AF of the particles ranges from 0-100 and is divided into five bins with a linear spacing at increments of 20. The smallest AF bin represents more spherical particles while the largest bin represents more rod-shaped particles.[1] Perring, A. E., et al. (2015), Airborne observations of regional variation in fluorescent aerosol across the United States, J. Geophys. Res. Atmos., 120, 1153–1170, doi:10.1002/2014JD022495.Abstract and description of the campaign can be found here : https://www.arm.gov/research/campaigns/amf2023epcape-pt-lanl.Files data_10min_WIBS_AFDist.csvHeader:- FBAP_AFDist[/cm3]_Bin_1 to Bin_5: Concentration of fluorescent bioaerosol particles in the each of 5 AF bins, measured in particles per cubic centimeter. Each bin represents a specific range of particle AF, capturing the shapes of FBAPs detected during the measurement.- NFBAP_AFDist[/cm3]_Bin_1 to Bin_5: Concentration of non-fluorescent bioaerosol particles in the each of 5 AF bins, measured in particles per cubic centimeter. Each bin represents a specific range of particle AF, capturing the shapes of NFBAPs detected during the measurement.- CVI_Flag[bool]: A boolean flag indicating whether the Counterflow Virtual Impactor (CVI) was active (true) or inactive (false) during the measurement.AF Bins:• Bin 1: 0 – 20 [unitless]• Bin 2: 21 – 40 [unitless]• Bin 3: 41 – 60 [unitless]• Bin 4: 61 – 80 [unitless]• Bin 5: 81 – 100 [unitless] Files data_10min_WIBS_Conc.csvHeader:- NumberConcentrationA[/cm3]: Number concentration of bioaerosol particles detected by fluorescence channel A, measured in particles per cubic centimeter.- NumberConcentrationB[/cm3]: Number concentration of bioaerosol particles detected by fluorescence channel B, measured in particles per cubic centimeter.- NumberConcentrationC[/cm3]: Number concentration of bioaerosol particles detected by fluorescence channel C, measured in particles per cubic centimeter.- NumberConcentrationAB[/cm3]: Combined number concentration of bioaerosol particles detected by both fluorescence channels A and B, measured in particles per cubic centimeter.- NumberConcentrationBC[/cm3]: Combined number concentration of bioaerosol particles detected by both fluorescence channels B and C, measured in particles per cubic centimeter.- NumberConcentrationAC[/cm3]: Combined number concentration of bioaerosol particles detected by both fluorescence channels A and C, measured in particles per cubic centimeter.- NumberConcentrationABC[/cm3]: Combined number concentration of bioaerosol particles detected by all three fluorescence channels A, B, and C, measured in particles per cubic centimeter.- NumberConcentrationNFBAP[/cm3]: Number concentration of non-fluorescent bioaerosol particles, measured in particles per cubic centimeter.- CVI_Flag[bool]: A boolean flag indicating whether the Counterflow Virtual Impactor (CVI) was active (true) or inactive (false) during the measurement. Files data_10min_WIBS_SizeDist.csvHeader:- FBAP_SizeDist[/cm3]_Bin_1 to FBAP_SizeDist[/cm3]_Bin_26: Number concentrations of FBAP in each of 26 size bins, measured in particles per cubic centimeter. Each bin represents a specific range of particle sizes, capturing the size distribution of FBAPs detected during the measurement.- NFBAP_SizeDist[/cm3]_Bin_1 to NFBAP_SizeDist[/cm3]_Bin_26: Number concentrations of NFBAP in each of 26 size bins, measured in particles per cubic centimeter. Similar to FBAP, each bin covers a specific range of particle sizes, detailing the size distribution of NFBAPs detected.- CVI_Flag[bool]: A boolean flag indicating whether the Counterflow Virtual Impactor (CVI) was active (true) or inactive (false) during the measurement.Size Bins:• Bin 1: 0.48 to 0.57 μm• Bin 2: 0.57 to 0.67 μm• Bin 3: 0.67 to 0.79 μm• Bin 4: 0.79 to 0.93 μm• Bin 5: 0.93 to 1.1 μm• Bin 6: 1.1 to 1.29 μm• Bin 7: 1.29 to 1.52 μm• Bin 8: 1.52 to 1.8 μm• Bin 9: 1.8 to 2.11 μm• Bin 10: 2.11 to 2.5 μm• Bin 11: 2.5 to 2.94 μm• Bin 12: 2.94 to 3.46 μm• Bin 13: 3.46 to 4.08 μm• Bin 14: 4.08 to 4.81 μm• Bin 15: 4.81 to 5.67 μm• Bin 16: 5.67 to 6.68 μm• Bin 17: 6.68 to 7.88 μm• Bin 18: 7.88 to 9.29 μm• Bin 19: 9.29 to 10.96 μm• Bin 20: 10.96 to 12.92 μm• Bin 21: 12.92 to 15.23 μm• Bin 22: 15.23 to 17.96 μm• Bin 23: 17.96 to 21.17 μm• Bin 24: 21.17 to 24.96 μm• Bin 25: 24.96 to 29.43 μm• Bin 26: 29.43 to 34.70 μm « less

Authors:

Gorkowski, Kyle ;

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Lee, James ;

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Shawon, Abu Sayeed Md ;

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• Search DOE Data Explorer for ORCID "0000-0002-9309-5701"

Farley, Ryan ;

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Franco, Nevil ;

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Benedict, Katherine ;

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• Search DOE Data Explorer for ORCID "0000-0002-0530-8835"

Dueby, Manvendra ;

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Aiken, Allison

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1. ORNL

Publication Date:

Mon Jul 01 04:00:00 UTC 2024

Other Number(s):

ARM0863

DOE Contract Number:  

AC05-00OR22725

Research Org.:

Atmospheric Radiation Measurement (ARM) Archive, Oak Ridge National Laboratory (ORNL), Oak Ridge, TN (US); ARM Data Center, Oak Ridge National Laboratory (ORNL), Oak Ridge, TN (United States)

Sponsoring Org.:

USDOE Office of Science (SC), Biological and Environmental Research (BER)

Collaborations:

PNNL, BNL, ANL, ORNL

Subject:

54 ENVIRONMENTAL SCIENCES; fluorescent bioaerosol particles

OSTI Identifier:

2382704

DOI:

https://doi.org/10.5439/2382704