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Doping Dependent Thermopower of PbTe from Boltzmann Transport

Journal Article · · Physical Review B
The thermopower of PbTe as a function of temperature and doping level is reported based on Boltzmann transport calculations using the first principles relativistic electronic structure as obtained with the Engel-Vosko generalized gradient approximation. The results are discussed in relation to experimental data. For p-type material there is an enhancement at high-doping levels due to the onset of an increased density of states starting {approx}0.2 eV below the valence band edge. This leads to agreement between the calculated thermopower and recent results on PbTe with heavy Tl doping.
Research Organization:
Oak Ridge National Laboratory (ORNL)
Sponsoring Organization:
EE USDOE - Office of Energy Efficiency and Renewable Energy (EE); SC USDOE - Office of Science (SC)
DOE Contract Number:
AC05-00OR22725
OSTI ID:
983560
Journal Information:
Physical Review B, Journal Name: Physical Review B Journal Issue: 19 Vol. 81; ISSN 1098-0121; ISSN 1550-235X
Country of Publication:
United States
Language:
English

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