Ultraintense x-ray induced ionization, dissociation and frustrated absorption in molecular nitrogen.
Journal Article
·
· Phys. Rev. Lett.
Sequential multiple photoionization of the prototypical molecule N2 is studied with femtosecond time resolution using the Linac Coherent Light Source (LCLS). A detailed picture of intense x-ray induced ionization and dissociation dynamics is revealed, including a molecular mechanism of frustrated absorption that suppresses the formation of high charge states at short pulse durations. The inverse scaling of the average target charge state with x-ray peak brightness has possible implications for single-pulse imaging applications.
- Research Organization:
- Argonne National Lab. (ANL), Argonne, IL (United States)
- Sponsoring Organization:
- USDOE Office of Science (SC); National Science Foundation (NSF); Academy of Finland
- DOE Contract Number:
- DE-AC02-06CH11357
- OSTI ID:
- 983762
- Report Number(s):
- ANL/CSE/JA-66584; TRN: US1005375
- Journal Information:
- Phys. Rev. Lett., Vol. 104, Issue Jun. 23, 2010
- Country of Publication:
- United States
- Language:
- ENGLISH
Similar Records
Ultraintense X-Ray Induced Ionization, Dissociation, and Frustrated Absorption in Molecular Nitrogen
Rate equations for nitrogen molecules in ultrashort and intense x-ray pulses
Ultrafast Excited State Relaxation of a Metalloporphyrin Revealed by Femtosecond X-ray Absorption Spectroscopy
Journal Article
·
Fri Jun 25 00:00:00 EDT 2010
· Physical Review Letters
·
OSTI ID:983762
+17 more
Rate equations for nitrogen molecules in ultrashort and intense x-ray pulses
Journal Article
·
Wed Mar 16 00:00:00 EDT 2016
· Journal of Physics. B, Atomic, Molecular and Optical Physics
·
OSTI ID:983762
+4 more
Ultrafast Excited State Relaxation of a Metalloporphyrin Revealed by Femtosecond X-ray Absorption Spectroscopy
Journal Article
·
Wed Jul 06 00:00:00 EDT 2016
· Journal of the American Chemical Society
·
OSTI ID:983762
+9 more