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Frozen Low-Spin Interface in Ultrathin Fe Films on Cu(111)

Journal Article · · Physical Review Letters
 [1];  [1];  [2];  [1];  [1]
  1. ORNL
  2. University of Tennessee, Knoxville (UTK) & Oak Ridge National Laboratory (ORNL)
In ultrathin film systems, it is a major challenge to understand how a thickness-driven phase transition proceeds along the cross-sectional direction of the films. We use ultrathin Fe films on Cu(111) as a prototype system to demonstrate how to obtain such information using an in situ scanning tunneling microscope and the surface magneto-optical Kerr effect. The magnetization depth profile of a thickness-driven low-spin to high-spin magnetic phase transition is deduced from the experimental data, which leads us to conclude that a low-spin Fe layer at the Fe/Cu interface stays live upon the phase transition. The magnetically live low-spin phase is believed to be induced by a frozen fcc Fe layer that survives a thickness-driven fcc {yields} bcc structural transition.
Research Organization:
Oak Ridge National Laboratory (ORNL)
Sponsoring Organization:
SC USDOE - Office of Science (SC)
DOE Contract Number:
AC05-00OR22725
OSTI ID:
978027
Journal Information:
Physical Review Letters, Journal Name: Physical Review Letters Journal Issue: 2 Vol. 95; ISSN 0031-9007; ISSN PRLTAO
Country of Publication:
United States
Language:
English

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