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Controlling X-rays With Light

Journal Article · · Nature Physics
DOI:https://doi.org/10.1038/nphys1430· OSTI ID:986321
Ultrafast x-ray science is an exciting frontier that promises the visualization of electronic, atomic and molecular dynamics on atomic time and length scales. A largelyunexplored area of ultrafast x-ray science is the use of light to control how x-rays interact with matter. In order to extend control concepts established for long wavelengthprobes to the x-ray regime, the optical control field must drive a coherent electronic response on a timescale comparable to femtosecond core-hole lifetimes. An intense field is required to achieve this rapid response. Here an intense optical control pulse isobserved to efficiently modulate photoelectric absorption for x-rays and to create an ultrafast transparency window. We demonstrate an application of x-ray transparencyrelevant to ultrafast x-ray sources: an all-photonic temporal cross-correlation measurement of a femtosecond x-ray pulse. The ability to control x-ray/matterinteractions with light will create new opportunities at current and next-generation x-ray light sources.
Research Organization:
Ernest Orlando Lawrence Berkeley National Laboratory, Berkeley, CA (US)
Sponsoring Organization:
Advanced Light Source Division; Chemical Sciences Division; Materials Sciences Division
DOE Contract Number:
AC02-05CH11231
OSTI ID:
986321
Report Number(s):
LBNL-3819E
Journal Information:
Nature Physics, Journal Name: Nature Physics
Country of Publication:
United States
Language:
English

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