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CoAl2O4-Fe2O3 p-n Nanocomposite Electrodes for Photoelectrochemical Cells

Journal Article · · Applied Physics Letters
DOI:https://doi.org/10.1063/1.3183585· OSTI ID:974457
CoAl{sub 2}O{sub 4}-Fe{sub 2}O{sub 3} p-n nanocomposite electrodes were deposited on Ag-coated stainless-steel substrates and annealed at 800 C. Their photoelectrochemical (PEC) properties were investigated and compared with that of p-type CoAl{sub 2}O{sub 4} films. We found that the nanocomposite electrodes exhibit much improved PEC photoresponse as compared to the reference p-type CoAl{sub 2}O{sub 4} electrodes. We speculate that the enhancement is due to the formation of a three-dimensional junction between p-type CoAl{sub 2}O{sub 4} and n-type Fe{sub 2}O{sub 3} nanoparticles, which improves electron-hole separation, thus reducing charge recombination upon light illumination.
Research Organization:
National Renewable Energy Laboratory (NREL), Golden, CO.
Sponsoring Organization:
USDOE
DOE Contract Number:
AC36-08GO28308
OSTI ID:
974457
Journal Information:
Applied Physics Letters, Journal Name: Applied Physics Letters Journal Issue: 2, July 2009 Vol. 95; ISSN APPLAB; ISSN 0003-6951
Country of Publication:
United States
Language:
English

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